481 research outputs found

    Presence of 3d Quadrupole Moment in LaTiO3 Studied by 47,49Ti NMR

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    Ti NMR spectra of LaTiO3 are reexamined and the orbital state of this compound is discussed. The NMR spectra of LaTiO3 taken at 1.5 K under zero external field indicate a large nuclear quadrupole splitting. This splitting is ascribed to the presence of the rather large quadrupole moment of 3d electrons at Ti sites, suggesting that the orbital liquid model proposed for LaTiO3 is inappropriate. The NMR spectra are well explained by the orbital ordering model expressed approximately as 1/3(dxy+dyz+dzx)1/\sqrt{3}(d_{xy}+d_{yz}+d_{zx}) originating from a crystal field effect. It is also shown that most of the orbital moment is quenched.Comment: 4 pages, 3 fugures; to appear in Phys. Rev. Let

    Tuning the electrically evaluated electron Lande g factor in GaAs quantum dots and quantum wells of different well widths

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    We evaluate the Lande g factor of electrons in quantum dots (QDs) fabricated from GaAs quantum well (QW) structures of different well width. We first determine the Lande electron g factor of the QWs through resistive detection of electron spin resonance and compare it to the enhanced electron g factor determined from analysis of the magneto-transport. Next, we form laterally defined quantum dots using these quantum wells and extract the electron g factor from analysis of the cotunneling and Kondo effect within the quantum dots. We conclude that the Lande electron g factor of the quantum dot is primarily governed by the electron g factor of the quantum well suggesting that well width is an ideal design parameter for g-factor engineering QDs

    Strategic locus for the activation of the superoxide dismutase gene in the nephron

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    Strategic locus for the activation of the superoxide dismutase gene in the nephron. Upon exposure to a transient ischemia, the distal tubule of the kidney often escapes the severe damage which afflicts the proximal tubule. To ascertain whether this feature of the distal tubule is attributable to its intrinsic cellular properties, we focused on two pairs of unique tubule segments; distal versus proximal convoluted tubules in the superficial cortex and distal versus proximal straight tubules in the outer stripe of the outer medulla. These tubules were chosen because, firstly, they can be identified by morphology and immunostaining, and secondly, each pair has the same anatomical relationship to the circulation. Detailed morphometric analyses were performed six hours following unilateral transient ischemia in adult rats to semiquantitate the local tissue damage in these specific nephron segments. The architecture of the distal convoluted and straight tubules was remarkably well preserved, contrasting to the moderate to extensive necrotic changes seen in the proximal tubules. In search of the potential intrinsic cellular mechanism that underlies the observed difference, we examined the segmental distribution along the nephron of manganese superoxide dismutase gene transcripts by in situ hybridization. This antioxidant enzyme gene was expressed primarily in the distal tubules with contrastingly low levels of expression in the proximal tubules. Moreover, following ischemia-reperfusion, this distal tubule-dominant pattern was further accentuated immediately following reperfusion. The study indicates that the marked difference between the proximal and distal tubules in their susceptibility to injury in vivo is attributable to their intrinsic cellular properties, which include the local level of antioxidants

    Scaling of the anomalous Hall effect in Sr1x_{1-x}Cax_xRuO3_3

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    The anomalous Hall effect (AHE) of ferromagnetic thin films of Sr1x_{1-x}Cax_{x}RuO3_3 (0 x\leq x \leq 0.4) is studied as a function of xx and temperature TT. As xx increases, both the transition temperature TcT_c and the magnetization MM are reduced and vanish near xx \sim 0.7. For all compositions, the transverse resistivity ρH\rho_{H} varies non-monotonously with TT, and even changes sign, thus violating the conventional expression ρH=RoB+4πRsM(T)\rho_{H}=R_o B + 4\pi R_s M(T) (BB is the magnetic induction, while RoR_o and RsR_s are the ordinary and anomalous Hall coefficients). From the rather complicated data of ρH\rho_H, we find a scaling behavior of the transverse conductivity σxy\sigma_{xy} with M(T)M(T), which is well reproduced by the first-principles band calculation assuming the intrinsic origin of the AHE.Comment: REVTeX 4 style; 5 pages, 3 figures; revised 23/2 and accepted for publicatio

    Gelatine Cavity Dynamics of High-Speed Sphere Impact

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    We investigate the impact and penetration of a solid sphere passing through gelatine at various impact speeds up to 143.2 m s-1 Tests were performed with several concentrations of gelatine. Impacts for low elastic Froude number Fre a ratio between inertia and gelatine elasticity, resulted in rebound. Higher Fre values resulted in penetration, forming cavities with prominent surface textures. The overall shape of the cavities resembles those observed in water-entry experiments, yet they appear in a different order with respect to increasing inertia: rebound, quasi-seal, deep-seal, shallow-seal and surface-seal. Remarkably, similar to the We – Bo phase diagram in water-entry experiments, the elastic Froude number Fre and elastic Grashof number Gre (a ratio between gravity and gelatine elasticity) classify all five different phenomena into distinguishable regimes. We find that Fre can be a good indicator to describe the cavity length H , particularly in the shallow-seal regime. Finally, the evolution of cavity shape, pinch-off depth, and lower cavity radius are investigated for different Fre values

    Disorder Induced Ferromagnetism in CaRuO3

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    The magnetic ground state of perovskite structure CaRuO3 has been enigmatic for decades. Here we show that paramagnetic CaRuO3 can be made ferromagnetic by very small amounts of partial substitution of Ru by Ti. Magnetic hysteresis loops are observed at 5 K for as little as 2% Ti substitution. Ti is non-magnetic and isovalent with Ru, indicating that the primary effect of the substitution is the disruption of the magnetic ground state of CaRuO3 through disorder. The data suggest that CaRuO3 is poised at a critical point between ferromagnetic and paramagnetic ground states

    Relative contributions of lattice distortion and orbital ordering to resonant x-ray scattering in manganites

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    We investigated the origin of the energy splitting observed in the resonant x-ray scattering (RXS) in manganites. Using thin film samples with controlled lattice parameters and orbital states at a fixed orbital filling, we estimated that the contribution of the interatomic Coulomb interaction relative to the Jahn-Teller mechanism is insignificant and at most 0.27. This indicates that RXS probes mainly Jahn-Teller distortion in manganites.Comment: 8 pages, 4 figure

    Crystal structure, electronic, and magnetic properties of the bilayered rhodium oxide Sr3Rh2O7

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    The bilayered rhodium oxide Sr3Rh2O7 was synthesized by high-pressure and high-temperature heating techniques. The single-phase polycrystalline sample of Sr3Rh2O7 was characterized by measurements of magnetic susceptibility, electrical resistivity, specific heat, and thermopower. The structural characteristics were investigated by powder neutron diffraction study. The rhodium oxide Sr3Rh2O7 [Bbcb, a = 5.4744(8) A, b = 5.4716(9) A, c = 20.875(2) A] is isostructural to the metamagnetic metal Sr3Ru2O7, with five 4d electrons per Rh, which is electronically equivalent to the hypothetic bilayered ruthenium oxide, where one electron per Ru is doped into the Ru-327 unit. The present data show the rhodium oxide Sr3Rh2O7 to be metallic with enhanced paramagnetism, similar to Sr3Ru2O7. However, neither manifest contributions from spin fluctuations nor any traces of a metamagnetic transition were found within the studied range from 2 K to 390 K below 70 kOe.Comment: To be published in PR
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