Charge amplification in sub-atmospheric CF4:He mixtures for directional dark matter searches

Low pressure gaseous Time Projection Chambers (TPCs) are a viable technology for directional Dark Matter (DM) searches and have the potential for exploring the parameter space below the neutrino fog [1,2]. Gases like CF4 are advantageous because they contain flourine which is predicted to have heightened elastic scattering rates with a possible Weakly Interacting Massive Particle (WIMP) DM candidate [3,4,5]. The low pressure of CF4 must be maintained, ideally lower than 100 Torr, in order to elongate potential Nuclear Recoil (NR) tracks which allows for improved directional sensitivity and NR/Electron Recoil (ER) discrimination [6]. Recent evidence suggests that He can be added to heavier gases, like CF4, without significantly affecting the length of 12C and 19F recoils due to its lower mass. Such addition of He has the advantage of improving sensitivity to lower mass WIMPs [1]. Simulations can not reliably predict operational stability in these low pressure gas mixtures and thus must be demonstrated experimentally. In this paper we investigate how the addition of He to low pressure CF4 affects the gas gain and energy resolution achieved with a single Thick Gaseous Electron Multiplier (ThGEM)

Directional dark matter readout with a novel multi-mesh ThGEM for SF6 negative ion operation

Direct searches for Weakly Interacting Massive Particle (WIMP) dark matter could greatly benefit from directional measurement of the expected induced nuclear recoils. Gas-based Time Projection Chambers (TPCs) offer potential for this, opening the possibility of measuring WIMP signals below the so-called neutrino floor but also of directional measurement of recoils induced by neutrinos from the Sun, for instance as proposed by the CYGNUS collaboration. Presented here for the first time are results from a Multi-Mesh Thick Gas Electron Multiplier (MM-ThGEM) using negative ion gases for operation with such a directional dark matter TPC. Negative ion drift gases are favoured for directionality due to their low diffusion characteristics. The multiple internal mesh structure is designed to provide a high gain amplification stage when coupled to future large area Micromegas, strip or pixel charge readout planes. Experimental results and simulations are presented of MM-ThGEM gain and functionality using low pressure pure CF4, SF6 and SF6:CF4 mixtures irradiated with alpha particles and 55Fe x-rays. The concept is found to work well, providing stable operation with gains over 103 in pure SF6

Molecular sieve vacuum swing adsorption purification and radon reduction system for gaseous dark matter and rare-event detectors

In the field of directional dark matter experiments SF6 has emerged as an ideal target gas. A critical challenge with this gas, and with other proposed gases, is the effective removal of contaminant gases. This includes radon which produce unwanted background events, but also common pollutants such as water, oxygen and nitrogen, which can capture ionisation electrons, resulting in loss of detector gas gain over time. We present here a novel molecular sieve (MS) based gas recycling system for the simultaneous removal of both radon and common pollutants from SF6. The apparatus has the additional benefit of minimising gas required in experiments and utilises a Vacuum Swing Adsorption (VSA) technique for continuous, long-term operation. The gas system's capabilities were tested with a 100 L low-pressure SF6 Time Projection Chamber (TPC) detector. For the first time, we present a newly developed low-radioactive MS type 5 Å. This material was found to emanate radon at 98% less per radon captured compared to commercial counterparts, the lowest known MS emanation at the time of writing. Consequently, the radon activity in the TPC detector was reduced, with an upper limit of less than 7.2 mBq at a 95% confidence level (C.L.). Incorporation of MS types 3 Å and 4 Å to absorb common pollutants was found successfully to mitigate against gain deterioration while recycling the target gas

Demonstration of radon removal from SF6 using molecular sieves

The gas SF6 has become of interest as a negative ion drift gas for use in directional dark matter searches. However, as for other targets in such searches, it is important that radon contamination can be removed as this provides a source of unwanted background events. In this work we demonstrate for the first time filtration of radon from SF6 gas by using a molecular sieve. Four types of sieves from Sigma-Aldrich were investigated, namely 3Å, 4Å, 5Å and 13X. A manufactured radon source was used for the tests. This was attached to a closed loop system in which gas was flowed through the filters and a specially adapted Durridge RAD7 radon detector. In these measurements, it was found that only the 5Å type was able to significantly reduce the radon concentration without absorbing the SF6 gas. The sieve was able to reduce the initial radon concentration of 3875 ± 13 Bqm−3 in SF6 gas by 87% when cooled with dry ice. The ability of the cooled 5Å molecular sieve filter to significantly reduce radon concentration from SF6 provides a promising foundation for the construction of a radon filtration setup for future ultra-sensitive SF6 gas rare-event physics experiments

Test of low radioactive molecular sieves for radon filtration in SF6 gas-based rare-event physics experiments

