19 research outputs found

    Strain engineering and one-dimensional organization of metal-insulator domains in single-crystal VO2 beams

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    Spatial phase inhomogeneity at the nano- to microscale is widely observed in strongly-correlated electron materials. The underlying mechanism and possibility of artificially controlling the phase inhomogeneity are still open questions of critical importance for both the phase transition physics and device applications. Lattice strain has been shown to cause the coexistence of metallic and insulating phases in the Mott insulator VO2. By continuously tuning strain over a wide range in single-crystal VO2 micro- and nanobeams, here we demonstrate the nucleation and manipulation of one-dimensionally ordered metal-insulator domain arrays along the beams. Mott transition is achieved in these beams at room temperature by active control of strain. The ability to engineer phase inhomogeneity with strain lends insight into correlated electron materials in general, and opens opportunities for designing and controlling the phase inhomogeneity of correlated electron materials for micro- and nanoscale device applications.Comment: 14 pages, 4 figures, with supplementary informatio

    Nanoscale Magnetostrictive Response in a Thin Film Owing to a Local magnetic Field

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    Scanning probe microscope experiments are presented in which thin magnetostrictive films deposited on top of micrometer-sized magnetic write heads as used in magnetic hard disk drives, are used to visualize their emanating magnetic field. The magnetostrictive expansion owing to magnetic writing fields is discussed, together with the transduction mechanisms that lead to the vertical and lateral contrast observed. Experimental results verify that the techniques described have a lateral resolution in the realm of 100 n

    Strain control of oxygen kinetics in the Ruddlesden-Popper oxide La1.85Sr0.15CuO4

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    Oxygen defect control has long been considered an important route to functionalizing complex oxide films. However, the nature of oxygen defects in thin films is often not investigated beyond basic redox chemistry. One of the model examples for oxygen-defect studies is the layered Ruddlesden-Popper phase La2-xSrxCuO4-delta (LSCO), in which the superconducting transition temperature is highly sensitive to epitaxial strain. However, previous observations of strain-superconductivity coupling in LSCO thin films were mainly understood in terms of elastic contributions to mechanical buckling, with minimal consideration of kinetic or thermodynamic factors. Here, we report that the oxygen non-stoichiometry commonly reported for strained cuprates is mediated by the strain-modified surface exchange kinetics, rather than reduced thermodynamic oxygen formation energies. Remarkably, tensile-strained LSCO shows nearly an order of magnitude faster oxygen exchange rate than a compressively strained film, providing a strategy for developing high-performance energy materials
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