Evidences for magnetic dimers and skyrmion lattice formation in Eu2_2Pd2_2Sn

Magnetic, thermal and transport properties of the non-centrosymmetric compound Eu$_2$Pd$_2$Sn are revisited after including new measurements. In its paramagnetic phase, the outstanding feature of this compound is the formation of Eu$^{2+}$ dimers that allows to understand the deviation of the magnetic susceptibility $\chi(T)$ from the C-W law below about 70\,K, the field dependent magnetization $M(B)$ variation below $\approx 80$\,K and the reduced entropy at the ordering temperature $S(T_N)= 0.64R\ln(8)$. A significant change of the exchange interactions occurs between $T\approx 70$\,K (where $\theta_P = 18$\,K) and $T_N = 13.3$\,K (where $\theta_P =-4.5$\,K). The strong electronic overlap, arising from the reduced Eu-Eu spacing compared with that of pure Eu$^{2+}$ is expected to power these quasiparticles formation, inducing a significant reformulation of the magnetic structure. A rich magnetic phase diagram is obtained from the analysis of the derivatives of the magnetic parameters: $\partial \chi/\partial T$ and $\partial M/\partial B$, and the field dependence of the specific heat. Two critical points are recognized and a tentative description of the magnetic structures is proposed. The possible formation of a skyrmion lattice, that arises from the presence of magnetically frustrated pockets in the phase diagram, is suggested by theoretical studies on hexagonal structures exhibiting similar interactions pattern.Comment: 13 pages, 11 figure

Searching for a quantum critical point in YbCu5-xAux

Structural, magnetic, transport and thermal properties of YbCu5-xAux alloys with Au concentration between the limit of structural stability of AuBe5 type at x = 0.4 up to x = 0.7 are reported. The outstanding features of this system are: i) the constant and record high values of Cm /T 7J/molK^2 below a characteristic temperature T*, ranging between 150 mK and 350 mK. ii) A power law thermal dependence dependence Cm/T(T>T*)=A/T^q, with q = 1.3 +/- 0.1, and iii) an arising incoherent electronic scattering observed in the resistivity at T < 1K for x < 0.6 despite the fact that Yb magnetic atoms are placed in a lattice. Magnetic frustration, originated in the tetrahedral distribution of Yb atoms, appears as the responsible of the exotic behavior of this system.Comment: 14 pages, 9 figure

Calorimetric tunneling study of heat generation in metal-vacuum-metal tunnel junction

We have proposed novel calorimetric tunneling (CT) experiment allowing exact determination of heat generation (or heat sinking) in individual tunnel junction (TJ) electrodes which opens new possibilities in the field of design and development of experimental techniques for science and technology. Using such experiment we have studied the process of heat generation in normal-metal electrodes of the vacuum-barrier tunnel junction (VBTJ). The results show there exists dependence of the mutual redistribution of the heat on applied bias voltage and the direction of tunnel current, although the total heat generated in tunnel process is equal to Joule heat, as expected. Moreover, presented study indicates generated heat represents the energy of non-equilibrium quasiparticles coming from inelastic electron processes accompanying the process of elastic tunneling.Comment: 8 pages, 3 figures, LaTe

Disappearance of Magnetic Transition in (Ce,Gd)Ni5 System

We present the results of an experimental study focused around CeNi5 in the CexGd1??xNi5 system. Pseudobinary bulk samples were prepared with concentration of x = 0:85, 0.9, 0.95, and 0.97 by arc melting method. The structural analysis confirmed the CaCu5 hexagonal crystal structure with P6/mmm space group and proved the existence of a single phase in all of them. The measurement of the magnetic properties shows that the increase of the Ce content leads to lower TC values. Above x = 0:9 spin fluctuations behaviour appears with a shoulder in M(T) around T = 130 K. Heat capacity measurements support these observations.This work was supported by the projects VEGA 2/0032/16, VEGA 1/0956/17, VEGA 1/0611/18, VEGA 1/0053/19, APVV-16-0079 and the Spanish MINECO MAT2017-83631-C3-

YbPd2In : A promising candidate for strong entropy accumulation at very low temperature

We report on synthesis, crystal structure, magnetic, thermodynamic, and transport properties of the compound YbPd2In, crystallizing as a Heusler structure type. A trivalent state of the rare earth was determined by fitting the magnetic susceptibility with a Curie-Weiss law. This compound is characterized by showing very weak magnetic interactions and a negligible Kondo effect. A specific-heat jump was observed at T 48250mK, followed at higher temperature by a power-law decrease of CP(T)/T. The resulting large electronic entropy increase at very low temperature is rapidly shifted to higher temperature by the application of magnetic field. This magnetocaloric effect places YbPd2In as a very good candidate for adiabatic demagnetization cooling processes