Type 5 Å molecular sieves (MS) have been demonstrated to remove radon from SF6 gas. This is important for ultra-sensitive SF6 gas-based directional dark matter and related rare-event physics experiments, as radon can provide a source of unwanted background events. Unfortunately, commercially available sieves intrinsically emanate radon at levels not suitable for ultra-sensitive physics experiments. A method to produce a low radioactive MS has been developed in Nihon University (NU). In this work, we explore the feasibility of the NU-developed 5 Å type MS for use in such experiments. A comparison with a commercially available Sigma-Aldrich 5 Å type MS was made. The comparison was done by calculating a parameter indicating the amount of radon intrinsically emanated by the MS per unit radon captured from SF6 gas. The measurements were made using a specially adapted DURRIDGE RAD7 radon detector. The NU-developed 5 Å MS emanated radon up to 61 ± 9% less per radon captured (2.1 ± 0.1) × 10−3, compared to the commercial Sigma-Aldrich MS (5.4 ± 0.4) × 10−3, making it a better candidate for use in a radon filtration setup for future ultra-sensitive SF6 gas based experiments

Gas gains over 104 and optimisation using 55Fe X-rays in low pressure SF6 with a novel Multi-Mesh ThGEM for directional dark matter searches

The Negative Ion Drift (NID) gas SF6 has favourable properties for track reconstruction in directional Dark Matter (DM) searches utilising low pressure gaseous Time Projection Chambers (TPCs). However, the electronegative nature of the gas means that it is more difficult to achieve significant gas gains with regular Thick Gaseous Electron Multipliers (ThGEMs). Typically, the maximum attainable gas gain in SF6 and other Negative Ion (NI) gas mixtures, previously achieved with an 55Fe X-ray source or electron beam, is on the order of 103 [1,2,3,4]; whereas electron drift gases like CF4 and similar mixtures are readily capable of reaching gas gains on the order of 104 or greater [5,9,7,8,6]. In this paper, a novel two stage Multi-Mesh ThGEM (MMThGEM) structure is presented. The MMThGEM was used to amplify charge liberated by an 55Fe X-ray source in 40 Torr of SF6. By expanding on previously demonstrated results [10], the device was pushed to its sparking limit and stable gas gains up to ˜50000 were observed. The device was further optimised by varying the field strengths of both the collection and transfer regions in isolation. Following this optimisation procedure, the device was able to produce a maximum stable gas gain of ˜90000. These results demonstrate an order of magnitude improvement in gain with the NID gas over previously reported values and ultimately benefits the sensitivity of a NITPC to low energy recoils in the context of a directional DM search

The CYGNO experiment

The search for a novel technology able to detect and reconstruct nuclear and electron recoil events with the energy of a few keV has become more and more important now that large regions of high-mass dark matter (DM) candidates have been excluded. Moreover, a detector sensitive to incoming particle direction will be crucial in the case of DM discovery to open the possibility of studying its properties. Gaseous time projection chambers (TPC) with optical readout are very promising detectors combining the detailed event information provided by the TPC technique with the high sensitivity and granularity of latest-generation scientific light sensors. The CYGNO experiment (a CYGNus module with Optical readout) aims to exploit the optical readout approach of multiple-GEM structures in large volume TPCs for the study of rare events as interactions of low-mass DM or solar neutrinos. The combined use of high-granularity sCMOS cameras and fast light sensors allows the reconstruction of the 3D direction of the tracks, offering good energy resolution and very high sensitivity in the few keV energy range, together with a very good particle identification useful for distinguishing nuclear recoils from electronic recoils. This experiment is part of the CYGNUS proto-collaboration, which aims at constructing a network of underground observatories for directional DM search. A one cubic meter demonstrator is expected to be built in 2022/23 aiming at a larger scale apparatus (30 m3–100 m3) at a later stage

The CYGNO experiment: a directional Dark Matter detector with optical readout

We are going to discuss the R&D and the prospects for the CYGNO project, towards the development of an innovative, high precision 3D tracking Time Projection Chamber with optical readout using He:CF4 gas at 1 bar. CYGNO uses a stack of triple thin GEMs for charge multiplication, this induces scintillation in CF4 gas, which is readout by PMTs and sCMOS cameras. High granularity and low readout noise of sCMOS along with high sampling of PMT allows CYGNO to have 3D tracking with head tail capability and particle identification down to O(keV) energy for directional Dark Matter searches and solar neutrino spectroscopy. We will present the most recent R&D results from the CYGNO project, and in particular the overground commissioning of the largest prototype developed so far, LIME with a 33×33 cm2 readout plane and 50 cm of drift length, for a total of 50 litres active volume. We will illustrate the LIME response characterisation between 3.7 keV and 44 keV by means of multiple X-ray sources, and the data Monte-Carlo comparison of simulated sCMOS images in this energy range. Furthermore, we will present current LIME installation, operation and data taking at underground Laboratori Nazionali del Gran Sasso (LNGS), serving as demonstrator for the development of a 0.4 m3 CYGNO detector. We will conclude by mentioning the technical choices and the prospects of the 0.4 m3 detector, as laid out in the Technical Design Report (TDR) recently produced by our collaboration