High Dynamic Range, Heterogeneous, Terahertz Quantum Cascade Lasers Featuring Thermally Tunable Frequency Comb Operation over a Broad Current Range

We report on the engineering of broadband quantum cascade lasers (QCLs) emitting at Terahertz (THz) frequencies, which exploit a heterogeneous active region scheme and have a current density dynamic range (Jdr) of 3.2, significantly larger than the state-of-the-art, over a 1.3 THz bandwidth. We demonstrate that the devised broadband lasers operate as THz optical frequency comb synthesizers, in continuous-wave, with a maximum optical output power of 4 mW (0.73 mW in the comb regime). Measurement of the intermode beatnote map reveals a clear dispersion-compensated frequency comb regime extending over a continuous 106 mA current range (current density dynamic range of 1.24), significantly broader than the state-of-the-art at similar geometries, with a corresponding emission bandwidth of ≈1.05 THz and a stable and narrow (4.15 kHz) beatnote detected with a signal-to-noise ratio of 34 dB. Analysis of the electrical and thermal beatnote tuning reveals a current-tuning coefficient ranging between 5 and 2.1 MHz/mA and a temperature-tuning coefficient of −4 MHz/K. The ability to tune the THz QCL combs over their full operating dynamic range, by temperature and current, paves the way for their use as a powerful spectroscopy tool that can provide broad frequency coverage combined with high precision spectral accuracy

Ultrafast terahertz saturable absorbers using tailored intersubband polaritons

Semiconductor heterostructures have enabled a great variety of applications ranging from GHz electronics to photonic quantum devices. While nonlinearities play a central role for cutting-edge functionality, they require strong field amplitudes owing to the weak light-matter coupling of electronic resonances of naturally occurring materials. Here, we ultrastrongly couple intersubband transitions of semiconductor quantum wells to the photonic mode of a metallic cavity in order to custom-tailor the population and polarization dynamics of intersubband cavity polaritons in the saturation regime. Two-dimensional THz spectroscopy reveals strong subcycle nonlinearities including six-wave mixing and a collapse of light-matter coupling within 900 fs. This collapse bleaches the absorption, at a peak intensity one order of magnitude lower than previous all-integrated approaches and well achievable by state-of-the-art QCLs, as demonstrated by a saturation of the structure under cw-excitation. We complement our data by a quantitative theory. Our results highlight a path towards passively mode-locked QCLs based on polaritonic saturable absorbers in a monolithic single-chip design

THz quantum cascade laser frequency combs

We demonstrate THz optical frequency comb (FC) operation based on ultra-broadband, record dynamic range Quantum Cascade Lasers (QCLs) which exploit a heterogeneous active region design to achieve low and flat chromatic dispersion at the center of the gain curve. By implementing a Gires-Tournois Interferometer (GTI), as tightly coupled at one end of the QCL cavity, we provide lithographically-independent control of the free-running coherence properties of such THz-QCL FC and attain wide dispersion compensation regions, where stable and narrow (~3 kHz linewidth) single beatnotes extend over an operation range that is significantly larger than that of dispersiondominated bare laser cavity counterparts

Terahertz Frequency Combs Exploiting an On-Chip, Solution-Processed, Graphene-Quantum Cascade Laser Coupled-Cavity.

The ability to engineer quantum-cascade-lasers (QCLs) with ultrabroad gain spectra, and with a full compensation of the group velocity dispersion, at terahertz (THz) frequencies, is key for devising monolithic and miniaturized optical frequency-comb-synthesizers (FCSs) in the far-infrared. In THz QCLs four-wave mixing, driven by intrinsic third-order susceptibility of the intersubband gain medium, self-locks the optical modes in phase, allowing stable comb operation, albeit over a restricted dynamic range (∼20% of the laser operational range). Here, we engineer miniaturized THz FCSs, comprising a heterogeneous THz QCL, integrated with a tightly coupled, on-chip, solution-processed, graphene saturable-absorber reflector that preserves phase-coherence between lasing modes, even when four-wave mixing no longer provides dispersion compensation. This enables a high-power (8 mW) FCS with over 90 optical modes, through 55% of the laser operational range. We also achieve stable injection-locking, paving the way to a number of key applications, including high-precision tunable broadband-spectroscopy and quantum-metrology

Quantum cascade laser based hybrid dual comb spectrometer

Four-wave-mixing-based quantum cascade laser frequency combs (QCL-FC) are a powerful photonic tool, driving a recent revolution in major molecular fingerprint regions, i.e. mid- and far-infrared domains. Their compact and frequency-agile design, together with their high optical power and spectral purity, promise to deliver an all-in-one source for the most challenging spectroscopic applications. Here, we demonstrate a metrological-grade hybrid dual comb spectrometer, combining the advantages of a THz QCL-FC with the accuracy and absolute frequency referencing provided by a free-standing, optically-rectified THz frequency comb. A proof-of-principle application to methanol molecular transitions is presented. The multi-heterodyne molecular spectra retrieved provide state-of-the-art results in line-center determination, achieving the same precision as currently available molecular databases. The devised setup provides a solid platform for a new generation of THz spectrometers, paving the way to more refined and sophisticated systems exploiting full phase control of QCL-FCs, or Doppler-free spectroscopic schemes

Investigation of plume dynamics during picosecond laser ablation of H13 steel using high-speed digital holography

Ablation of H13 tool steel using pulse packets with repetition rates of 400 and 1000 kHz and pulse energies of 75 and 44μJ, respectively, is investigated. A drop in ablation efficiency (defined here as the depth per pulse or μm/μJ) is shown to occur when using pulse energies of E$_{pulse}$>44μJ, accompanied by a marked difference in crater morphology. A pulsed digital holographic system is applied to image the resulting plumes, showing a persistent plume in both cases. Holographic data are used to calculate the plume absorption and subsequently the fraction of pulse energy arriving at the surface after traversing the plume for different pulse arrival times. A significant proportion of the pulse energy is shown to be absorbed in the plume for E$_{pulse}$>44μJ for pulse arrival times corresponding to > 1 MHz pulse repetition rate, shifting the interaction to a vapour-dominated ablation regime, an energetically costlier ablation mechanism.This work was collaboratively carried out under EPSRC Grant Number EP/K030884/1, as part of the EPSRC Centre for Innovative Manufacturing in Laser-based Production Processes. One of the authors acknowledges his PhD studentship by the Federal Government of Nigeria (TETFUND) in conjunction with the Federal University of Petroleum Resources Effurun (FUPRE)

Minimize friction of lubricated laser-microtextured-surfaces by tuning microholes depth

We have investigated the friction properties of lubricated laser microtextured surfaces. The microtexture consists of a square lattice of micro-holes whose diameter, depth and spacing are controlled during the laser texturing process. All surfaces have the same texture area density, but different diameter and depth of the micro-holes. We measure the coefficient of friction on a range of sliding velocities covering the range from the mixed lubrication to the hydrodynamic regime. We find that the depth and diameter of the micro-holes have a huge influence in determining the amount of friction reduction at the interface. Interestingly experiments also show that optimal micro-hole depth values, minimizing the friction in the hydrodynamic regime, are remarkably effective also in the mixed lubrication regime