18 research outputs found
Magnetic-Field-Induced 4f-Octupole in CeB6 Probed by Resonant X-ray Diffraction
CeB6, a typical Gamma_8-quartet system, exhibits a mysterious
antiferroquadrupolar ordered phase in magnetic fields, which is considered as
originating from the T_{xyz}-type magnetic octupole moment induced by the
field. By resonant x-ray diffraction in magnetic fields, we have verified that
the T_{xyz}-type octupole is indeed induced in the 4f-orbital of Ce with a
propagation vector (1/2, 1/2, 1/2), thereby supporting the theory. We observed
an asymmetric field dependence of the intensity for an electric quadrupole (E2)
resonance when the field was reversed, and extracted a field dependence of the
octupole by utilizing the interference with an electric dipole (E1) resonance.
The result is in good agreement with that of the NMR-line splitting, which
reflects the transferred hyperfine field at the Boron nucleus from the
anisotropic spin distribution of Ce with an O_{xy}-type quadrupole. The
field-reversal method used in the present study opens up the possibility of
being widely applied to other multipole ordering systems such as NpO2,
Ce_{x}La_{1-x}B_{6}, SmRu_{4}P_{12}, and so on.Comment: 5 pages, 4 figures, submitte
Elastic properties of the Non-Fermi liquid metal and the Dense Kondo semiconductor
We have investigated the elastic properties of the Ce-based filled
skutterudite antimonides CeRuSb and CeOsSb by means
of ultrasonic measurements. CeRuSb shows a slight increase around
130 K in the temperature dependence of the elastic constants ,
(-)/2 and . No apparent softening toward low
temperature due to a quadrupolar response of the 4-electronic ground state
of the Ce ion was observed at low temperatures. In contrast CeOsSb
shows a pronounced elastic softening toward low temperature in the longitudinal
as a function of temperature () below about 15 K, while a slight
elastic softening was observed in the transverse below about 1.5 K.
Furthermore, CeOsSb shows a steep decrease around a phase
transition temperature of 0.9 K in both and. The elastic
softening observed in below about 15 K cannot be explained
reasonably only by the crystalline electric field effect. It is most likely to
be responsible for the coupling between the elastic strain and the
quasiparticle band with a small energy gap in the vicinity of Fermi level. The
elastic properties and the 4 ground state of Ce ions in CeRuSb
and CeOsSb are discussed from the viewpoint of the crystalline
electric field effect and the band structure in the vicinity of Fermi level.Comment: 9 pages, 11 figures, regular pape