Dephasing of Mollow Triplet Sideband Emission of a Resonantly Driven Quantum Dot in a Microcavity

Detailed properties of resonance fluorescence from a single quantum dot in a micropillar cavity are investigated, with particular focus on emission coherence in dependence on optical driving field power and detuning. Power-dependent series over a wide range could trace characteristic Mollow triplet spectra with large Rabi splittings of $|\Omega| \leq 15$ GHz. In particular, the effect of dephasing in terms of systematic spectral broadening $\propto \Omega^2$ of the Mollow sidebands is observed as a strong fingerprint of excitation-induced dephasing. Our results are in excellent agreement with predictions of a recently presented model on phonon-dressed QD Mollow triplet emission in the cavity-QED regime

Indistinguishable photons from the resonance fluorescence of a single quantum dot in a microcavity

We demonstrate purely resonant continuous-wave optical laser excitation to coherently prepare an excitonic state of a single semiconductor quantum dot (QDs) inside a high quality pillar microcavity. As a direct proof of QD resonance fluorescence, the evolution from a single emission line to the characteristic Mollow triplet10 is observed under increasing pump power. By controlled utilization of weak coupling between the emitter and the fundamental cavity mode through Purcell-enhancement of the radiative decay, a strong suppression of pure dephasing is achieved, which reflects in close to Fourier transform-limited and highly indistinguishable photons with a visibility contrast of 90%. Our experiments reveal the model-like character of the coupled QD-microcavity system as a promising source for the generation of ideal photons at the quantum limit. From a technological perspective, the vertical cavity symmetry -- with optional dynamic tunability -- provides strongly directed light emission which appears very desirable for future integrated emitter devices.Comment: 24 pages, 6 figure

Fracture strength and Young's modulus of ZnO nanowires

The fracture strength of ZnO nanowires vertically grown on sapphire substrates was measured in tensile and bending experiments. Nanowires with diameters between 60 and 310 nm and a typical length of 2 um were manipulated with an atomic force microscopy tip mounted on a nanomanipulator inside a scanning electron microscope. The fracture strain of (7.7 +- 0.8)% measured in the bending test was found close to the theoretical limit of 10% and revealed a strength about twice as high as in the tensile test. From the tensile experiments the Young's modulus could be measured to be within 30% of that of bulk ZnO, contrary to the lower values found in literature.Comment: 5 pages, 3 figures, 1 tabl

Phonon-Assisted Incoherent Excitation of a Quantum Dot and its Emission Properties

We present a detailed study of a phonon-assisted incoherent excitation mechanism of single quantum dots. A spectrally-detuned laser couples to a quantum dot transition by mediation of acoustic phonons, whereby excitation efficiencies up to 20 % with respect to strictly resonant excitation can be achieved at T = 9 K. Laser frequency-dependent analysis of the quantum dot intensity distinctly maps the underlying acoustic phonon bath and shows good agreement with our polaron master equation theory. An analytical solution for the photoluminescence is introduced which predicts a broadband incoherent coupling process when electron-phonon scattering is in the strong phonon coupling (polaronic) regime. Additionally, we investigate the coherence properties of the emitted light and study the impact of the relevant pump and phonon bath parameters

Non-resonant dot-cavity coupling and its applications in resonant quantum dot spectroscopy

We present experimental investigations on the non-resonant dot-cavity coupling of a single quantum dot inside a micro-pillar where the dot has been resonantly excited in the s-shell, thereby avoiding the generation of additional charges in the QD and its surrounding. As a direct proof of the pure single dot-cavity system, strong photon anti-bunching is consistently observed in the autocorrelation functions of the QD and the mode emission, as well as in the cross-correlation function between the dot and mode signals. Strong Stokes and anti-Stokes-like emission is observed for energetic QD-mode detunings of up to ~100 times the QD linewidth. Furthermore, we demonstrate that non-resonant dot-cavity coupling can be utilized to directly monitor and study relevant QD s-shell properties like fine-structure splittings, emission saturation and power broadening, as well as photon statistics with negligible background contributions. Our results open a new perspective on the understanding and implementation of dot-cavity systems for single-photon sources, single and multiple quantum dot lasers, semiconductor cavity quantum electrodynamics, and their implementation, e.g. in quantum information technology.Comment: 17 pages, 4 figure

Optical readout of charge and spin in a self-assembled quantum dot in a strong magnetic field

We present a theory and experiment demonstrating optical readout of charge and spin in a single InAs/GaAs self-assembled quantum dot. By applying a magnetic field we create the filling factor 2 quantum Hall singlet phase of the charged exciton. Increasing or decreasing the magnetic field leads to electronic spin-flip transitions and increasing spin polarization. The increasing total spin of electrons appears as a manifold of closely spaced emission lines, while spin flips appear as discontinuities of emission lines. The number of multiplets and discontinuities measures the number of carriers and their spin. We present a complete analysis of the emission spectrum of a single quantum dot with N=4 electrons and a single hole, calculated and measured in magnetic fields up to 23 Tesla.Comment: 9 pages, 3 figures, submitted to Europhysics Letter