149 research outputs found

    Pressure dependence of the Shubnikov-de Haas oscillation pectrum of beta''-(BEDT-TTF)4(NH4)[Cr(C2O4)3].DMF

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    The Shubnikov-de Haas (SdH) oscillation spectra of the beta''-(BEDT-TTF)4(NH4)[Cr(C2O4)\_3].DMF organic metal have been studied in pulsed magnetic fields of up to either 36 T at ambient pressure or 50 T under hydrostatic pressures of up to 1 GPa. The ambient pressure SdH oscillation spectra can be accounted for by up to six fundamental frequencies which points to a rather complex Fermi surface (FS). A noticeable pressure-induced modification of the FS topology is evidenced since the number of frequencies observed in the spectra progressively decreases as the pressure increases. Above 0.8 GPa, only three compensated orbits are observed, as it is the case for several other isostructural salts of the same family at ambient pressure. Contrary to other organic metals, of which the FS can be regarded as a network of orbits, no frequency combinations are observed for the studied salt, likely due to high magnetic breakdown gap values or (and) high disorder level evidenced by Dingle temperatures as large as about 7 K.Comment: To be published in European Physical Journal

    Landau quantization effects in the charge-density-wave system (Per)2M_2M(mnt)2_2 (where M=M=Au and Pt)

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    A finite transfer integral tat_a orthogonal to the conducting chains of a highly one-dimensional metal gives rise to empty and filled bands that simulate an indirect-gap semiconductor upon formation of a commensurate charge-density-wave (CDW). In contrast to semiconductors such as Ge and Si with bandgaps 1\sim 1 eV, the CDW system possesses an indirect gap with a greatly reduced energy scale, enabling moderate laboratory magnetic fields to have a major effect. The consequent variation of the thermodynamic gap with magnetic field due to Zeeman splitting and Landau quantization enables the electronic bandstructure parameters (transfer integrals, Fermi velocity) to be determined accurately. These parameters reveal the orbital quantization limit to be reached at 20\sim 20 T in (Per)2M_2M(mnt)2_2 salts, making them highly unlikely candidates for a recently-proposed cascade of field-induced charge-density wave states

    On the transport and thermodynamic properties of quasi-two-dimensional purple bronzes A0.9_{0.9}Mo6_6O17_{17} (A=Na, K)

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    We report a comparative study of the specific heat, electrical resistivity and thermal conductivity of the quasi-two-dimensional purple bronzes Na0.9_{0.9}Mo6_6O17_{17} and K0.9_{0.9}Mo6_6O17_{17}, with special emphasis on the behavior near their respective charge-density-wave transition temperatures TPT_P. The contrasting behavior of both the transport and the thermodynamic properties near TPT_P is argued to arise predominantly from the different levels of intrinsic disorder in the two systems. A significant proportion of the enhancement of the thermal conductivity above TPT_P in Na0.9_{0.9}Mo6_6O17_{17}, and to a lesser extent in K0.9_{0.9}Mo6_6O17_{17}, is attributed to the emergence of phason excitations.Comment: 8 pages, 6 figures, To appear in Physical Review

    Fermi-surface reconstruction and two-carrier model for the Hall effect in YBa2Cu4O8

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    Pulsed field measurements of the Hall resistivity and magnetoresistance of underdoped YBa2Cu4O8 are analyzed self-consistently using a simple model based on coexisting electron and hole carriers. The resultant mobilities and Hall numbers are found to vary markedly with temperature. The conductivity of the hole carriers drops by one order of magnitude below 30 K, explaining the absence of quantum oscillations from these particular pockets. Meanwhile the Hall coefficient of the electron carriers becomes strongly negative below 50 K. The overall quality of the fits not only provides strong evidence for Fermi-surface reconstruction in Y-based cuprates, it also strongly constrains the type of reconstruction that might be occurring.Comment: 5 pages, 4 figures, updated after publication in Physical Review B (Rapid Communication

    Wide Range Thin-FIlm Ceramic Metal-Alloy Thermometers with Low Magnetoresistance

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    Many thermal measurements in high magnetic fields require thermometers that are sensitive over a wide temperature range, are low mass, have a rapid thermal response, and have a minimal, easily correctable magnetoresistance. Here we report the development of a new granular-metal oxide ceramic composite (cermet) for this purpose formed by co-sputtering of the metallic alloy nichrome Ni0.8_{0.8}Cr0.2_{0.2} and the insulator silcon dioxide SiO2_2. The resulting thin films are sensitive enough to be used from room temperature down to below 100 mK in magnetic fields up to at least 35 tesla

    Fermiology and electronic homogeneity of the superconducting overdoped cuprate Tl-2201 revealed by quantum oscillations

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    We report an angular quantum oscillation study of Tl_2Ba_2CuO_{6+delta} for two different doping levels (Tc = 10K and 26 K) and determine the Fermi surface size and topology in considerable detail. Our results show that Fermi liquid behavior is not confined to the edge of the superconducting dome and is robust up to at least T_c^{max}/3.5. Superconductivity is found to survive up to a larger doping p_c = 0.31 than in La_{2-x}Sr_xCuO_4. Our data imply that electronic inhomogeneity does not play a significant role in the loss of superconductivity and superfluid density in overdoped cuprates, and point towards a purely magnetic or electronic pairing mechanismComment: 4 page

    Low-Frequency Quantum Oscillations due to Strong Electron Correlations

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    The normal-state energy spectrum of the two-dimensional tt-JJ model in a homogeneous perpendicular magnetic field is investigated. The density of states at the Fermi level as a function of the inverse magnetic field 1B\frac{1}{B} reveals oscillations in the range of hole concentrations 0.08<x<0.180.08<x<0.18. The oscillations have both high- and low-frequency components. The former components are connected with large Fermi surfaces, while the latter with van Hove singularities in the Landau subbands, which traverse the Fermi level with changing BB. The singularities are related to bending the Landau subbands due to strong electron correlations. Frequencies of these components are of the same order of magnitude as quantum oscillation frequencies observed in underdoped cuprates.Comment: 10 pages, 3 figures, Proc. NSS-2013, Yalta. arXiv admin note: text overlap with arXiv:1308.056

    Wide Range Thin-Film Ceramic Metal-Alloy Thermometers with Low Magnetoresistance

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    Many thermal measurements in high magnetic fields require thermometers that are sensitive over a wide temperature range, are low mass, have a rapid thermal response, and have a minimal, easily correctable magnetoresistance. Here we report the development of a new granular-metal oxide ceramic composite (cermet) for this purpose formed by co-sputtering of the metallic alloy nichrome Ni0.8Cr0.2 and the insulator silcon dioxide SiO2. The resulting thin films are sensitive enough to be used from room temperature down to below 100 mK in magnetic fields up to at least 35 tesla
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