Collective states in highly symmetric atomic configurations, and single-photon traps

Abbreviated Abstract: We study correlated states in a circular and linear-chain configuration of identical two-level atoms containing the energy of a single quasi-resonant photon in the form of a collective excitation, where the collective behaviour is mediated by exchange of transverse photons between the atoms. For a circular configuration of atoms the effective Hamiltonian on the radiationless subspace of the system can be diagonalized analytically. In this case, the radiationless energy eigenstates carry a $\mathbb{Z}_N$ quantum number $p=0,1, ..., N$ which is analogous to the angular momentum quantum number $l= 0, 1, ...$, carried by particles propagating in a central potential, such as a hydrogen-like system. Just as the hydrogen s-states are the only electronic wave functions which can occupy the central region of the Coulomb potential, the quasi-particle corresponding to a collective excitation of the circular atomic sample can occupy the central atom only for vanishing $\mathbb{Z}_N$ quantum number $p$. For large numbers of atoms in a maximally subradiant state, a critical interatomic distance of $\lambda/2$ emerges both in the linear-chain and the circular configuration of atoms. The spontaneous decay rate of the linear configuration exhibits a jump-like "critical" behaviour for next-neighbour distances close to a half-wavelength. Furthermore, both the linear-chain and the circular configuration exhibit exponential photon trapping once the next-neighbour distance becomes less than a half-wavelength, with the suppression of spontaneous decay being particularly pronounced in the circular system. In this way, circular configurations containing sufficiently many atoms may be natural candidates for {\it single-photon traps}.Comment: Invited contribution to "Xth International Conference on Quantum Optics ICQO 2004" in Minsk, Belarus. To be published in Optics and Spectroscop

Femtosecond pulses and dynamics of molecular photoexcitation: RbCs example

We investigate the dynamics of molecular photoexcitation by unchirped femtosecond laser pulses using RbCs as a model system. This study is motivated by a goal of optimizing a two-color scheme of transferring vibrationally-excited ultracold molecules to their absolute ground state. In this scheme the molecules are initially produced by photoassociation or magnetoassociation in bound vibrational levels close to the first dissociation threshold. We analyze here the first step of the two-color path as a function of pulse intensity from the low-field to the high-field regime. We use two different approaches, a global one, the 'Wavepacket' method, and a restricted one, the 'Level by Level' method where the number of vibrational levels is limited to a small subset. The comparison between the results of the two approaches allows one to gain qualitative insights into the complex dynamics of the high-field regime. In particular, we emphasize the non-trivial and important role of far-from-resonance levels which are adiabatically excited through 'vertical' transitions with a large Franck-Condon factor. We also point out spectacular excitation blockade due to the presence of a quasi-degenerate level in the lower electronic state. We conclude that selective transfer with femtosecond pulses is possible in the low-field regime only. Finally, we extend our single-pulse analysis and examine population transfer induced by coherent trains of low-intensity femtosecond pulses.Comment: 25 pages, 12 figure

Mean field ground state of a spin-1 condensate in a magnetic field

We revisit the topic of the mean field ground state of a spin-1 atomic condensate inside a uniform magnetic field ($B$) under the constraints that both the total number of atoms ($N$) and the magnetization ($\cal M$) are conserved. In the presence of an internal state (spin component) independent trap, we also investigate the dependence of the so-called single spatial mode approximation (SMA) on the magnitude of the magnetic field and ${\cal M}$. Our result indicate that the quadratic Zeeman effect is an important factor in balancing the mean field energy from elastic atom-atom collisions that are known to conserve both $N$ and $\cal M$.Comment: 13 pages, 9 figures, to be published in New J. Phys. (http://www.njp.org/

Dual-probe decoherence microscopy: Probing pockets of coherence in a decohering environment

We study the use of a pair of qubits as a decoherence probe of a non-trivial environment. This dual-probe configuration is modelled by three two-level-systems which are coupled in a chain in which the middle system represents an environmental two-level-system (TLS). This TLS resides within the environment of the qubits and therefore its coupling to perturbing fluctuations (i.e. its decoherence) is assumed much stronger than the decoherence acting on the probe qubits. We study the evolution of such a tripartite system including the appearance of a decoherence-free state (dark state) and non-Markovian behaviour. We find that all parameters of this TLS can be obtained from measurements of one of the probe qubits. Furthermore we show the advantages of two qubits in probing environments and the new dynamics imposed by a TLS which couples to two qubits at once.Comment: 29 pages, 10 figure

