6,796 research outputs found
Optical spectroscopy study of Nd(O,F)BiS2 single crystals
We present an optical spectroscopy study on F-substituted NdOBiS
superconducting single crystals grown using KCl/LiCl flux method. The
measurement reveals a simple metallic response with a relatively low screened
plasma edge near 5000 \cm. The plasma frequency is estimated to be 2.1 eV,
which is much smaller than the value expected from the first-principles
calculations for an electron doping level of x=0.5, but very close to the value
based on a doping level of 7 of itinerant electrons per Bi site as
determined by ARPES experiment. The energy scales of the interband transitions
are also well reproduced by the first-principles calculations. The results
suggest an absence of correlation effect in the compound, which essentially
rules out the exotic pairing mechanism for superconductivity or scenario based
on the strong electronic correlation effect. The study also reveals that the
system is far from a CDW instability as being widely discussed for a doping
level of x=0.5.Comment: 5 pages, 5 figure
Mott physics, sign structure, ground state wavefunction, and high-Tc superconductivity
In this article I give a pedagogical illustration of why the essential
problem of high-Tc superconductivity in the cuprates is about how an
antiferromagnetically ordered state can be turned into a short-range state by
doping. I will start with half-filling where the antiferromagnetic ground state
is accurately described by the Liang-Doucot-Anderson (LDA) wavefunction. Here
the effect of the Fermi statistics becomes completely irrelevant due to the no
double occupancy constraint. Upon doping, the statistical signs reemerge,
albeit much reduced as compared to the original Fermi statistical signs. By
precisely incorporating this altered statistical sign structure at finite
doping, the LDA ground state can be recast into a short-range antiferromagnetic
state. Superconducting phase coherence arises after the spin correlations
become short-ranged, and the superconducting phase transition is controlled by
spin excitations. I will stress that the pseudogap phenomenon naturally emerges
as a crossover between the antiferromagnetic and superconducting phases. As a
characteristic of non Fermi liquid, the mutual statistical interaction between
the spin and charge degrees of freedom will reach a maximum in a
high-temperature "strange metal phase" of the doped Mott insulator.Comment: 12 pages, 12 figure
Charge dynamics in the phase string model for high-Tc superconductors
An understanding of the anomalous charge dynamics in the high-Tc cuprates is
obtained based on a model study of doped Mott insulators. The high-temperature
optical conductivity is found to generally have a two-component structure: a
Drude like part followed by a mid-infrared band. The scattering rate associated
with the Drude part exhibits a linear-temperature dependence over a wide range
of high temperature, while the Drude term gets progressively suppressed below a
characteristic energy of magnetic origin as the system enters the pseudogap
phase. The high-energy optical conductivity shows a resonancelike feature in an
underdoped case and continuously evolves into a 1/\omega tail at higher doping,
indicating that they share the same physical origin. In particular, such a
high-energy component is closely correlated with the \omega-peak structure of
the density-density correlation function at different momenta, in systematic
consistency with exact diagonalization results based on the t-J model. The
underlying physics is attributed to the high-energy spin-charge separation in
the model, in which the "mode coupling" responsible for the anomalous charge
properties is not between the electrons and some collective mode but rather
between new charge carriers, holons, and a novel topological gauge field
controlled by spin dynamics, as the consequence of the strong short-range
electron-electron Coulomb repulsion in the doped Mott insulator.Comment: 19 pages, 13 figures; final version to appear in Phys. Rev.
Mean-Field Description of Phase String Effect in the Model
A mean-field treatment of the phase string effect in the model is
presented. Such a theory is able to unite the antiferromagnetic (AF) phase at
half-filling and metallic phase at finite doping within a single theoretical
framework. We find that the low-temperature occurrence of the AF long range
ordering (AFLRO) at half-filling and superconducting condensation in metallic
phase are all due to Bose condensations of spinons and holons, respectively, on
the top of a spin background described by bosonic resonating-valence-bond (RVB)
pairing. The fact that both spinon and holon here are bosonic objects, as the
result of the phase string effect, represents a crucial difference from the
conventional slave-boson and slave-fermion approaches. This theory also allows
an underdoped metallic regime where the Bose condensation of spinons can still
exist. Even though the AFLRO is gone here, such a regime corresponds to a
microscopic charge inhomogeneity with short-ranged spin ordering. We discuss
some characteristic experimental consequences for those different metallic
regimes. A perspective on broader issues based on the phase string theory is
also discussed.Comment: 18 pages, five figure
Magnetic Incommensurability in Doped Mott Insulator
In this paper we explore the incommensurate spatial modulation of spin-spin
correlations as the intrinsic property of the doped Mott insulator, described
by the model. We show that such an incommensurability is a direct
manifestation of the phase string effect introduced by doped holes in both one-
and two-dimensional cases. The magnetic incommensurate peaks of dynamic spin
susceptibility in momentum space are in agreement with the neutron-scattering
measurement of cuprate superconductors in both position and doping dependence.
