Towards first-principles understanding of the metal-insulator transition in fluid alkali metals

By treating the electron-ion interaction as perturbation in the first-principles Hamiltonian, we have calculated the density response functions of a fluid alkali metal to find an interesting charge instability due to anomalous electronic density fluctuations occurring at some finite wave vector {\bi Q} in a dilute fluid phase above the liquid-gas critical point. Since |{\bi Q}| is smaller than the diameter of the Fermi surface, this instability necessarily impedes the electric conduction, implying its close relevance to the metal-insulator transition in fluid alkali metals.Comment: 11 pages, 5 figure

Theory of Anisotropic Hopping Transport due to Spiral Correlations in the Spin-Glass Phase of Underdoped Cuprates

We study the in-plane resistivity anisotropy in the spin-glass phase of the high-$T_{c}$ cuprates, on the basis of holes moving in a spiral spin background. This picture follows from analysis of the extended $t-J$ model with Coulomb impurities. In the variable-range hopping regime the resistivity anisotropy is found to have a maximum value of around 90%, and it decreases with temperature, in excellent agreement with experiments in La$_{2-x}$Sr$_x$CuO$_4$. In our approach the transport anisotropy is due to the non-collinearity of the spiral spin state, rather than an intrinsic tendency of the charges to self-organize.Comment: 5 pages, 4 figures; expanded versio

Fingerprints of intrinsic phase separation: magnetically doped two-dimensional electron gas

In addition to Anderson and Mott localization, intrinsic phase separation has long been advocated as the third fundamental mechanism controlling the doping-driven metal-insulator transitions. In electronic system, where charge neutrality precludes global phase separation, it may lead to various inhomogeneous states and dramaticahttp://arxiv.org/submit/215787/metadata arXiv Submission metadatally affect transport. Here we theoretically predict the precise experimental signatures of such phase-separation-driven metal-insulator transitions. We show that anomalous transport is expected in an intermediate regime around the transition, displaying very strong temperature and magnetic field dependence, but very weak density dependence. Our predictions find striking agreement with recent experiments on Mn-doped CdTe quantum wells, a system where we identify the microscopic origin for intrinsic phase separation.Comment: 4+epsilon pages, 4 figure

Transport properties in correlated systems: An analytical model

Several studies have so far investigated transport properties of strongly correlated systems. Interesting features of these materials are the lack of resistivity saturation well beyond the Mott-Ioffe-Regel limit and the scaling of the resistivity with the hole density in underdoped cuprates. Due to the strongly correlated nature of these materials, mainly numerical techniques have been employed. A key role in this regards is thought to be played by the continuous transfer of spectral weight from coherent to incoherent states. In this paper we employ a simple analytical expression for the electronic Green's function to evaluate both quasi-particle and transport properties in correlated systems. Our analytical approach permits to enlighten the specific role of the spectral transfer due to the correlation on different features. In particular we investigate the dependence of both quasi-particle and transport scattering rate on the correlation degree and the criterion for resistivity saturation. systems.Comment: 11 pages, 8 figures. New version correcting a mistake of the previous version and added figure

Colossal electroresistance in ferromagnetic insulating state of single crystal Nd0.7_0.7Pb0.3_0.3MnO3_3

Colossal electroresistance (CER) has been observed in the ferromagnetic insulating (FMI) state of a manganite. Notably, the CER in the FMI state occurs in the absence of magnetoresistance (MR). Measurements of electroresistance (ER) and current induced resistivity switching have been performed in the ferromagnetic insulating state of a single crystal manganite of composition Nd$_0.7$Pb$_0.3$MnO$_3$ (NPMO30). The sample has a paramagnetic to ferromagnetic (Curie) transition temperature, Tc = 150 K and the ferromagnetic insulating state is realized for temperatures, T <~ 130 K. The colossal electroresistance, arising from a strongly nonlinear dependence of resistivity ($\rho$) on current density (j), attains a large value ($\approx 100$) in the ferromagnetic insulating state. The severity of this nonlinear behavior of resistivity at high current densities is progressively enhanced with decreasing temperature, resulting ultimately, in a regime of negative differential resistivity (NDR, d$\rho$/dj < 0) for temperatures <~ 25 K. Concomitant with the build-up of the ER however, is a collapse of the MR to a small value (< 20%) even in magnetic field, H = 7 T. This demonstrates that the mechanisms that give rise to ER and MR are effectively decoupled in the ferromagnetic insulating phase of manganites. We establish that, the behavior of ferromagnetic insulating phase is distinct from the ferromagnetic metallic (FMM) phase as well as the charge ordered insulating (COI) phase, which are the two commonly realized ground state phases of manganites.Comment: 24 pages (RevTeX4 preprint), 8 figures, submitted to PR