Preparation of decoherence-free, subradiant states in a cavity

The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to the environment, there are collective, subradiant states, that have no dipole coupling to photon modes, and therefore they are expected to decay slower. This property also implies that these type of states, which form an N-1 dimensional subspace of the atomic subsytem, also decohere slower. We propose a scheme which will create such states. First the two-level atoms are placed in a strongly detuned cavity and one of the atoms, called the control atom is excited. The time evolution of the coupled atom-cavity system leads to an appropriately entangled state of the atoms. By applying subsequent laser pulses at a well defined time instant, it is possible to drive the atomic state into the subradiant, i. e., decoherence free subspace. Up to a certain average number of the photons, the result is independent of the state of the cavity. The analysis of the conditions shows that this scheme is feasible with present day techniques achieved in atom cavity interaction experiments.Comment: 5 page

Complete eigenstates of identical qubits arranged in regular polygons

We calculate the energy eigenvalues and eigenstates corresponding to coherent single and multiple excitations of an array of N identical qubits or two-level atoms (TLA's) arranged on the vertices of a regular polygon. We assume only that the coupling occurs via an exchange interaction which depends on the separation between the qubits. We include the interactions between all pairs of qubits, and our results are valid for arbitrary distances relative to the radiation wavelength. To illustrate the usefulness of these states, we plot the distance dependence of the decay rates of the n=2 (biexciton) eigenstates of an array of 4 qubits, and tabulate the biexciton eigenvalues and eigenstates, and absorption frequencies, line widths, and relative intensities for polygons consisting of N=2,...,9 qubits in the long-wavelength limit.Comment: Added a figure showing how these results can be used to compute deviations from "equal collective decoherence" approximation

Energies and damping rates of elementary excitations in spin-1 Bose-Einstein condensed gases

Finite temperature Green's function technique is used to calculate the energies and damping rates of elementary excitations of the homogeneous, dilute, spin-1 Bose gases below the Bose-Einstein condensation temperature both in the density and spin channels. For this purpose the self-consistent dynamical Hartree-Fock model is formulated, which takes into account the direct and exchange processes on equal footing by summing up certain classes of Feynman diagrams. The model is shown to fulfil the Goldstone theorem and to exhibit the hybridization of one-particle and collective excitations correctly. The results are applied to the gases of ^{23}Na and ^{87}Rb atoms.Comment: 26 pages, 21 figures. Added 2 new figures, detailed discussio

On the single mode approximation in spinor-1 atomic condensate

We investigate the validity conditions of the single mode approximation (SMA) in spinor-1 atomic condensate when effects due to residual magnetic fields are negligible. For atomic interactions of the ferromagnetic type, the SMA is shown to be exact, with a mode function different from what is commonly used. However, the quantitative deviation is small under current experimental conditions (for $^{87}$Rb atoms). For anti-ferromagnetic interactions, we find that the SMA becomes invalid in general. The differences among the mean field mode functions for the three spin components are shown to depend strongly on the system magnetization. Our results can be important for studies of beyond mean field quantum correlations, such as fragmentation, spin squeezing, and multi-partite entanglement.Comment: Revised, newly found analytic proof adde

Calculation of the interspecies s-wave scattering length in an ultracold Na-Rb vapor

We report the calculation of the interspecies scattering length for the sodium-rubidium (Na-Rb) system. We present improved hybrid potentials for the singlet $X^1\Sigma^+$ and triplet $a^3\Sigma^+$ ground states of the NaRb molecule, and calculate the singlet and triplet scattering lengths $a_{s}$ and $a_{t}$ for the isotopomers $^{23}$Na$^{87}$Rb and $^{23}$Na$^{85}$Rb. Using these values, we assess the prospects for producing a stable two-species Bose-Einstein condensate in the Na-Rb system.Comment: v2: report correct units in Table captions, fix error in conclusions for $^{23}$Na$^{85}$Rb TBEC. Otherwise, more concise presentation, typos fixed. 6 pages, 1 figur

Superradiance from an ultrathin film of three-level V-type atoms: Interplay between splitting, quantum coherence and local-field effects

We carry out a theoretical study of the collective spontaneous emission (superradiance) from an ultrathin film comprised of three-level atoms with $V$-configuration of the operating transitions. As the thickness of the system is small compared to the emission wavelength inside the film, the local-field correction to the averaged Maxwell field is relevant. We show that the interplay between the low-frequency quantum coherence within the subspace of the upper doublet states and the local-field correction may drastically affect the branching ratio of the operating transitions. This effect may be used for controlling the emission process by varying the doublet splitting and the amount of low-frequency coherence.Comment: 15 pages, 5 figure