7,122 research outputs found
Electron Paramagnetic Resonance of Boron Acceptors in Isotopically Purified Silicon
The electron paramagnetic resonance (EPR) linewidths of B acceptors in Si are
found to reduce dramatically in isotopically purified 28Si single crystals.
Moreover, extremely narrow substructures in the EPR spectra are visible
corresponding to either an enhancement or a reduction of the absorbed microwave
on resonance. The origin of the substructures is attributed to a combination of
simultaneous double excitation and spin relaxation in the four level spin
system of the acceptors. A spin population model is developed which
qualitatively describes the experimental results.Comment: 4 pages, 3 figure
Coherence of Spin Qubits in Silicon
Given the effectiveness of semiconductor devices for classical computation
one is naturally led to consider semiconductor systems for solid state quantum
information processing. Semiconductors are particularly suitable where local
control of electric fields and charge transport are required. Conventional
semiconductor electronics is built upon these capabilities and has demonstrated
scaling to large complicated arrays of interconnected devices. However, the
requirements for a quantum computer are very different from those for classical
computation, and it is not immediately obvious how best to build one in a
semiconductor. One possible approach is to use spins as qubits: of nuclei, of
electrons, or both in combination. Long qubit coherence times are a
prerequisite for quantum computing, and in this paper we will discuss
measurements of spin coherence in silicon. The results are encouraging - both
electrons bound to donors and the donor nuclei exhibit low decoherence under
the right circumstances. Doped silicon thus appears to pass the first test on
the road to a quantum computer.Comment: Submitted to J Cond Matter on Nov 15th, 200
Host isotope mass effects on the hyperfine interaction of group-V donors in silicon
The effects of host isotope mass on the hyperfine interaction of group-V
donors in silicon are revealed by pulsed electron nuclear double resonance
(ENDOR) spectroscopy of isotopically engineered Si single crystals. Each of the
hyperfine-split P-31, As-75, Sb-121, Sb-123, and Bi-209 ENDOR lines splits
further into multiple components, whose relative intensities accurately match
the statistical likelihood of the nine possible average Si masses in the four
nearest-neighbor sites due to random occupation by the three stable isotopes
Si-28, Si-29, and Si-30. Further investigation with P-31 donors shows that the
resolved ENDOR components shift linearly with the bulk-averaged Si mass.Comment: 5 pages, 4 figures, 1 tabl
Fluorescent Silicon Clusters and Nanoparticles
The fluorescence of silicon clusters is reviewed. Atomic clusters of silicon
have been at the focus of research for several decades because of the relevance
of size effects for material properties, the importance of silicon in
electronics and the potential applications in bio-medicine. To date numerous
examples of nanostructured forms of fluorescent silicon have been reported.
This article introduces the principles and underlying concepts relevant for
fluorescence of nanostructured silicon such as excitation, energy relaxation,
radiative and non-radiative decay pathways and surface passivation.
Experimental methods for the production of silicon clusters are presented. The
geometric and electronic properties are reviewed and the implications for the
ability to emit fluorescence are discussed. Free and pure silicon clusters
produced in molecular beams appear to have properties that are unfavourable for
light emission. However, when passivated or embedded in a suitable host, they
may emit fluorescence. The current available data show that both quantum
confinement and localised transitions, often at the surface, are responsible
for fluorescence. By building silicon clusters atom by atom, and by embedding
them in shells atom by atom, new insights into the microscopic origins of
fluorescence from nanoscale silicon can be expected.Comment: 5 figures, chapter in "Silicon Nanomaterials Sourcebook", editor
Klaus D. Sattler, CRC Press, August 201
Coherent state transfer between an electron- and nuclear spin in 15N@C60
Electron spin qubits in molecular systems offer high reproducibility and the
ability to self assemble into larger architectures. However, interactions
between neighbouring qubits are 'always-on' and although the electron spin
coherence times can be several hundred microseconds, these are still much
shorter than typical times for nuclear spins. Here we implement an
electron-nuclear hybrid scheme which uses coherent transfer between electron
and nuclear spin degrees of freedom in order to both controllably turn on/off
dipolar interactions between neighbouring spins and benefit from the long
nuclear spin decoherence times (T2n). We transfer qubit states between the
electron and 15N nuclear spin in 15N@C60 with a two-way process fidelity of
88%, using a series of tuned microwave and radiofrequency pulses and measure a
nuclear spin coherence lifetime of over 100 ms.Comment: 5 pages, 3 figures with supplementary material (8 pages
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