Anomalous quantum-critical scaling corrections in two-dimensional antiferromagnets

We study the N\'eel-paramagnetic quantum phase transition in two-dimensional dimerized $S=1/2$ Heisenberg antiferromagnets using finite-size scaling of quantum Monte Carlo data. We resolve the long standing issue of the role of cubic interactions arising in the bond-operator representation when the dimer pattern lacks a certain symmetry. We find non-monotonic (monotonic) size dependence in the staggered (columnar) dimerized model, where cubic interactions are (are not) present. We conclude that there is an irrelevant field in the staggered model that is not present in the columnar case, but, at variance with previous claims, it is not the leading irrelevant field. The new exponent is $\omega_2 \approx 1.25$ and the prefactor of the correction $L^{-\omega_2}$ is large and comes with a different sign from that of the formally leading conventional correction with exponent $\omega_1 \approx 0.78$. Our study highlights the possibility of competing scaling corrections at quantum critical points.Comment: 6 pages, 6 figure

Investigating Berezinskii-Kosterlitz-Thouless phase transitions in Kagome spin ice by quantifying Monte Carlo process: Distribution of Hamming distances

We reinvestigate the phase transitions of the Ising model on the Kagome lattice with antiferromagnetic nearest-neighbor and ferromagnetic next-nearest-neighbor interactions, which has a six-state-clock spin ice ground state and two consecutive Berezinskii-Kosterlitz-Thouless (BKT) phase transitions. Employing the classical Monte Carlo (MC) simulations, the phases are characterized by the magnetic order parameter, and the critical temperatures are obtained by the finite-size scaling of related physical quantities. Moreover, we attempt to gain general information on the phase transitions from the MC process instead of MC results and successfully extract the correct transition points with surprisingly high accuracy. Specifically, we focus on the selected data set of uncorrelated MC configurations and quantify the MC process using the distribution of two-configuration Hamming distances in this small data collection. This distribution is more than a quantity that features different behaviors in different phases but also nicely supports the same BKT scaling form as the order parameter, from which we successfully determine the two BKT transition points with surprisingly high accuracy. We also discuss the connection between the phase transitions and the intrinsic dimension extracted from the Hamming distances, which is widely used in the growing field of machine learning and is reported to be able to detect critical points. Our findings provide a new understanding of the spin ice transitions in the Kagome lattice and can hopefully be used similarly to identify transitions in the quantum system on the same lattice with strong frustrations.Comment: 12 figure

Scaling of disorder operator at deconfined quantum criticality

We study scaling behavior of the disorder parameter, defined as the expectation value of a symmetry transformation applied to a finite region, at the deconfined quantum critical point in (2+1)$d$ in the $J$-$Q_3$ model via large-scale quantum Monte Carlo simulations. We show that the disorder parameter for U(1) spin rotation symmetry exhibits perimeter scaling with a logarithmic correction associated with sharp corners of the region, as generally expected for a conformally-invariant critical point. However, for large rotation angle the universal coefficient of the logarithmic corner correction becomes negative, which is not allowed in any unitary conformal field theory. We also extract the current central charge from the small rotation angle scaling, whose value is much smaller than that of the free theory.Comment: 8 pages, 6 figures; v2 improved measurement on disorder operato

Dynamical signature of fractionalization at a deconfined quantum critical point

Deconfined quantum critical points govern continuous quantum phase transitions at which fractionalized (deconfined) degrees of freedom emerge. Here we study dynamical signatures of the fractionalized excitations in a quantum magnet (the easy-plane J-Q model) that realize a deconfined quantum critical point with emergent O(4) symmetry. By means of large-scale quantum Monte Carlo simulations and stochastic analytic continuation of imaginary-time correlation functions, we obtain the dynamic spin-structure factors in the S x and S z channels. In both channels, we observe broad continua that originate from the deconfined excitations. We further identify several distinct spectral features of the deconfined quantum critical point, including the lower edge of the continuum and its form factor on moving through the Brillouin zone. We provide field-theoretical and lattice model calculations that explain the overall shapes of the computed spectra, which highlight the importance of interactions and gauge fluctuations to explain the spectral-weight distribution. We make further comparisons with the conventional Landau O(2) transition in a different quantum magnet, at which no signatures of fractionalization are observed. The distinctive spectral signatures of the deconfined quantum critical point suggest the feasibility of its experimental detection in neutron scattering and nuclear magnetic resonance experiments.First author draf

