26 research outputs found

    Effect of pressure on the magnetic, transport, and thermal-transport properties of the electron-doped manganite CaMn1−x_{1-x}Sbx_{x}O3_{3}

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    We have demonstrated the effect of hydrostatic pressure on magnetic and transport properties, and thermal transport properties in electron-doped manganites CaMn1−x_{1-x}Sbx_{x}O3_{3}. The substitution of Sb5+^{5+} ion for Mn 4+^{4+}site of the parent matrix causes one-electron doping with the chemical formula CaMn1−2x4+^{4+}_{1-2x}Mnx3+^{3+}_{x}Sbx5+^{5+}_{x}O3_{3} accompanied by a monotonous increase in unit cell volume as a function of xx. Upon increasing the doping level of Sb, the magnitudes of both electrical resistivity and negative Seebeck coefficient are suppressed at high temperatures, indicating the electron doping. Anomalous diamagnetic behaviors at x=0.05x=0.05 and 0.08 are clearly observed in field cooled dc magnetization. The effect of hydrostatic pressure on dc magnetization is in contrast to the chemical pressure effect due to Sb doping. The dynamical effect of ac magnetic susceptibility measurement points to the formation of the magnetically frustrated clusters such as FM clusters embedded in canted AFM matrix.Comment: 12 pages,11 figures, 3 table

    Effect of pressure on the magnetic, transport, and thermal-transport properties of the electron-doped manganite CaMn1−x_{1-x}Sbx_{x}O3_{3}

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    We have demonstrated the effect of hydrostatic pressure on magnetic and transport properties, and thermal transport properties in electron-doped manganites CaMn1−x_{1-x}Sbx_{x}O3_{3}. The substitution of Sb5+^{5+} ion for Mn 4+^{4+}site of the parent matrix causes one-electron doping with the chemical formula CaMn1−2x4+^{4+}_{1-2x}Mnx3+^{3+}_{x}Sbx5+^{5+}_{x}O3_{3} accompanied by a monotonous increase in unit cell volume as a function of xx. Upon increasing the doping level of Sb, the magnitudes of both electrical resistivity and negative Seebeck coefficient are suppressed at high temperatures, indicating the electron doping. Anomalous diamagnetic behaviors at x=0.05x=0.05 and 0.08 are clearly observed in field cooled dc magnetization. The effect of hydrostatic pressure on dc magnetization is in contrast to the chemical pressure effect due to Sb doping. The dynamical effect of ac magnetic susceptibility measurement points to the formation of the magnetically frustrated clusters such as FM clusters embedded in canted AFM matrix.Comment: 12 pages,11 figures, 3 table

    Onset Temperatures for Superconducting Fluctuations in Te-annealed FeTe1−x_{1-x}Sex_x Single Crystals: Evidence for the BCS-BEC Crossover

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    Recently, the superconductors' community has witnessed an unsettled debate regarding whether iron-based superconductors, in particular FeSe and FeSe1−x_{1-x}Sx_x, are in the Bardeen-Cooper-Shrieffer (BCS) - Bose-Einstein condensation (BEC) crossover regime. Nonetheless, one particular system, FeTe1−x_{1-x}Sex_x, has been less investigated in this regard owing to the screening of its intrinsic superconducting properties by the inevitable iron excess. Herein, the onset temperatures for superconducting fluctuations (TscfT_{scf}) are investigated by measuring the magnetoresistance (MR) of Te-annealed, high-quality FeTe1−x_{1-x}Sex_x (xx = 0.1, 0.2, 0.3, and 0.4) single crystals. The results reveal very high TscfT_{scf} values for these crystals. Particularly for xx = 0.4, TscfT_{scf} reaches approximately 40 K, which is 2.7 times larger than TcT_c. This indicates that the superconductivity of the FeTe1−x_{1-x}Sex_x system is well within the BCS-BEC crossover regime.Comment: 6 pages, 3 figures, and 1 table. to be published in JPS Conference Proceeding

    Crystal structures and superconducting properties of metallic double-chain based cuprate Pr2Ba4Cu7O15-delta

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    We demonstrated the lattice structures and the superconducting phases of metallic double-chain based cuprate Pr2Ba4Cu7O15-delta exhibiting higher Tc. After the oxygen heat treatment on citrate pyrolysis precursors, their reduction treatment followed by a quench procedure caused higher Tc samples with 26.5-30 K. The crystal structural parameters for the superconducting sample (delta = 0.81) were analyzed from the powder synchrotron X-ray diffraction data using RIETAN-FP program. The effect of magnetic field on the superconducting phase of these samples with different oxygen defects (delta =0.73, 0.81 and 0.87) was examined, for our understanding of the superconducting magnetic field-temperature phase diagram. For delta = 0.87 sample with Tc = 30 K, the resistive critical field Hc* was estimated to be 13 T at 4.2 K. The oxygen deficiency dependence on Tc,on for our samples was compared with the data of several other groups.Comment: 8 pages, 6 figure
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