465 research outputs found
Ferroelectricity induced by spin-dependent metal-ligand hybridization in BaCoGeO
We have investigated the variation of induced ferroelectric polarization
under magnetic field with various directions and magnitudes in a staggered
antiferromagnet BaCoGeO. While the ferroelectric polarization
cannot be explained by the well-accepted spin current model nor exchange
striction mechanism, we have shown that it is induced by the spin-dependent
- hybridization between the transition-metal (Co) and ligand (O) via the
spin-orbit interaction. On the basis of the correspondence between the
direction of electric polarization and the magnetic state, we have also
demonstrated the electrical control of the magnetization direction.Comment: 4 pages, 4 figure
Giant directional dichroism of terahertz light in resonance with magnetic excitations of the multiferroic oxide BaCoGeO
We propose that concurrently magnetic and ferroelectric, i.e. multiferroic,
compounds endowed with electrically-active magnetic excitations
(electromagnons) provide a key to produce large directional dichroism for long
wavelengths of light. By exploiting the control of ferroelectric polarization
and magnetization in a multiferroic oxide BaCoGeO, we demonstrate
the realization of such a directional light-switch function at terahertz
frequecies in resonance with the electromagnon absorption. Our results imply
that this hidden potential is present in a broad variety of multiferroics
Mechanisms of enhanced orbital dia- and paramagnetism: Application to the Rashba semiconductor BiTeI
We study the magnetic susceptibility of a layered semiconductor BiTeI with
giant Rashba spin splitting both theoretically and experimentally to explore
its orbital magnetism. Apart from the core contributions, a large
temperature-dependent diamagnetic susceptibility is observed when the Fermi
energy E_F is near the crossing point of the conduction bands, while the
susceptibility turns to be paramagnetic when E_F is away from it. These
features are consistent with first-principles calculations, which also predict
an enhanced orbital magnetic susceptibility with both positive and negative
signs as a function of E_F due to band (anti)crossings. Based on these
observations, we propose two mechanisms for an enhanced paramagnetic orbital
susceptibility.Comment: 4 figures; added reference
Anomalous Nernst Effect in Nonmagnetic Nodal Line Semimetal PbTaSe
PbTaSe is a unique topological material, in which the number of nodal
lines is expected to change at the structural transition between the lower
temperature/pressure "L" phase and the higher temperature/pressure "H" phase.
We report the anomalous Nernst effect attributed to the Berry curvature of
nodal lines and its change with the structural transition. In the L phase, the
Nernst coefficient () shows the step-like magnetic field dependence
reminiscent of the anomalous Nernst effect of nonmagnetic Dirac/Weyl
semimetals. By applying hydrostatic pressure, we discovered that the amplitude
of the anomalous component significantly decreases at the transition to the H
phase, which might correspond to the partial annihilation of nodal line
structures.Comment: 29 page, 14 figure
Dynamics of Multiferroic Domain Wall in Spin-Cycloidal Ferroelectric DyMnO
We report the dielectric dispersion of the giant magnetocapacitance (GMC) in
multiferroic DyMnO over a wide frequency range. The GMC is found to be
attributable not to the softened electromagnon but to the electric-field-driven
motion of multiferroic domain wall (DW). In contrast to conventional
ferroelectric DWs, the present multiferroic DW motion holds extremely high
relaxation rate of s even at low temperatures. This
mobile nature as well as the model simulation suggests that the multiferroic DW
is not atomically thin as in ferroelectrics but thick, reflecting its magnetic
origin.Comment: 4 pages, 4 figure
Giant magneto-optical response in non-magnetic semiconductor BiTeI driven by bulk Rashba spin splitting
We study the magneto-optical (MO) response of polar semiconductor BiTeI with
giant bulk Rashba spin splitting at various carrier densities. Despite being
non-magnetic, the material is found to yield a huge MO activity in the infrared
region under moderate magnetic fields (<3 T). By comparison with
first-principles calculations, we show that such an enhanced MO response is
mainly due to the intraband transitions between the Rashba-split bulk
conduction bands in BiTeI, which give rise to distinct novel features and
systematic doping dependence of the MO spectra. We further predict an even more
pronounced enhancement in the low-energy MO response and dc Hall effect near
the crossing (Dirac) point of the conduction bands
Three-dimensional bulk band dispersion in polar BiTeI with giant Rashba-type spin splitting
In layered polar semiconductor BiTeI, giant Rashba-type spin-split band
dispersions show up due to the crystal structure asymmetry and the strong
spin-orbit interaction. Here we investigate the 3-dimensional (3D) bulk band
structures of BiTeI using the bulk-sensitive -dependent soft x-ray angle
resolved photoemission spectroscopy (SX-ARPES). The obtained band structure is
shown to be well reproducible by the first-principles calculations, with huge
spin splittings of meV at the conduction-band-minimum and
valence-band-maximum located in the plane. It provides the first
direct experimental evidence of the 3D Rashba-type spin splitting in a bulk
compound.Comment: 9 pages, 4 figure
Coexistence of Ferromagnetism and Superconductivity in Noncentrosymmetric Materials with Cubic Symmetry
This is a model study for the emergence of superconductivity in
ferromagnetically ordered phases of cubic materials whose crystal structure
lacks inversion symmetry. A Ginzburg-Landau-type theory is used to find the
ferromagnetic state and to determine the coupling of magnetic order to
superconductivity. It is found that noncentrosymmetricity evokes a helical
magnetic phase. If the wavelength of the magnetic order is long enough, it
gives rise to modulations of the order parameter of superconductivity, both in
modulus and complex phase. At magnetic domain walls the nucleation of
superconductivity is found to be suppressed as compared to the interior of
ferromagnetic domains.Comment: 5 pages, 2 figure
Strongly spin-orbit coupled two-dimensional electron gas emerging near the surface of polar semiconductors
We investigate the two-dimensional (2D) highly spin-polarized electron
accumulation layers commonly appearing near the surface of n-type polar
semiconductors BiTeX (X = I, Br, and Cl) by angular-resolved photoemission
spectroscopy. Due to the polarity and the strong spin-orbit interaction built
in the bulk atomic configurations, the quantized conduction-band subbands show
giant Rashba-type spin-splitting. The characteristic 2D confinement effect is
clearly observed also in the valence-bands down to the binding energy of 4 eV.
The X-dependent Rashba spin-orbit coupling is directly estimated from the
observed spin-split subbands, which roughly scales with the inverse of the
band-gap size in BiTeX.Comment: 15 pages 4 figure
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