Doping Dependence of Polaron Hopping Energies in La(1-x)Ca(x)MnO(3) (0<= x<= 0.15)

Measurements of the low-frequency (f<= 100 kHz) permittivity at T<= 160 K and dc resistivity (T<= 430 K) are reported for La(1-x)Ca(x)MnO(3) (0<= x<= 0.15). Static dielectric constants are determined from the low-T limiting behavior of the permittivity. The estimated polarizability for bound holes ~ 10^{-22} cm^{-3} implies a radius comparable to the interatomic spacing, consistent with the small polaron picture established from prior transport studies near room temperature and above on nearby compositions. Relaxation peaks in the dielectric loss associated with charge-carrier hopping yield activation energies in good agreement with low-T hopping energies determined from variable-range hopping fits of the dc resistivity. The doping dependence of these energies suggests that the orthorhombic, canted antiferromagnetic ground state tends toward an insulator-metal transition that is not realized due to the formation of the ferromagnetic insulating state near Mn(4+) concentration ~ 0.13.Comment: PRB in press, 5 pages, 6 figure

Quantum-defect theory of resonant charge exchange

We apply the quantum-defect theory for $-1/R^4$ potential to study the resonant charge exchange process. We show that by taking advantage of the partial-wave-insensitive nature of the formulation, resonant charge exchange of the type of $^1$S+$^2$S can be accurately described over a wide range of energies using only three parameters, such as the \textit{gerade} and the \textit{ungerade} $s$ wave scattering lengths, and the atomic polarizability, even at energies where many partial waves contribute to the cross sections. The parameters can be determined experimentally, without having to rely on accurate potential energy surfaces, of which few exist for ion-atom systems. The theory further relates ultracold interactions to interactions at much higher temperatures.Comment: 8 pages, 7 figure

Asymptotic Expansion for the Wave Function in a one-dimensional Model of Inelastic Interaction

We consider a two-body quantum system in dimension one composed by a test particle interacting with an harmonic oscillator placed at the position $a>0$. At time zero the test particle is concentrated around the position $R_0$ with average velocity $\pm v_0$ while the oscillator is in its ground state. In a suitable scaling limit, corresponding for the test particle to a semi-classical regime with small energy exchange with the oscillator, we give a complete asymptotic expansion of the wave function of the system in both cases $R_0 <a$ and $R_0 >a$.Comment: 23 page

Transport in disordered graphene nanoribbons

We study electronic transport in graphene nanoribbons with rough edges. We first consider a model of weak disorder that corresponds to an armchair ribbon whose width randomly changes by a single unit cell size. We find that in this case, the low-temperature conductivity is governed by an effective one-dimensional hopping between segments of distinct band structure. We then provide numerical evidence and qualitative arguments that similar behavior also occurs in the limit of strong uncorrelated boundary disorder.Comment: 5 pages, 3 figures. version as published in PR

Anderson-Hubbard model with box disorder: Statistical dynamical mean-field theory investigation

Strongly correlated electrons with box disorder in high-dimensional lattices are investigated. We apply the statistical dynamical mean-field theory, which treats local correlations non-perturbatively. The incorporation of a finite lattice connectivity allows for the detection of disorder-induced localization via the probability distribution function of the local density of states. We obtain a complete paramagnetic ground state phase diagram and find correlation-induced as well as disorder-induced metal-insulator transitions. Our results qualitatively confirm predictions obtained by typical medium theory. Moreover, we find that the probability distribution function of the local density of states in the metallic phase strongly deviates from a log-normal distribution as found for the non-interacting case.Comment: 13 pages, 15 figures, published versio