Two-dimensional quantum antiferromagnets

This review presents some theoretical advances in the field of quantum magnetism in two-dimensional systems, and quantum spin liquids in particular. It is to be published as a chapter in the second edition of the book "Frustrated spin systems", edited by H. T. Diep (World-Scientific). The section (Sec. 7) devoted to the kagome antiferromagnet has been completely rewritten/updated, as well as the concluding section (Sec. 8). The other sections (Secs. 1-6) are unchanged from the first edition of the book (published in 2005)Comment: 87 pages. 396 references. To be published as a chapter in the second edition of the book "Frustrated spin systems", edited by H. T. Diep (World-Scientific

From Neel long-range order to spin-liquids in the multiple-spin exchange model

The phase diagram of the multiple-spin exchange model on the triangular lattice is studied using exact diagonalizations. The two-spin (J_2) and four-spin (J_4) exchanges have been taken into account for 12, 16, 19, 21, 24, and 27 site samples in the parameter region J_4=0 - 0.25 (for a fixed J_2=1). It is found that the three-sublattice N\'eel ordered state built up by the pure two-spin exchange can be destroyed by the four-spin exchange, forming a spin-liquid state. The different data suggest that the phase diagram in this range of parameters exhibits two phases. The pure J_2 phase is a three-sublattice Neel ordered phase, a small J_4 drives it into a spin-liquid state with a spin gap filled of a large number of singlets. This spin-liquid phase is not of the same generic kind as the phase studied by Misguich et al. [Phys. Rev. B 60, 1064 (1999)]. It is observed on the finite-size samples that the spin liquid phase, as the Neel ordered phase, exhibits a magnetization plateau at m = 1/3, and for J_4 >0.15 a second plateau atm=1/2. These two plateaus are associated respectively to the semi-classical orderings uud and uuud.Comment: 6 pages (RevTex), 5 figures (eps). Published versio

Quantum dimer model with Z_2 liquid ground-state: interpolation between cylinder and disk topologies and toy model for a topological quantum-bit

We consider a quantum dimer model (QDM) on the kagome lattice which was introduced recently [Phys. Rev. Lett. 89, 137202 (2002)]. It realizes a Z_2 liquid phase and its spectrum was obtained exactly. It displays a topological degeneracy when the lattice has a non-trivial geometry (cylinder, torus, etc). We discuss and solve two extensions of the model where perturbations along lines are introduced: first the introduction of a potential energy term repelling (or attracting) the dimers along a line is added, second a perturbation allowing to create, move or destroy monomers. For each of these perturbations we show that there exists a critical value above which, in the thermodynamic limit, the degeneracy of the ground-state is lifted from 2 (on a cylinder) to 1. In both cases the exact value of the gap between the first two levels is obtained by a mapping to an Ising chain in transverse field. This model provides an example of solvable Hamiltonian for a topological quantum bit where the two perturbations act as a diagonal and a transverse operator in the two-dimensional subspace. We discuss how crossing the transitions may be used in the manipulation of the quantum bit to optimize simultaneously the frequency of operation and the losses due to decoherence.Comment: 11 pages, 7 (.eps) figures. Improved discussion of the destruction of the topological degeneracy and other minor corrections. Version to appear in Phys. Rev.

Twelve sublattice ordered phase in the J1-J2 model on the kagome lattice

Motivated by recent experiments on an S=1/2 antiferromagnet on the kagome lattice, we investigate the Heisenberg J1-J2 model with ferromagnetic J1 and antiferromagnetic J2. Classically the ground state displays Neel long range order with 12 non-coplanar sublattices. The order parameter has the symmetry of a cuboctahedron so that it fully breaks SO(3) as well as the spin-flip symmetry, and we expect from the latter a Z2 symmetry breaking pattern. As might be expected from the Mermin-Wagner theorem in two dimensions, the SO(3) symmetry is restored by thermal fluctuations while the Z2 symmetry breaking persists up to a finite temperature. A complete study of S=1/2 exact spectra reveals that the classical order subsists for quantum spins in a finite range of parameters. First order spin wave calculations give the range of existence of this phase and the renormalisations at T=0 of the order parameters associated to both symmetry breakings. This phase is destroyed by quantum fluctuations for a small but finite J2/|J1|\simeq3 consistently with exact spectra studies which indicate a gapped phase.Comment: Accepted for publication in Phys. Rev. B (2005

The kagome antiferromagnet: a chiral topological spin liquid ?

Inspired by the recent discovery of a new instability towards a chiral phase of the classical Heisenberg model on the kagome lattice, we propose a specific chiral spin liquid that reconciles different, well-established results concerning both the classical and quantum models. This proposal is analyzed in an extended mean-field Schwinger boson framework encompassing time reversal symmetry breaking phases which allows both a classical and a quantum phase description. At low temperatures, we find quantum fluctuations favor this chiral phase, which is stable against small perturbations of second and third neighbor interactions. For spin-1/2 this phase may be, beyond mean-field, a chiral gapped spin liquid. Such a phase is consistent with Density Matrix Renormalization Group results of Yan et al. (Science 322, 1173 (2011)). Mysterious features of the low lying excitations of exact diagonalization spectra also find an explanation in this framework. Moreover, thermal fluctuations compete with quantum ones and induce a transition from this flux phase to a planar zero flux phase at a non zero value of the renormalized temperature (T/S^2), reconciling these results with those obtained for the classical system.Comment: 4 pages, 4 figures, 1 tabl

Thermal destruction of chiral order in a two-dimensional model of coupled trihedra

We introduce a minimal model describing the physics of classical two-dimensional (2D) frustrated Heisenberg systems, where spins order in a non-planar way at T=0. This model, consisting of coupled trihedra (or Ising-$\mathbb{R}P^3$ model), encompasses Ising (chiral) degrees of freedom, spin-wave excitations and $\Z_2$ vortices. Extensive Monte Carlo simulations show that the T=0 chiral order disappears at finite temperature in a continuous phase transition in the 2D Ising universality class, despite misleading intermediate-size effects observed at the transition. The analysis of configurations reveals that short-range spin fluctuations and $\Z_2$ vortices proliferate near the chiral domain walls explaining the strong renormalization of the transition temperature. Chiral domain walls can themselves carry an unlocalized $\Z_2$ topological charge, and vortices are then preferentially paired with charged walls. Further, we conjecture that the anomalous size-effects suggest the proximity of the present model to a tricritical point. A body of results is presented, that all support this claim: (i) First-order transitions obtained by Monte Carlo simulations on several related models (ii) Approximate mapping between the Ising-$\mathbb{R}P^3$ model and a dilute Ising model (exhibiting a tricritical point) and, finally, (iii) Mean-field results obtained for Ising-multispin Hamiltonians, derived from the high-temperature expansion for the vector spins of the Ising-$\mathbb{R}P^3$ model.Comment: 15 pages, 12 figures, 1 tabl