A solid state spin-wave quantum memory for time-bin qubits

We demonstrate the first solid-state spin-wave optical quantum memory with on-demand read-out. Using the full atomic frequency comb scheme in a \PrYSO crystal, we store weak coherent pulses at the single-photon level with a signal to noise ratio $> 10$. Narrow-band spectral filtering based on spectral hole burning in a second \PrYSO crystal is used to filter out the excess noise created by control pulses to reach an unconditional noise level of $(2.0 \pm 0.3) \times10^{-3}$ photons per pulse. We also report spin-wave storage of photonic time-bin qubits with conditional fidelities higher than a measure and prepare strategy, demonstrating that the spin-wave memory operates in the quantum regime. This makes our device the first demonstration of a quantum memory for time-bin qubits, with on demand read-out of the stored quantum information. These results represent an important step for the use of solid-state quantum memories in scalable quantum networks.Comment: 10 pages, 10 figure

Photon echo without a free induction decay in a double-Lambda system

We have characterized a novel photon-echo pulse sequence for a double-$\Lambda$ type energy level system where the input and rephasing transitions are different to the applied $\pi$-pulses. We show that despite having imperfect $\pi$-pulses (associated with large coherent emission due to free induction decay), the noise added is only 0.019$\pm$0.001 relative to the shot noise in the spectral mode of the echo. Using this echo pulse sequence in the `rephased amplified spontaneous emission' (RASE) scheme \cite{Ledingham2010} will allow for generation of entangled photon pairs that are in different frequency, temporal, and potentially spatial modes to any bright driving fields. The coherence and efficiency properties of this sequence were characterized in a Pr:YSO crystal

Coherent Storage of Temporally Multimode Light Using a Spin-Wave Atomic Frequency Comb Memory

We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory is promising as a quantum memory for light.Comment: 17 pages, 5 figure

Non-classical photon streams using rephased amplified spontaneous emission

We present a fully quantum mechanical treatment of optically rephased photon echoes. These echoes exhibit noise due to amplified spontaneous emission, however this noise can be seen as a consequence of the entanglement between the atoms and the output light. With a rephasing pulse one can get an "echo" of the amplified spontaneous emission, leading to light with nonclassical correlations at points separated in time, which is of interest in the context of building wide bandwidth quantum repeaters. We also suggest a wideband version of DLCZ protocol based on the same ideas.Comment: 5 pages, 4 figures. Added section

Storage of up-converted telecom photons in a doped crystal

We report on an experiment that demonstrates the frequency up-conversion of telecommunication wavelength single-photon-level pulses to be resonant with a $\mathrm{Pr}^{3+}$:$\mathrm{Y}_2\mathrm{Si}\mathrm{O}_5$ crystal. We convert the telecom photons at $1570\,\mathrm{nm}$ to $606\,\mathrm{nm}$ using a periodically-poled potassium titanyl phosphate nonlinear waveguide. The maximum device efficiency (which includes all optical loss) is inferred to be $\eta_{\mathrm{dev}}^{\mathrm{max}} = 22 \pm 1\,$ (internal efficiency $\eta_{\mathrm{int}} = 75\pm8\,$) with a signal to noise ratio exceeding 1 for single-photon-level pulses with durations of up to 560$\,$ns. The converted light is then stored in the crystal using the atomic frequency comb scheme with storage and retrieval efficiencies exceeding $\eta_{\mathrm{AFC}} = 20\,$ for predetermined storage times of up to $5\,\mu\mathrm{s}$. The retrieved light is time delayed from the noisy conversion process allowing us to measure a signal to noise ratio exceeding 100 with telecom single-photon-level inputs. These results represent the first demonstration of single-photon-level optical storage interfaced with frequency up-conversion

Experimental realization of light with time separated correlations by rephasing amplified spontaneous emission

Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a {\pi}-pulse, resulting in amplified spontaneous emission. The application of a second {\pi}-pulse leads to a coherent echo of the amplified spontaneous emission that is correlated in both amplitude and phase. For small optical thicknesses, we see evidence that the amplified spontaneous emission and its echo are entangled.Comment: 6 pages, 5 figures, the supplementary information pdf was uploaded with latex source files. This version accepted for publication in PR

Quantum Storage of a Photonic Polarization Qubit in a Solid

We report on the quantum storage and retrieval of photonic polarization quantum bits onto and out of a solid state storage device. The qubits are implemented with weak coherent states at the single photon level, and are stored for 500 ns in a praseodymium doped crystal with a storage and retrieval efficiency of 10%, using the atomic frequency comb scheme. We characterize the storage by using quantum state tomography, and find that the average conditional fidelity of the retrieved qubits exceeds 95% for a mean photon number mu=0.4. This is significantly higher than a classical benchmark, taking into account the Poissonian statistics and finite memory efficiency, which proves that our device functions as a quantum storage device for polarization qubits, even if tested with weak coherent states. These results extend the storage capabilities of solid state quantum memories to polarization encoding, which is widely used in quantum information science.Comment: 6 pages, 6 figures, 1 table. New reference adde

Raman Quantum Memory with Built-In Suppression of Four-wave Mixing Noise

Quantum memories are essential for large-scale quantum information networks. Along with high efficiency, storage lifetime and optical bandwidth, it is critical that the memory add negligible noise to the recalled signal. A common source of noise in optical quantum memories is spontaneous four-wave mixing. We develop and implement a technically simple scheme to suppress this noise mechanism by means of quantum interference. Using this scheme with a Raman memory in warm atomic vapour we demonstrate over an order of magnitude improvement in noise performance. Furthermore we demonstrate a method to quantify the remaining noise contributions and present a route to enable further noise suppression. Our scheme opens the way to quantum demonstrations using a broadband memory, significantly advancing the search for scalable quantum photonic networks.Comment: 6 pages, 5 figures plus Supplementary Materia

Experimental demonstration of quantum effects in the operation of microscopic heat engines

The heat engine, a machine that extracts useful work from thermal sources, is one of the basic theoretical constructs and fundamental applications of classical thermodynamics. The classical description of a heat engine does not include coherence in its microscopic degrees of freedom. By contrast, a quantum heat engine might possess coherence between its internal states. Although the Carnot efficiency cannot be surpassed, and coherence can be performance degrading in certain conditions, it was recently predicted that even when using only thermal resources, internal coherence can enable a quantum heat engine to produce more power than any classical heat engine using the same resources. Such a power boost therefore constitutes a quantum thermodynamic signature. It has also been shown that the presence of coherence results in the thermodynamic equivalence of different quantum heat engine types, an effect with no classical counterpart. Microscopic heat machines have been recently implemented with trapped ions, and proposals for heat machines using superconducting circuits and optomechanics have been made. When operated with standard thermal baths, however, the machines implemented so far have not demonstrated any inherently quantum feature in their thermodynamic quantities. Here we implement two types of quantum heat engines by use of an ensemble of nitrogen-vacancy centres in diamond, and experimentally demonstrate both the coherence power boost and the equivalence of different heat-engine types. This constitutes the first observation of quantum thermodynamic signatures in heat machines