Various series expansions for the bilayer S=1/2 Heisenberg antiferromagnet

Various series expansions have been developed for the two-layer, S=1/2, square lattice Heisenberg antiferromagnet. High temperature expansions are used to calculate the temperature dependence of the susceptibility and specific heat. At T=0, Ising expansions are used to study the properties of the N\'{e}el-ordered phase, while dimer expansions are used to calculate the ground-state properties and excitation spectra of the magnetically disordered phase. The antiferromagnetic order-disorder transition point is determined to be $(J_2/J_1)_c=2.537(5)$. Quantities computed include the staggered magnetization, the susceptibility, the triplet spin-wave excitation spectra, the spin-wave velocity, and the spin-wave stiffness. We also estimates that the ratio of the intra- and inter-layer exchange constants to be $J_2/J_1\simeq 0.07$ for cuprate superconductor $YBa_2Cu_3O_{6.2}$.Comment: RevTeX, 9 figure

Monte Carlo Simulations for the Magnetic Phase Diagram of the Double Exchange Hamiltonian

We have used Monte Carlo simulation techniques to obtain the magnetic phase diagram of the double exchange Hamiltonian. We have found that the Berry's phase of the hopping amplitude has a negligible effect in the value of the magnetic critical temperature. To avoid finite size problems in our simulations we have also developed an approximated expression for the double exchange energy. This allows us to obtain the critical temperature for the ferromagnetic to paramagnetic transition more accurately. In our calculations we do not observe any strange behavior in the kinetic energy, chemical potential or electron density of states near the magnetic critical temperature. Therefore, we conclude that other effects, not included in the double exchange Hamiltonian, are needed to understand the metal-insulator transition which occurs in the manganites.Comment: 6 pages Revtex, 8 PS figure

Towards a Classification of the Effects of Disorder on Materials Properties

Many 'interesting; correlated electron materials exhibit an unusual sensitivity of measured properties to external perturbations, and in particular to imperfections in the sample being measured. It is argued that in addition to its inconvenience, this sensitivity may indicated potentially useful properties. A partial classification of causes of such sensitivity is given.Comment: Solid State Communications, in press (Proceedings of the June 2002 Williamsburg conference on Muon Spin Rotation

Landau theory of phase separation in cuprates

I discuss the problem of phase separation in cuprates from the point of view of the Landau theory of Fermi liquids. I calculate the rate of growth of unstable regions for the hydrodymanics and collisionless limit and, in presence of long range Coulomb interactions, the size of these regions. These are analytic results valid for any strength of the Landau parameters.Comment: RevteX, preprint ITP (1994

Conductance as a Function of the Temperature in the Double Exchange Model

We have used the Kubo formula to calculate the temperature dependence of the electrical conductance of the double exchange Hamiltonian. We average the conductance over an statistical ensemble of clusters, which are obtained by performing Monte Carlo simulations on the classical spin orientation of the double exchange Hamiltonian. We find that for electron concentrations bigger than 0.1, the system is metallic at all temperatures. In particular it is not observed any change in the temperature dependence of the resistivity near the magnetical critical temperature. The calculated resistivity near $T_c$ is around ten times smaller than the experimental value. We conclude that the double exchange model is not able to explain the metal to insulator transition which experimentally occurs at temperatures near the magnetic critical temperature.Comment: 6 pages, 5 figures included in the tex

T=0 Phase Diagram of the Double-Exchange Model

We present the T=0 phase diagram of the double-exchange model (ferromagnetic Kondo lattice model) for all values of the carrier concentration $n$ and Hund's couplng $J$, within dynamical mean field theory. We find that depending on the values of $n$ and $J$, the ground state is either a ferromagnet, a commensurate antiferromagnet or some other incommensurate phase with intermediate wave vectors . The antiferromagnetic phase is separated by first order phase boundaries and wide regimes of phase separation. The transition from the ferromagnetic phase to an incommensurate phase is second order.Comment: 4 pages, 5 figures. The analysis now includes incommensurate phases with arbitrary wave vectors. Correspondingly, the figures have been change

Dynamical mean field theory for transition temperature and optics of CMR manganites

A tight binding parametrization of local spin density functional band theory is combined with a dynamical mean field treatment of correlations to obtain a theory of the magnetic transition temperature, optical conductivity and T=0 spinwave stiffness of a minimal model for the pseudocubic metallic $CMR$ manganites such a $La_{1-X}Sr_{x}MnO_{3}$. The results indicate that previous estimates of $T_{c}$ obtained by one of us (Phys. Rev. \textbf{B61} 10738-49 (2000)) are in error, that in fact the materials are characterized by Hunds coupling $J\approx 1.5eV$, and that magnetic-order driven changes in the kinetic energy may not be the cause of the observed 'colossal' magnetoresistive and multiphase behavior in the manganites, raising questions about our present understanding of these materials.Comment: Published version; 10 pages, 9 figure

Temperature Dependence of Low-Lying Electronic Excitations of LaMnO_3

We report on the optical properties of undoped single crystal LaMnO_3, the parent compound of the colossal magneto-resistive manganites. Near-Normal incidence reflectance measurements are reported in the frequency range of 20-50,000 cm-1 and in the temperature range 10-300 K. The optical conductivity, s_1(w), is derived by performing a Kramers-Kronig analysis of the reflectance data. The far-infrared spectrum of s_1(w) displays the infrared active optical phonons. We observe a shift of several of the phonon to high frequencies as the temperature is lowered through the Neel temperature of the sample (T_N = 137 K). The high-frequency s_1(w) is characterized by the onset of absorption near 1.5 eV. This energy has been identified as the threshold for optical transitions across the Jahn-Teller split e_g levels. The spectral weight of this feature increases in the low-temperature state. This implies a transfer of spectral weight from the UV to the visible associated with the paramagnetic to antiferromagnetic state. We discuss the results in terms of the double exchange processes that affect the optical processes in this magnetic material.Comment: 7 pages, 5 figure

Polaronic Signatures in Mid-Infrared Spectra: Prediction for LaMnO3 and CaMnO3

Hole-doped LaMnO3 and electron-doped CaMnO3 form self-trapped electronic states. The spectra of these states have been calculated using a two orbital (Mn eg Jahn-Teller) model, from which the non-adiabatic optical conductivity spectra are obtained. In both cases the optical spectrum contains weight in the gap region, whose observation will indicate the self-trapped nature of the carrier states. The predicted spectra are proportional to the concentration of the doped carriers in the dilute regime, with coefficients calculated with no further model parameters.Comment: 6 pages with 3 figures imbedde

Semiclassical approach to calculating the influence of local lattice fluctuations on electronic properties of metals

We propose a new semiclassical approach based on the dynamical mean field theory to treat the interactions of electrons with local lattice fluctuations. In this approach the classical (static) phonon modes are treated exactly whereas the quantum (dynamical) modes are expanded to second order and give rise to an effective semiclassical potential. We determine the limits of validity of the approximation, and demonstrate its usefulness by calculating the temperature dependent resistivity in the Fermi liquid to polaron crossover regime (leading to `saturation behavior') and also isotope effects on electronic properties including the spectral function, resistivity, and optical conductivity, problems beyond the scope of conventional diagrammatic perturbation theories.Comment: 11 pages, 7 figure