Enhanced Spontaneous Emission Into The Mode Of A Cavity QED System

We study the light generated by spontaneous emission into a mode of a cavity QED system under weak excitation of the orthogonally polarized mode. Operating in the intermediate regime of cavity QED with comparable coherent and decoherent coupling constants, we find an enhancement of the emission into the undriven cavity mode by more than a factor of 18.5 over that expected by the solid angle subtended by the mode. A model that incorporates three atomic levels and two polarization modes quantitatively explains the observations.Comment: 9 pages, 2 figures, to appear in May 2007 Optics Letter

Kaolinite-catalyzed air oxidation of hydrazine: Consideration of several compositional, structural and energetic factors in surface activation

Clay minerals have been shown to have numerous, curious, energetic properties by virtue of ultra-violet light release which can be triggered by gentle environmental changes such as wetting and dewetting by a variety of liquids, unique among them water and hydrazine. Since both water and hydrazine play multiple key roles in the air-oxidation of hydrazine on kaolinite surfaces, this reaction would seem to have prime potential for studying interrelationships of energy storage, release and chemical reactivity of clay surfaces, capacities basic to either the Bernal or Cairns-Smith roles of minerals in the origin of life. Establishment of the capacity for stored electronic energy to significantly alter surface chemistry is important, regardless of the reaction chosen to demonstrate it. Hydrazine air oxidation is overawingly complex, given the possibilities for step-wise control and monitoring of parameters. In the light of recently extended characterization of the kaolinite and model sheet catalysts we used to study hydrazine oxidation and gamma-irradiated silica, previous studies of hydrazine air-oxidation on aluminosilicate surfaces have been reevaluated. Our former conclusion remains intact that, whereas trace structural and surface contaminants do play some role in the catalysis of oxidation, they are not the only, nor even the dominant, catalytic centers. Initial intermediates in the oxidation can now be proposed which are consistent with production via O(-)-centers as well as ferric iron centers. The greater than square dependence of the initial reaction rate on the weight of the clay is discussed in the light of these various mechanistic possibilities

3-D Photoionization Structure and Distances of Planetary Nebulae III. NGC 6781

Continuing our series of papers on the three-dimensional (3-D) structures of and accurate distances to Planetary Nebulae (PNe), we present our study of the planetary nebula NGC6781. For this object we construct a 3-D photoionization model and, using the constraints provided by observational data from the literature we determine the detailed 3-D structure of the nebula, the physical parameters of the ionizing source and the first precise distance. The procedure consists in simultaneously fitting all the observed emission line morphologies, integrated intensities and the 2-D density map from the [SII] line ratios to the parameters generated by the model, and in an iterative way obtain the best fit for the central star parameters and the distance to NGC6781, obtaining values of 950+-143pc and 385 Lsun for the distance and luminosity of the central star respectively. Using theoretical evolutionary tracks of intermediate and low mass stars, we derive the mass of the central star of NGC6781 and its progenitor to be 0.60+-0.03 Msun and 1.5+-0.5 Msun respectively.Comment: 16 pp, 6 figues, 2 tables, submitted to the Ap

Steady State Entanglement in Cavity QED

We investigate steady state entanglement in an open quantum system, specifically a single atom in a driven optical cavity with cavity loss and spontaneous emission. The system reaches a steady pure state when driven very weakly. Under these conditions, there is an optimal value for atom-field coupling to maximize entanglement, as larger coupling favors a loss port due to the cavity enhanced spontaneous emission. We address ways to implement measurements of entanglement witnesses and find that normalized cross-correlation functions are indicators of the entanglement in the system. The magnitude of the equal time intensity-field cross correlation between the transmitted field of the cavity and the fluorescence intensity is proportional to the concurrence for weak driving fields.Comment: enhanced discussion, corrected formulas, title change, 1 added figur

Strong Coupling Expansions for Antiferromagnetic Heisenberg S=1/2 Ladders

The properties of antiferromagnetic Heisenberg $S=\frac{1}{2}$ ladders with 2, 3, and 4 chains are expanded in the ratio of the intra- and interchain coupling constants. A simple mapping procedure is introduced to relate the 4 and 2-chain ladders which holds down to moderate values of the expansion parameters. A second order calculation of the spin gap to the lowest triplet excitation in the 2- and 4-chain ladders is found to be quite accurate even at the isotropic point where the couplings are equal. Similar expansions and mapping procedures are presented for the 3-chain ladders which are in the same universality class as single chains.Comment: 10 physical pages, uuencoded compressed PostScript file including 12 figures, ETH-TH/942

Temperature dependent photoluminescence of single CdS nanowires

Temperature dependent photoluminescence (PL) is used to study the electronic properties of single CdS nanowires. At low temperatures, both near-band edge (NBE) photoluminescence (PL) and spatially-localized defect-related PL are observed in many nanowires. The intensity of the defect states is a sensitive tool to judge the character and structural uniformity of nanowires. As the temperature is raised, the defect states rapidly quench at varying rates leaving the NBE PL which dominates up to room temperature. All PL lines from nanowires follow closely the temperature-dependent band edge, similar to that observed in bulk CdS.Comment: 11 pages, 4 figure