6,477 research outputs found
Thermodynamic and magnetic properties of the layered triangular magnet NaNiO2
We report muon-spin rotation, heat capacity, magnetization, and ac magnetic
susceptibility measurements of the layered spin-1/2 antiferromagnet NaNiO2.
These show the onset of long-range magnetic order below T_N = 19.5K. Rapid muon
depolarization persisting to about 5K above T_N is consistent with the presence
of short-range magnetic order. The temperature and frequency dependence of the
ac susceptibility suggests that magnetic clusters persist above 25K in the
paramagnetic state and that their volume fraction decreases with increasing
temperature. A frequency dependent peak in the ac magnetic susceptibility at
T_sf = 3K is observed, consistent with a slowing of spin fluctuations at this
temperature. A partial magnetic phase diagram is deduced.Comment: 4 pages, 4 figure
Anomalous temperature evolution of the internal magnetic field distribution in the charge-ordered triangular antiferromagnet AgNiO2
Zero-field muon-spin relaxation measurements of the frustrated triangular
quantum magnet AgNiO2 are consistent with a model of charge disproportionation
that has been advanced to explain the structural and magnetic properties of
this compound. Below an ordering temperature of T_N=19.9(2) K we observe six
distinct muon precession frequencies, due to the magnetic order, which can be
accounted for with a model describing the probable muon sites. The precession
frequencies show an unusual temperature evolution which is suggestive of the
separate evolution of two opposing magnetic sublattices.Comment: 4 pages, 3 figure
Two-dimensional magnetism in the pnictide superconductor parent material SrFeAsF probed by muon-spin relaxation
We report muon-spin relaxation measurements on SrFeAsF, which is the parent
compound of a newly discovered iron-arsenic-fluoride based series of
superconducting materials. We find that this material has very similar magnetic
properties to LaFeAsO, such as separated magnetic and structural transitions
(TN = 120 K, Ts = 175 K), contrasting with SrFe2As2 where they are coincident.
The muon oscillation frequencies fall away very sharply at TN, which suggests
that the magnetic exchange between the layers is weaker than in comparable
oxypnictide compounds. This is consistent with our specific heat measurements,
which find that the entropy change S = 0.05 J/mol/K largely occurs at the
structural transition and there is no anomaly at TN.Comment: 4 pages, 3 figure
How to Test for Diagonalizability: The Discretized PT-Invariant Square-Well Potential
Given a non-hermitean matrix M, the structure of its minimal polynomial
encodes whether M is diagonalizable or not. This note will explain how to
determine the minimal polynomial of a matrix without going through its
characteristic polynomial. The approach is applied to a quantum mechanical
particle moving in a square well under the influence of a piece-wise constant
PT-symmetric potential. Upon discretizing the configuration space, the system
is decribed by a matrix of dimension three. It turns out not to be
diagonalizable for a critical strength of the interaction, also indicated by
the transition of two real into a pair of complex energy eigenvalues. The
systems develops a three-fold degenerate eigenvalue, and two of the three
eigenfunctions disappear at this exceptional point, giving a difference between
the algebraic and geometric multiplicity of the eigenvalue equal to two.Comment: 5 page
Magnetic order in the quasi-one-dimensional spin 1/2 chain, copper pyrazine dinitrate
We present the first evidence of magnetic order in the quasi-one-dimensional
spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}.
Zero field muon-spin relaxation measurements made at dilution refrigerator
temperatures show oscillations in the measured asymmetry, characteristic of a
quasistatic magnetic field at the muon sites. Our measurements provide
convincing evidence for long range magnetic order below a temperature
T_N=107(1) mK. This leads to an estimate of the interchain coupling constant of
|J'|/k_B=0.046 K and to a ratio |J'/J| = 4.4 x 10^-3.Comment: 4 pages, 3 figures. Submitted to Physical Review Letter
Spin freezing and dynamics in Ca_{3}Co_{2-x}Mn_{x}O_{6} (x ~ 0.95) investigated with implanted muons: disorder in the anisotropic next-nearest neighbor Ising model
We present a muon-spin relaxation investigation of the Ising chain magnet
Ca_{3}Co_{2-x}Mn_{x}O_{6} (x~0.95). We find dynamic spin fluctuations
persisting down to the lowest measured temperature of 1.6 K. The previously
observed transition at around T ~18 K is interpreted as a subtle change in
dynamics for a minority of the spins coupling to the muon that we interpret as
spins locking into clusters. The dynamics of this fraction of spins freeze
below a temperature T_{SF}~8 K, while a majority of spins continue to
fluctuate. An explanation of the low temperature behavior is suggested in terms
of the predictions of the anisotropic next-nearest-neighbor Ising model.Comment: 4 pages, 2 figure
Muon-spin relaxation and heat capacity measurements on the magnetoelectric and multiferroic pyroxenes LiFeSi2O6 and NaFeSi2O6
The results of muon-spin relaxation and heat capacity measurements on two
pyroxene compounds LiFeSi2O6 and NaFeSi2O6 demonstrate that despite their
underlying structural similarity the magnetic ordering is considerably
different. In LiFeSi2O6 a single muon precession frequency is observed below
TN, consistent with a single peak at TN in the heat capacity and a commensurate
magnetic structure. In applied magnetic fields the heat capacity peak splits in
two. In contrast, for natural NaFeSi2O6, where multiferroicity has been
observed in zero-magnetic-field, a rapid Gaussian depolarization is observed
showing that the magnetic structure is more complex. Synthetic NaFeSi2O6 shows
a single muon precession frequency but with a far larger damping rate than in
the lithium compound. Heat capacity measurements reproduce the phase diagrams
previously derived from other techniques and demonstrate that the magnetic
entropy is mostly associated with the build up of correlations in the
quasi-one-dimensional Fe3+ chains
The phase transition in the localized ferromagnet EuO probed by muSR
We report results of muon spin rotation measurements performed on the
ferromagnetic semiconductor EuO, which is one of the best approximations to a
localized ferromagnet. We argue that implanted muons are sensitive to the
internal field primarily through a combination of hyperfine and Lorentz fields.
The temperature dependences of the internal field and the relaxation rate have
been measured and are compared with previous theoretical predictions.Comment: 4 pages, 4 figure
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