Coherent Imaging Spectroscopy of a Quantum Many-Body Spin System

Quantum simulators, in which well controlled quantum systems are used to reproduce the dynamics of less understood ones, have the potential to explore physics that is inaccessible to modeling with classical computers. However, checking the results of such simulations will also become classically intractable as system sizes increase. In this work, we introduce and implement a coherent imaging spectroscopic technique to validate a quantum simulation, much as magnetic resonance imaging exposes structure in condensed matter. We use this method to determine the energy levels and interaction strengths of a fully-connected quantum many-body system. Additionally, we directly measure the size of the critical energy gap near a quantum phase transition. We expect this general technique to become an important verification tool for quantum simulators once experiments advance beyond proof-of-principle demonstrations and exceed the resources of conventional computers

Interaction of H_2 and O_2 on platinum (111)

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Realization of a Decoherence-free, Optimally Distinguishable Mesoscopic Quantum Superposition

We report the realization of an entangled quantum superposition of M=12 photons by a high gain, quantum-injected optical parametric amplification. The system is found so highly resilient against decoherence to exhibit directly accessible mesoscopic interference effects at normal temperature. By modern tomographic methods the non-separability and the quantum superposition are demonstrated for the overall mesoscopic output state of the dynamic ''closed system''. The device realizes the condition conceived by Erwin Schroedinger with his 1935 paradigmatic ''Cat'' apologue, a fundamental landmark in quantum mechanics.Comment: 10 pages, 3 figure

Drivers of membrane fouling in the vanadium acetylacetonate flow battery

Vanadium acetylacetonate (V(acac)3) disproportionation electrochemistry promises a crossover-tolerant, high-voltage flow battery, but exhibits low efficiency and short cycle life. We show that membrane fouling, rather than a parasitic side reaction, dominates early performance fade. Crossover rates through porous membranes were estimated from voltage transients with an adaptive observer while cycling flow-through reactors. For 0.1M V(acac)3 and 0.3M TEABF4 in acetonitrile flowed countercurrently at 5.0cms−1 parallel to the separator, fresh Daramic 175 and Celgard 4650 afforded active-species mass-transfer coefficients of 3.8μms−1 and 7.5μms−1, respectively, which decreased and became non-Fickian as cycling progressed. At ±10mAcm−2 from 0%–20% state of charge, voltage efficiency with Celgard fell from 96% to 60% over 27 cycles. Separator replacement restored the coulombic and voltage efficiencies, which repeated their first progression. Impedance spectra from series-connected canary cells reveal that separator resistances remain stable during open-circuit exposure to charged single electrolytes, but increase under applied current or open-circuit contact with differently charged electrolytes

Non-thermalization in trapped atomic ion spin chains

Linear arrays of trapped and laser cooled atomic ions are a versatile platform for studying emergent phenomena in strongly-interacting many-body systems. Effective spins are encoded in long-lived electronic levels of each ion and made to interact through laser mediated optical dipole forces. The advantages of experiments with cold trapped ions, including high spatiotemporal resolution, decoupling from the external environment, and control over the system Hamiltonian, are used to measure quantum effects not always accessible in natural condensed matter samples. In this review we highlight recent work using trapped ions to explore a variety of non-ergodic phenomena in long-range interacting spin-models which are heralded by memory of out-of-equilibrium initial conditions. We observe long-lived memory in static magnetizations for quenched many-body localization and prethermalization, while memory is preserved in the periodic oscillations of a driven discrete time crystal state.Comment: 14 pages, 5 figures, submitted for edition of Phil. Trans. R. Soc. A on "Breakdown of ergodicity in quantum systems

Surface Incommensurate Structure in an Anisotropic Model with competing interactions on Semiinfinite Triangular Lattice

An anisotropic spin model on a triangular semiinfinite lattice with ferromagnetic nearest-neighbour interactions and one antiferromagnetic next-nearest-neighbour interaction is investigated by the cluster transfer-matrix method. A phase diagram with antiphase, ferromagnetic, incommensurate, and disordered phase is obtained. The bulk uniaxial incommensurate structure modulated in the direction of the competing interactions is found between the antiphase and the disordered phase. The incommensurate structure near the surface with free and boundary condition is studied at different temperatures. Paramagnetic damping at the surface and enhancement of the incommensurate structure in the subsurface region at high temperatures and a new subsurface incommensurate structure modulated in two directions at low temperatures are found.Comment: 13 pages, plainTex, 11 figures, paper submitted to J. Phys.

The capacity of the noisy quantum channel

An upper limit is given to the amount of quantum information that can be transmitted reliably down a noisy, decoherent quantum channel. A class of quantum error-correcting codes is presented that allow the information transmitted to attain this limit. The result is the quantum analog of Shannon's bound and code for the noisy classical channel.Comment: 19 pages, Submitted to Science. Replaced give correct references to work of Schumacher, to add a figure and an appendix, and to correct minor mistake

Entanglement of Atomic Qubits using an Optical Frequency Comb

We demonstrate the use of an optical frequency comb to coherently control and entangle atomic qubits. A train of off-resonant ultrafast laser pulses is used to efficiently and coherently transfer population between electronic and vibrational states of trapped atomic ions and implement an entangling quantum logic gate with high fidelity. This technique can be extended to the high field regime where operations can be performed faster than the trap frequency. This general approach can be applied to more complex quantum systems, such as large collections of interacting atoms or molecules.Comment: 4 pages, 5 figure