777 research outputs found

    Violation of Leggett-Garg inequalities in quantum measurements with variable resolution and back-action

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    Quantum mechanics violates Leggett-Garg inequalities because the operator formalism predicts correlations between different spin components that would correspond to negative joint probabilities for the outcomes of joint measurements. However, the uncertainty principle ensures that such joint measurements cannot be implemented without errors. In a sequential measurement of the spin components, the resolution and back-action errors of the intermediate measurement can be described by random spin flips acting on an intrinsic joint probability. If the error rates are known, the intrinsic joint probability can be reconstructed from the noisy statistics of the actual measurement outcomes. In this paper, we use the spin-flip model of measurement errors to analyze experimental data on photon polarization obtained with an interferometric setup that allows us to vary the measurement strength and hence the balance between resolution and back-action errors. We confirm that the intrinsic joint probability obtained from the experimental data is independent of measurement strength and show that the same violation of the Leggett-Garg inequality can be obtained for any combination of measurement resolution and back-action.Comment: 17 pages, 7 figure

    Characterisation and optimisation of a sample preparation method for the detection and quantification of atmospherically relevant carbonyl compounds in aqueous medium

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    Carbonyl compounds are ubiquitous in the atmosphere and either emitted primarily from anthropogenic and biogenic sources or they are produced secondarily from the oxidation of volatile organic compounds. Despite a number of studies about the quantification of carbonyl compounds a comprehensive description of optimised methods is scarce for the quantification of atmospherically relevant carbonyl compounds. The method optimisation was conducted for seven atmospherically relevant carbonyl compounds including acrolein, benzaldehyde, glyoxal, methyl glyoxal, methacrolein, methyl vinyl ketone and 2,3-butanedione. O-(2,3,4,5,6-pentafluorobenzyl)hydroxylamine hydrochloride (PFBHA) was used as derivatisation reagent and the formed oximes were detected by gas chromatography/mass spectrometry (GC/MS). With the present method quantification can be carried out for each carbonyl compound originating from fog, cloud and rain or sampled from the gas- and particle phase in water. Detection limits between 0.01 and 0.17 μmol L−1 were found, depending on carbonyl compounds. Furthermore, best results were found for the derivatisation with a PFBHA concentration of 0.43 mg mL−1 for 24 h followed by a subsequent extraction with dichloromethane for 30 min at pH = 1. The optimised method was evaluated in the present study by the OH radical initiated oxidation of 3-methylbutanone in the aqueous phase. Methyl glyoxal and 2,3-butanedione were found to be oxidation products in the samples with a yield of 2% for methyl glyoxal and 14% for 2,3-butanedione after a reaction time of 5 h

    Image Analysis of Intractable Epilepsy:18F-FDG PET Scan of the Cortical Dysplasia

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    開始ページ、終了ページ: 冊子体のページ付

    Contrasting P-T paths recorded in eclogitic garnet-clinopyroxene rocks from the Gondwana suture zone in southern India

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    第3回極域科学シンポジウム/第32回極域地学シンポジウム 11月30日(金) 国立極地研究所 3階ラウン

    Parity Violation in Neutron Resonances in 107,109Ag

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    Parity nonconservation (PNC) was studied in p-wave resonances in Ag by measuring the helicity dependence of the neutron total cross section. Transmission measurements on natural Ag were performed in the energy range 32 to 422 eV with the time-of-flight method at the Manuel Lujan Neutron Scattering Center at Los Alamos National Laboratory. A total of 15 p-wave neutron resonances were studied in 107Ag and ninep-wave resonances in 109Ag. Statistically significant asymmetries were observed for eight resonances in 107Ag and for four resonances in109Ag. An analysis treating the PNC matrix elements as random variables yields a weak spreading width of Γw=(2.67-1.21+2.65)×10-7 eV for107Ag and Γw=(1.30-0.74+2.49)×10-7 eV for 109Ag

    Multimodal Neuroimages of Adrenoleukodystrophy in Early Stage

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    開始ページ、終了ページ: 冊子体のページ付

    Reactive intermediates revealed in secondary organic aerosol formation from isoprene

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    Isoprene is a significant source of atmospheric organic aerosol; however, the oxidation pathways that lead to secondary organic aerosol (SOA) have remained elusive. Here, we identify the role of two key reactive intermediates, epoxydiols of isoprene (IEPOX = β-IEPOX + δ-IEPOX) and methacryloylperoxynitrate (MPAN), which are formed during isoprene oxidation under low- and high-NO_x conditions, respectively. Isoprene low-NO_x SOA is enhanced in the presence of acidified sulfate seed aerosol (mass yield 28.6%) over that in the presence of neutral aerosol (mass yield 1.3%). Increased uptake of IEPOX by acid-catalyzed particle-phase reactions is shown to explain this enhancement. Under high-NO_x conditions, isoprene SOA formation occurs through oxidation of its second-generation product, MPAN. The similarity of the composition of SOA formed from the photooxidation of MPAN to that formed from isoprene and methacrolein demonstrates the role of MPAN in the formation of isoprene high-NO_x SOA. Reactions of IEPOX and MPAN in the presence of anthropogenic pollutants (i.e., acidic aerosol produced from the oxidation of SO_2 and NO_2, respectively) could be a substantial source of “missing urban SOA” not included in current atmospheric models

    Parity Violation in 232Th Neutron Resonances Above 250 eV

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    The analysis of parity nonconservation (PNC) measurements performed on 232Th by the TRIPLE Collaboration has been extended to include the neutron energy range of 250 to 1900 eV. Below 250 eV all ten statistically significant parity violations have the same sign. However, at higher energies PNC effects of both signs were observed in the transmission of longitudinally polarized neutrons through a thick thorium target. Although the limited experimental energy resolution precluded analysis in terms of the longitudinal asymmetry, parity violations were observed and the cross section differences for positive and negative neutron helicities were obtained. For comparison, a similar analysis was performed on the data below 250 eV, for which longitudinal asymmetries were obtained previously. For energies below 250 eV, the p-wave neutron strength functions for the J=1/2 and J=3/2 states were extracted: S1/21=(1.68±0.61)×10-4 and S3/21=(0.75±0.18)×10-4. The data provide constraints on the properties of local doorway states proposed to explain the PNC sign effect in thorium
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