2 research outputs found
Nanofiber-Constructed Aerogel Solar Evaporator for Efficient Salt Resistance and Volatile Removal
Solar-driven
interfacial evaporation has been validated as an ecofriendly
and sustainable technique for energy-efficient water sanitation. However,
current solar evaporators grapple with the significant accumulation
of salt and the presence of volatiles. Herein, a multifunctional nanofiber-constructed
aerogel evaporator was successfully developed via electrospinning,
freeze-drying, high-temperature processing, and in situ synthesis.
This nanofibrous aerogel, characterized by its large and coterminous
pores constructed of nanofibers within a three-dimensional (3D) structure,
facilitates the transportation of accumulated salts from the evaporation
interface to less saline bulk water, effectively mitigating solar
evaporator scaling. Simultaneously, it also provides ample adsorption
and photocatalytic sites for highly efficient volatile removal. The
resultant evaporator exhibits a high evaporation rate of 1.88 kg m–2 h–1 and an exceptional aniline
removal efficiency of ∼95% and maintained stability during
the desalination of a 3.5 wt % of NaCl solution with 5 mg L–1 of volatile aniline under 1 sun irradiation. The elucidation of
the mechanism responsible for volatile removal was further accomplished
through a comparative analysis of adsorption and catalysis experiments.
This work may provide new insights into the development of multifunctional
nanofiber-constructed aerogel solar evaporators for more complex hypersaline
water treatment