36 research outputs found
Electron Spin Decoherence in Bulk and Quantum Well Zincblende Semiconductors
A theory for longitudinal (T1) and transverse (T2) electron spin coherence
times in zincblende semiconductor quantum wells is developed based on a
non-perturbative nanostructure model solved in a fourteen-band restricted basis
set. Distinctly different dependences of coherence times on mobility,
quantization energy, and temperature are found from previous calculations.
Quantitative agreement between our calculations and measurements is found for
GaAs/AlGaAs, InGaAs/InP, and GaSb/AlSb quantum wells.Comment: 11 pages, 3 figure
Electron Spin Relaxation in a Semiconductor Quantum Well
A fully microscopic theory of electron spin relaxation by the
D'yakonov-Perel' type spin-orbit coupling is developed for a semiconductor
quantum well with a magnetic field applied in the growth direction of the well.
We derive the Bloch equations for an electron spin in the well and define
microscopic expressions for the spin relaxation times. The dependencies of the
electron spin relaxation rate on the lowest quantum well subband energy,
magnetic field and temperature are analyzed.Comment: Revised version as will appear in Physical Review
Anisotropic splitting of intersubband spin plasmons in quantum wells with bulk and structural inversion asymmetry
In semiconductor heterostructures, bulk and structural inversion asymmetry
and spin-orbit coupling induce a k-dependent spin splitting of valence and
conduction subbands, which can be viewed as being caused by momentum-dependent
crystal magnetic fields. This paper studies the influence of these effective
magnetic fields on the intersubband spin dynamics in an asymmetric n-type
GaAs/AlGaAs quantum well. We calculate the dispersions of intersubband spin
plasmons using linear response theory. The so-called D'yakonov-Perel'
decoherence mechanism is inactive for collective intersubband excitations,
i.e., crystal magnetic fields do not lead to decoherence of spin plasmons.
Instead, we predict that the main signature of bulk and structural inversion
asymmetry in intersubband spin dynamics is a three-fold, anisotropic splitting
of the spin plasmon dispersion. The importance of many-body effects is pointed
out, and conditions for experimental observation with inelastic light
scattering are discussed.Comment: 8 pages, 6 figure
Semiclassical kinetic theory of electron spin relaxation in semiconductors
We develop a semiclassical kinetic theory for electron spin relaxation in
semiconductors. Our approach accounts for elastic as well as inelastic
scattering and treats Elliott-Yafet and motional-narrowing processes, such as
D'yakonov-Perel' and variable g-factor processes, on an equal footing. Focusing
on small spin polarizations and small momentum transfer scattering, we derive,
starting from the full quantum kinetic equations, a Fokker-Planck equation for
the electron spin polarization. We then construct, using a rigorous multiple
time scale approach, a Bloch equation for the macroscopic (-averaged)
spin polarization on the long time scale, where the spin polarization decays.
Spin-conserving energy relaxation and diffusion, which occur on a fast time
scale, after the initial spin polarization has been injected, are incorporated
and shown to give rise to a weight function which defines the energy averages
required for the calculation of the spin relaxation tensor in the Bloch
equation. Our approach provides an intuitive way to conceptualize the dynamics
of the spin polarization in terms of a ``test'' spin polarization which
scatters off ``field'' particles (electrons, impurities, phonons). To
illustrate our approach, we calculate for a quantum well the spin lifetime at
temperatures and densities where electron-electron and electron-impurity
scattering dominate. The spin lifetimes are non-monotonic functions of
temperature and density. Our results show that at electron densities and
temperatures, where the cross-over from the non-degenerate to the degenerate
regime occurs, spin lifetimes are particularly long.Comment: 29 pages, 10 figures, final versio
Intersubband spin-density excitations in quantum wells with Rashba spin splitting
In inversion-asymmetric semiconductors, spin-orbit coupling induces a
k-dependent spin splitting of valence and conduction bands, which is a
well-known cause for spin decoherence in bulk and heterostructures.
Manipulating nonequilibrium spin coherence in device applications thus requires
understanding how valence and conduction band spin splitting affects carrier
spin dynamics. This paper studies the relevance of this decoherence mechanism
for collective intersubband spin-density excitations (SDEs) in quantum wells. A
density-functional formalism for the linear spin-density matrix response is
presented that describes SDEs in the conduction band of quantum wells with
subbands that may be non-parabolic and spin-split due to bulk or structural
inversion asymmetry (Rashba effect). As an example, we consider a 40 nm
GaAs/AlGaAs quantum well, including Rashba spin splitting of the conduction
subbands. We find a coupling and wavevector-dependent splitting of the
longitudinal and transverse SDEs. However, decoherence of the SDEs is not
determined by subband spin splitting, due to collective effects arising from
dynamical exchange and correlation.Comment: 10 pages, 4 figure
Magnetotransport in two-dimensional electron gas at large filling factors
We derive the quantum Boltzmann equation for the two-dimensional electron gas
in a magnetic field such that the filling factor . This equation
describes all of the effects of the external fields on the impurity collision
integral including Shubnikov-de Haas oscillations, smooth part of the
magnetoresistance, and non-linear transport. Furthemore, we obtain quantitative
results for the effect of the external microwave radiation on the linear and
non-linear transport in the system. Our findings are relevant for the
description of the oscillating resistivity discovered by Zudov {\em et al.},
zero-resistance state discovered by Mani {\em et al.} and Zudov {\em et al.},
and for the microscopic justification of the model of Andreev {\em et al.}. We
also present semiclassical picture for the qualitative consideration of the
effects of the applied field on the collision integral.Comment: 28 pages, 19 figures; The discussion of the role of the effect of the
microwave field on the distribution function is revised (see also
cond-mat/0310668). Accepted in Phys. Rev.
