10,195 research outputs found
Torque magnetometry study of the spin reorientation transition and temperature-dependent magnetocrystalline anisotropy in NdCo5
We present the results of torque magnetometry and magnetic susceptibility measurements to study in detail the spin reorientation transition (SRT) and magnetic anisotropy in the permanent magnet NdCo5. We further show simulations of the measurements using first-principles calculations based on density-functional theory and the disordered local moment picture of magnetism at finite temperatures. The good agreement between theory and experimental data leads to a detailed description of the physics underpinning the SRT. In particular we are able to resolve the magnetization of, and to reveal a canting between, the Nd and Co sublattices. The torque measurements carried out in the ac and ab planes near the easy direction allow us to estimate the anisotropy constants, K 1, K 2 and K 4 and their temperature dependences. Torque curves, τ(γ) recorded by varying the direction of a constant magnetic field in the crystallographic ac plane show a reversal in the polarity as the temperature is changed across the SRT (240 < T < 285 K). Within this domain, τ(γ) exhibits unusual features different to those observed above and below the transition. The single crystals of NdCo5 were grown using the optical floating zone technique
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Contains research objectives and reports on one research project.National Science Foundatio
Tunability of the spin reorientation transitions with pressure in NdCo5
We present pressure-dependent magnetization measurements carried out in the domain of the spin reorientation transitions (SRTs) of a NdCo5 single crystal. The application of a hydrostatic pressure leads to a shift in the SRTs to higher temperatures. This shift is found to be very sensitive to pressure, with the SRT temperatures increasing at a rate of ≈17 K/GPa. To explain the experimental results, we have also performed first-principles calculations of the SRT temperatures for different applied strains, which corroborate the experimental findings. The calculations attribute the pressure dependence of the SRTs to a faster weakening of the Co contribution to the magnetocrystalline anisotropy with pressure compared to the Nd contribution
Observation of magnetic fragmentation in spin ice
Fractionalised excitations that emerge from a many body system have revealed
rich physics and concepts, from composite fermions in two-dimensional electron
systems, revealed through the fractional quantum Hall effect, to spinons in
antiferromagnetic chains and, more recently, fractionalisation of Dirac
electrons in graphene and magnetic monopoles in spin ice. Even more surprising
is the fragmentation of the degrees of freedom themselves, leading to
coexisting and a priori independent ground states. This puzzling phenomenon was
recently put forward in the context of spin ice, in which the magnetic moment
field can fragment, resulting in a dual ground state consisting of a
fluctuating spin liquid, a so-called Coulomb phase, on top of a magnetic
monopole crystal. Here we show, by means of neutron scattering measurements,
that such fragmentation occurs in the spin ice candidate NdZrO. We
observe the spectacular coexistence of an antiferromagnetic order induced by
the monopole crystallisation and a fluctuating state with ferromagnetic
correlations. Experimentally, this fragmentation manifests itself via the
superposition of magnetic Bragg peaks, characteristic of the ordered phase, and
a pinch point pattern, characteristic of the Coulomb phase. These results
highlight the relevance of the fragmentation concept to describe the physics of
systems that are simultaneously ordered and fluctuating.Comment: accepted in Nature Physic
Growth, transport, and magnetic properties of Pr0.67Ca0.33MnO3 thin films
We have grown Pr0.67Ca0.33MnO3 thin films on LaAlO3 using pulsed laser deposition. Below 50 K, a field induced insulator-metal transition results in changes in resistivity of at least 6 orders of magnitude. The field induced conducting state is metastable at low temperature. The temperature dependence of the resistivity exhibits considerable hysteresis in a field of 40 kOe but becomes reversible in a field of 80 kOe
Torsion–rotation global analysis of the first three torsional states (νt = 0, 1, 2) and terahertz database for methanol
Stimulated by recent THz measurements of the methanol spectrum in one of our laboratories, undertaken in support of NASA programs related to the Herschel Space Observatory (HSO) and the Atacama Large Millimeter Array (ALMA), we have carried out a global analysis of available microwave and high-resolution infrared data for the first three torsional states (νt = 0, 1, 2), and for J values up to 30. This global fit of approximately 5600 frequency measurements and 19 000 Fourier transform far infrared (FTFIR) wavenumber measurements to 119 parameters reaches the estimated experimental measurement accuracy for the FTFIR transitions, and about twice the estimated experimental measurement accuracy for the microwave, submillimeter-wave, and terahertz transitions. The present fit is essentially a continuation of our earlier work, but we have greatly expanded our previous data set and have added a large number of new torsion–rotation interaction terms to the Hamiltonian in our previously used computer program. The results, together with a number of calculated (but unmeasured) transitions, including their line strength, estimated uncertainty, and lower state energy, are made available in the supplementary material as a database formatted to be useful for astronomical searches. Some discussion of several open spectroscopic problems, e.g., (i) an improved notation for the numerous parameters in the torsion–rotation Hamiltonian, (ii) possible causes of the failure to fit frequency measurements to the estimated measurement uncertainty, and (iii) pitfalls to be avoided when intercomparing apparently identical parameters from the internal axis method and the rho axis method are also given
Structural and Magnetic Investigations of Single-Crystals of the Neodymium Zirconate Pyrochlore, Nd2Zr2O7
We report structural and magnetic properties studies of large high quality
single-crystals of the frustrated magnet, NdZrO. Powder x-ray
diffraction analysis confirms that NdZrO adopts the pyrochlore
structure. Room-temperature x-ray diffraction and time-of-flight neutron
scattering experiments show that the crystals are stoichiometric in composition
with no measurable site disorder. The temperature dependence of the magnetic
susceptibility shows no magnetic ordering at temperatures down to 0.5 K. Fits
to the magnetic susceptibility data using a Curie-Weiss law reveal a
ferromagnetic coupling between the Nd moments. Magnetization versus field
measurements show a local Ising anisotropy along the axes of the
Nd ions in the ground state. Specific heat versus temperature
measurements in zero applied magnetic field indicate the presence of a thermal
anomaly below K, but no evidence of magnetic ordering is observed down
to 0.5 K. The experimental temperature dependence of the single-crystal bulk dc
susceptibility and isothermal magnetization are analyzed using crystal field
theory and the crystal field parameters and exchange coupling constants
determined.Comment: 10 pages, 6 figures, 4 tables. Accepted for publication in Physical
Review
Nodal superconducting gap structure in the quasi-one-dimensional CsCrAs investigated using SR measurements
The superconducting ground state of the newly discovered superconductor
CsCrAs with a quasi-one-dimensional crystal structure ( 2.1(1) K) has been investigated using magnetization and muon-spin
relaxation or rotation (SR), both zero-field (ZF) and transverse-field
(TF), measurements. Our ZF SR measurements reveal the presence of spin
fluctuations below 4 K and the ZF relaxation rate () shows enhancement
below 2.1 K, which might indicate that the superconducting
state is unconventional. This observation suggests that the electrons are
paired via unconventional channels such as spin fluctuations, as proposed on
the basis of theoretical models. Our analysis of the TF SR results shows
that the temperature dependence of the superfluid density is fitted better with
a nodal gap structure than an isotropic s-wave model for the superconducting
gap. The observation of a nodal gap in CsCrAs is consistent with
that observed in the isostructural KCrAs compound through TF
SR measurements. Furthermore, from our TF SR study we have estimated
the magnetic penetration depth = 954 nm,
superconducting carrier density m, and
carrier's effective-mass enhancement = 1.61m.Comment: 7 pages, 4 figures. arXiv admin note: substantial text overlap with
arXiv:1505.0574
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