In particular, this incommensurate structure can naturally reconcile the
neutron-scattering and NMR experiments of cuprates.Comment: 12 pages (RevTex), five postscript figure
Stability of antiphase line defects in nanometer-sized boron-nitride cones
We investigate the stability of boron nitride conical sheets of nanometer
size, using first-principles calculations. Our results indicate that cones with
an antiphase boundary (a line defect that contains either B-B or N-N bonds) can
be more stable than those without one. We also find that doping the antiphase
boundaries with carbon can enhance their stability, leading also to the
appearance of localized states in the bandgap. Among the structures we
considered, the one with the smallest formation energy is a cone with a
carbon-modified antiphase boundary that presents a spin splitting of about 0.5
eV at the Fermi level.Comment: 5 two-column pages with 2 figures Accepted for publication in
Physical Review B (vol 70, 15 Nov.
3,3,6,6-Tetrakis(hydroxymethyl)-1,2,4,5-tetrazinane tetrahydrate
In the title compound, C6H16N4O4·4H2O, the tetrazinane molecule lies across an inversion centre. The tetrazinane ring adopts a chair conformation, and all imino H atoms occupy axial positions. In the crystal, adjacent molecules are linked through O—H⋯O, O—H⋯N and N—H⋯O hydrogen bonds with water molecules generating a three-dimensional network
Exploring the action landscape with trial world-lines
The Hamilton action principle, also known as the principle of least action,
and Lagrange equations are an integral part of advanced undergraduate
mechanics. At present, substantial efforts are ongoing to suitably incorporate
the action principle in introductory physics courses. Although the Hamilton
principle is oft stated as "the action for any nearby trial world-line is
greater than the action for the classical world-line", the landscape of action
in the space of world-lines is rarely explored. Here, for three common problems
in introductory physics - a free particle, a uniformly accelerating particle,
and a simple harmonic oscillator - we present families of trial world-lines,
characterized by a few parameters, that evolve continuously from their
respective classical world-lines. With explicit analytical expressions
available for the action, they permit a graphical visualization of the action
landscape in the space of nearby world-lines. Although these trial world-lines
form only a subset of the space of all nearby world-lines, they provide a
pedagogical tool that complements the traditional Lagrange equation approach
and is well-suited for advanced undergraduate students.Comment: 9 pages, 6 figures, significant structural revisio
Spin-Charge Separation in the Model: Magnetic and Transport Anomalies
A real spin-charge separation scheme is found based on a saddle-point state
of the model. In the one-dimensional (1D) case, such a saddle-point
reproduces the correct asymptotic correlations at the strong-coupling
fixed-point of the model. In the two-dimensional (2D) case, the transverse
gauge field confining spinon and holon is shown to be gapped at {\em finite
doping} so that a spin-charge deconfinement is obtained for its first time in
2D. The gap in the gauge fluctuation disappears at half-filling limit, where a
long-range antiferromagnetic order is recovered at zero temperature and spinons
become confined. The most interesting features of spin dynamics and transport
are exhibited at finite doping where exotic {\em residual} couplings between
spin and charge degrees of freedom lead to systematic anomalies with regard to
a Fermi-liquid system. In spin dynamics, a commensurate antiferromagnetic
fluctuation with a small, doping-dependent energy scale is found, which is
characterized in momentum space by a Gaussian peak at (, ) with
a doping-dependent width (, is the doping
concentration). This commensurate magnetic fluctuation contributes a
non-Korringa behavior for the NMR spin-lattice relaxation rate. There also
exits a characteristic temperature scale below which a pseudogap behavior
appears in the spin dynamics. Furthermore, an incommensurate magnetic
fluctuation is also obtained at a {\em finite} energy regime. In transport, a
strong short-range phase interference leads to an effective holon Lagrangian
which can give rise to a series of interesting phenomena including linear-
resistivity and Hall-angle. We discuss the striking similarities of these
theoretical features with those found in the high- cuprates and give aComment: 70 pages, RevTex, hard copies of 7 figures available upon request;
minor revisions in the text and references have been made; To be published in
July 1 issue of Phys. Rev. B52, (1995
Frustration induced Raman scattering in CuGeO_3
We present experimental data for the Raman intensity in the spin-Peierls
compound CuGeO_3 and theoretical calculations from a one-dimensional frustrated
spin model. The theory is based on (a) exact diagonalization and (b) a recently
developed solitonic mean field theory. We find good agreement between the
1D-theory in the homogeneous phase and evidence for a novel dimerization of the
Raman operator in the spin-Peierls state. Finally we present evidence for a
coupling between the interchain exchange, the spin-Peierls order parameter and
the magnetic excitations along the chains.Comment: Phys. Rev. B, Rapid Comm, in Pres
- …