Spin-dephasing anisotropy for electrons in a diffusive quasi-1D GaAs wire
We present a numerical study of dephasing of electron spin ensembles in a
diffusive quasi-one-dimensional GaAs wire due to the D'yakonov-Perel'
spin-dephasing mechanism. For widths of the wire below the spin precession
length and for equal strength of Rashba and linear Dresselhaus spin-orbit
fields a strong suppression of spin-dephasing is found. This suppression of
spin-dephasing shows a strong dependence on the wire orientation with respect
to the crystal lattice. The relevance for realistic cases is evaluated by
studying how this effect degrades for deviating strength of Rashba and linear
Dresselhaus fields, and with the inclusion of the cubic Dresselhaus term
Spin and energy transfer in nanocrystals without transport of charge
We describe a mechanism of spin transfer between individual quantum dots that
does not require tunneling. Incident circularly-polarized photons create
inter-band excitons with non-zero electron spin in the first quantum dot. When
the quantum-dot pair is properly designed, this excitation can be transferred
to the neighboring dot via the Coulomb interaction with either {\it
conservation} or {\it flipping} of the electron spin. The second dot can
radiate circularly-polarized photons at lower energy. Selection rules for spin
transfer are determined by the resonant conditions and by the strong spin-orbit
interaction in the valence band of nanocrystals. Coulomb-induced energy and
spin transfer in pairs and chains of dots can become very efficient under
resonant conditions. The electron can preserve its spin orientation even in
randomly-oriented nanocrystals.Comment: 13 pages, 3 figure
Theory of spin-polarized bipolar transport in magnetic p-n junctions
The interplay between spin and charge transport in electrically and
magnetically inhomogeneous semiconductor systems is investigated theoretically.
In particular, the theory of spin-polarized bipolar transport in magnetic p-n
junctions is formulated, generalizing the classic Shockley model. The theory
assumes that in the depletion layer the nonequilibrium chemical potentials of
spin up and spin down carriers are constant and carrier recombination and spin
relaxation are inhibited. Under the general conditions of an applied bias and
externally injected (source) spin, the model formulates analytically carrier
and spin transport in magnetic p-n junctions at low bias. The evaluation of the
carrier and spin densities at the depletion layer establishes the necessary
boundary conditions for solving the diffusive transport equations in the bulk
regions separately, thus greatly simplifying the problem. The carrier and spin
density and current profiles in the bulk regions are calculated and the I-V
characteristics of the junction are obtained. It is demonstrated that spin
injection through the depletion layer of a magnetic p-n junction is not
possible unless nonequilibrium spin accumulates in the bulk regions--either by
external spin injection or by the application of a large bias. Implications of
the theory for majority spin injection across the depletion layer, minority
spin pumping and spin amplification, giant magnetoresistance, spin-voltaic
effect, biasing electrode spin injection, and magnetic drift in the bulk
regions are discussed in details, and illustrated using the example of a GaAs
based magnetic p-n junction.Comment: 36 pages, 11 figures, 2 table
Spin dynamics in high-mobility two-dimensional electron systems
Understanding the spin dynamics in semiconductor heterostructures is highly
important for future semiconductor spintronic devices. In high-mobility
two-dimensional electron systems (2DES), the spin lifetime strongly depends on
the initial degree of spin polarization due to the electron-electron
interaction. The Hartree-Fock (HF) term of the Coulomb interaction acts like an
effective out-of-plane magnetic field and thus reduces the spin-flip rate. By
time-resolved Faraday rotation (TRFR) techniques, we demonstrate that the spin
lifetime is increased by an order of magnitude as the initial spin polarization
degree is raised from the low-polarization limit to several percent. We perform
control experiments to decouple the excitation density in the sample from the
spin polarization degree and investigate the interplay of the internal HF field
and an external perpendicular magnetic field. The lifetime of spins oriented in
the plane of a [001]-grown 2DES is strongly anisotropic if the Rashba and
Dresselhaus spin-orbit fields are of the same order of magnitude. This
anisotropy, which stems from the interference of the Rashba and the Dresselhaus
spin-orbit fields, is highly density-dependent: as the electron density is
increased, the kubic Dresselhaus term becomes dominant and reduces the
anisotropy.Comment: 13 pages, 6 figure