1,845 research outputs found

    NONLINEAR POLARIZATION SPECTROSCOPY (FREQUENCY DOMAIN) STUDIES OF EXCITED STATE PROCESSES: THE B800–850ANTENNA OF RHODOBACTER SPHAEROIDES

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    Nonlinear polarization spectroscopy in the frequency domain allows rate constant determinations of fast electronic energy and phase relaxations together with characterization of the type of line broadening. Application of this method to the B850 component of the isolated B800–850antenna ofRhodobacter sphaeroides at room temperature shows that B850 is inhomogeneously broadened, with homogeneous widths between 30 and 200 cm−1, depending on the spectral position of the subforms. The corresponding phase relaxation times are clearly in the subpicosecond range. There is also indication of an up-to-now unspecified1–5 ps energy relaxation channel per subunit

    Excited state properties of modified pigment of bacterial photosynthesis

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    Multiple Andreev reflections as a transport problem in energy space

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    We present an approach for analyzing the dc current in voltage biased quantum superconducting junctions. By separating terms from different nn-particle processes, we find that the nn-particle current can be mapped on the problem of wave transport through a potential structure with nn barriers. We discuss the relation between resonances in such structures and the subgap structures in the current-voltage characteristics. At zero temperature we find, exactly, that only processes creating real excitations contribute to the current. Our results are valid for a general SXS-junction, where the X-region is an arbitrary non-superconducting region described by an energy-dependent transfer matrix.Comment: 11 pages, 4 figures, submitted to Superlattices and Microstructure

    Regionale voedselketen : eindrapportage fase I

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    Sinds 2005 wordt door Ruraal Park en Groene Hoed gewerkt aan het opzetten van een volledige regionale keten voor versproducten in de regio Amsterdam. Ter realisatie van het regionale keten concept hebben Ruraal Park en Groene Hoed samengewerkt met verswinkel Marqt. Inmiddels is de opening van een eerste winkel in Amsterdam bewerkstelligd. Producenten zijn hiermee niet langer de uitwisselbare factor in de productieketen. Agrarische producenten zijn verenigd in een stichting, die partner is binnen een marktformule waar met name verse producten uit de regio worden aangeboden. Er is een nieuwe, stabiele productieketen van regionaal geproduceerde producten gerealiseerd. Deze rapportage beschrijft de opzet van het project ‘Regionale keten versproducten’ en beschrijft welke werkzaamheden zijn verricht. Speciale aandacht wordt geschonken aan opgedane ervaringen, lessen en inzichten die generiek en daarmee overdraagbaar zijn

    FLUORESCENCE AND CIRCULAR DICHROISM STUDIES ON THE PHYCOERYTHROCYANINS FROM THE CYANOBACTERIUM

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    Two phycoerythrocyanin (PEC) fractions have been obtained from the phycobilisomes of the cyanobac-terium Westiellopsis prolifica ARM 365. They have been characterized by absorption, fluorescence and circular dichroism spectroscopy. One of them is spectroscopically similar to a PEC trimer known from other organisms. Whereas efficient energy transfer from its violin (α-84) to the cyanin (ÎČ-84, 155) chromophores is efficient in the trimer (αÎČ it is impeded after dissociation to the monomer (α,ÎČ). A second fraction of PEC which we earlier termed PEC(X) (Maruthi Sai et al., Photochem. Photobiol. 55,119–124, 1992), exhibited the spectral properties similar to that of the α-subunit of PEC from Mastigocladus laminosus. With this highly photoactive fraction, the circular dichroism spectra of the violobilin chromophore in both photoreversible states were obtained

    Single-channel transmission in gold one-atom contacts and chains

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    We induce superconductivity by proximity effect in thin layers of gold and study the number of conduction channels which contribute to the current in one-atom contacts and atomic wires. The atomic contacts and wires are fabricated with a Scanning Tunneling Microscope. The set of transmission probabilities of the conduction channels is obtained from the analysis of the I(V)I(V) characteristic curve which is highly non-linear due to multiple Andreev reflections. In agreement with theoretical calculations we find that there is only one channel which is almost completely open.Comment: 4 pages, 2 figures. To be published in Phys. Rev. B, Rapid Communications (2003

    Transitions between "π\pi" and "0" states in superconductor -- ferromagnet -- superconductor junctions

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    Experimental and theoretical study of superconductor (S) -- ferromagnet (F) -- superconductor junctions showed that in certain range of parameters (e.g., the length of the ferromagnet dFd_F, the exchange field, EexE_{\rm ex}) the ground state of a SFS junction corresponds to superconducting phase difference π\pi or 0. The phase diagram of a SFS junction with the respect to π\pi and 0 states is investigated in this letter in Eex,dF,TE_{\rm ex}, d_{F}, T space. It is shown that the phase diagram is very sensitive to the geometry of the system, in particular, to the amount of disorder.Comment: Minor changes. References adde

    Non-equilibrium current noise in mesoscopic disordered SNS junctions

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    Current noise in superconductor-normal metal-superconductor (SNS) junctions is calculated within the scattering theory of multiple Andreev reflections (MAR). It is shown that the noise exhibits subharmonic gap singularities at eV=2Δ/neV=2\Delta/n, n=1,2,...n=1,2,... both in single-mode junctions with arbitrary transparency DD and in multi-mode disordered junctions. The subharmonic structure is superimposed with monotonic increase of the effective transferred charge q∗=SI(0)/2Iq^*=S_I(0)/2I with decreasing bias voltage. Other features of the noise include a step-like increase of q∗q^* in junctions with small DD, and a divergence SI(0)∝V−1/2S_I(0) \propto V^{-1/2} at small voltages and excess noise Sex=2eIexS_{ex} = 2eI_{ex}, where IexI_{ex} is the excess current, at large voltages, in junctions with diffusive transport.Comment: 5 page
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