Emergent O(4) symmetry at the phase transition from plaquette-singlet to antiferromagnetic order in quasi-two-dimensional quantum magnets

Recent experiments [J. Guo et al., Phys. Rev. Lett.124,206602 (2020)] on thermodynamic properties of the frustrated layered quantum magnet SrCu$_2$(BO$_3$)$_2$ -- the Shastry-Sutherland material -- have provided strong evidence for a low-temperature phase transition between plaquette-singlet and antiferromagnetic order as a function of pressure. Further motivated by the recently discovered unusual first-order quantum phase transition with an apparent emergent O(4) symmetry of the antiferromagnetic and plaquette-singlet order parameters in a two-dimensional "checkerboard J-Q" quantum spin model [B. Zhao et al., Nat. Phys. 15, 678 (2019)], we here study the same model in the presence of weak inter-layer couplings. Our focus is on the evolution of the emergent symmetry as the system crosses over from two to three dimensions and the phase transition extends from strictly zero temperature in two dimensions up to finite temperature as expected in SrCu$_2$(BO$_3$)$_2$. Using quantum Monte Carlo simulations, we map out the phase boundaries of the plaquette-singlet and antiferromagnetic phases, with particular focus on the triple point where these two order phases meet the paramagnetic phase for given strength of the inter-layer coupling. All transitions are first-order in the neighborhood of the triple points. We show that the emergent O(4) symmetry of the coexistence state breaks down clearly when the interlayer coupling becomes sufficiently large, but for a weak coupling, of the magnitude expected experimentally, the enlarged symmetry can still be observed at the triple point up to significant length scales. Thus, it is likely that the plaquette-singlet to antiferromagnetic transition in SrCu$_2$(BO$_3$)$_2$ exhibits remnants of emergent O(4) symmetry, which should be observable due to additional weakly gapped Goldstone modes.Comment: 14 pages, 8 figure

Quantum phases of SrCu2(BO3)2 from high-pressure thermodynamics

We report heat capacity measurements of SrCu$_2$(BO$_3$)$_2$ under high pressure along with simulations of relevant quantum spin models and map out the $(P,T)$ phase diagram of the material. We find a first-order quantum phase transition between the low-pressure quantum dimer paramagnet and a phase with signatures of a plaquette-singlet state below T = $2$ K. At higher pressures, we observe a transition into a previously unknown antiferromagnetic state below $4$ K. Our findings can be explained within the two-dimensional Shastry-Sutherland quantum spin model supplemented by weak inter-layer couplings. The possibility to tune SrCu$_2$(BO$_3$)$_2$ between the plaquette-singlet and antiferromagnetic states opens opportunities for experimental tests of quantum field theories and lattice models involving fractionalized excitations, emergent symmetries, and gauge fluctuations.Comment: 6 pages + 8 pages supplemental informatio

Zigzag magnetic order in a novel tellurate compound Na4−δ_{4-\delta}NiTeO6_{6} with S\mathit{S} = 1 chains

Na$_{4-\delta}$NiTeO$_{6}$ is a rare example in the transition-metal tellurate family of realizing an $S$ = 1 spin-chain structure. By performing neutron powder diffraction measurements, the ground-state magnetic structure of Na$_{4-\delta}$NiTeO$_{6}$ is determined. These measurements reveal that below $T\rm_{N}$ ${\sim}$ 6.8(2) K, the Ni$^{2+}$ moments form a screwed ferromagnetic (FM) spin-chain structure running along the crystallographic $a$ axis but these FM spin chains are coupled antiferromagnetically along the $b$ and $c$ directions, giving rise to a magnetic propagation vector of $k$ = (0, 1/2, 1/2). This zigzag magnetic order is well supported by first-principles calculations. The moment size of Ni$^{2+}$ spins is determined to be 2.1(1) $\mu$$\rm_{B}$ at 3 K, suggesting a significant quenching of the orbital moment due to the crystalline electric field (CEF) effect. The previously reported metamagnetic transition near $H\rm_{C}$ ${\sim}$ 0.1 T can be understood as a field-induced spin-flip transition. The relatively easy tunability of the dimensionality of its magnetism by external parameters makes Na$_{4-\delta}$NiTeO$_{6}$ a promising candidate for further exploring various types of novel spin-chain physics.Comment: 10 pages, 6 figure