Plasma Processing of Large Curved Surfaces for SRF Cavity Modification

Plasma based surface modification of niobium is a promising alternative to wet etching of superconducting radio frequency (SRF) cavities. The development of the technology based on Cl2/Ar plasma etching has to address several crucial parameters which influence the etching rate and surface roughness, and eventually, determine cavity performance. This includes dependence of the process on the frequency of the RF generator, gas pressure, power level, the driven (inner) electrode configuration, and the chlorine concentration in the gas mixture during plasma processing. To demonstrate surface layer removal in the asymmetric non-planar geometry, we are using a simple cylindrical cavity with 8 ports symmetrically distributed over the cylinder. The ports are used for diagnosing the plasma parameters and as holders for the samples to be etched. The etching rate is highly correlated with the shape of the inner electrode, radio-frequency (RF) circuit elements, chlorine concentration in the Cl2/Ar gas mixtures, residence time of reactive species and temperature of the cavity. Using cylindrical electrodes with variable radius, large-surface ring-shaped samples and d.c. bias implementation in the external circuit we have demonstrated substantial average etching rates and outlined the possibility to optimize plasma properties with respect to maximum surface processing effect

Resonant-Frequency Discharge in a Multi-Cell Radio Frequency Cavity

We are reporting experimental results on a microwave discharge operating at resonant frequency in a multi-cell radio frequency (RF) accelerator cavity. Although the discharge operated at room temperature, the setup was constructed so that it could be used for plasma generation and processing in fully assembled active superconducting radio-frequency cryo-module. This discharge offers a mechanism for removal of a variety of contaminants, organic or oxide layers, and residual particulates from the interior surface of RF cavities through the interaction of plasma-generated radicals with the cavity walls. We describe resonant RF breakdown conditions and address the issues related to resonant detuning due to sustained multi-cell cavity plasma. We have determined breakdown conditions in the cavity, which was acting as a plasma vessel with distorted cylindrical geometry. We discuss the spectroscopic data taken during plasma removal of contaminants and use them to evaluate plasma parameters, characterize the process, and estimate the volatile contaminant product removal

On Wheeler's delayed-choice Gedankenexperiment and its laboratory realization

Here, we present an analysis and interpretation of the experiment performed by Jacques et al. (2007 Science 315, 966), which represents a realization of Wheeler's delayed-choice Gedankenexperiment. Our analysis is based on the evolution of the photon state, since the photon enters into the Mach-Zehnder interferometer with a removable beam-splitter until it exits. Given the same incident photon state onto the output beam-splitter, BS_output, the photon's state at the exit will be very different depending on whether BS_output is on or off. Hence, the statistics of photon counts collected by the two detectors, positioned along orthogonal directions at the exit of the interferometer, is also going to be very different in either case. Therefore, it is not that the choice of inserting (on) or removing (off) a beam-splitter leads to a delayed influence on the photon behavior before arriving at the beam-splitter, but that such a choice influences the photon state at and after BS_output, i.e., after it has exited from the Mach-Zehnder interferometer. The random on/off choice at BS_output has no delayed effect on the photon to behave as a wave or a corpuscle at the entrance and inside the interferometer, but influences the subsequent evolution of the photon state incident onto BS_output.Comment: 7 pages, 4 figure

Characterizing Plasma with Emission Tomography-Feasibility Study on Synthetic and Experimental Data

We present a feasibility study on different tomographic algorithms to overcome the issues of finite sets of projection data, limited viewing angles, and noisy data, which cause the tomographic reconstruction to be an ill-posed inversion problem. We investigated three approaches: single angle Abel inversion, two angle approach, and multiple angle 2D plasma tomography. These methods were tested on symmetric and asymmetric sample functions and on experimental results from a supersonic flowing argon microwave plasma sustained in a cylindrical quartz cavity. The analysis focused on the afterglow region of the microwave flow where a plasmoid-like formation was observed. We investigated the effects of the uniform random noise added to the simulated data by applying smoothing techniques. The quality of reconstructed images was assessed by using peak signal-to-noise ratio and universal quality image measures. The results showed that the Abel inversion approach could be employed only when the system is radially symmetric, while the systems with slight asymmetry could be reconstructed with the two angle approach. In the complete absence of symmetry, full 2D tomographic reconstruction should be applied. The data analysis showed that the best results were obtained by employing either the filtered back projection or the simultaneous algebraic reconstruction technique. The total variation minimization method proved to be the best denoising technique. Each approach was used to obtain the spatial distributions of argon excited states taken at three positions along the plasmoid-like structure. The results indicated that the plasma was asymmetric with argon populating the cavity surface

Effect of Self-Bias on Cylindrical Capacitive Discharge for Processing of Inner Walls of Tubular Structures-Case of SRF Cavities

Cylindrical capacitive discharge is a convenient medium for generating reactive ions to process inner walls superconductive radio-frequency (SRF) cavities. These cavities, used in particle accelerators, presents a three-dimensional structure made of bulk Niobium, with axial cylindrical symmetry. Manufactured cavity walls are covered with Niobium oxides and scattered particulates, which must be removed for desired SRF performance. Cylindrical capacitive discharge in a mixture of Ar and Cl2 is a sole and natural non-wet acid choice to purify the inner surfaces of SRF cavities by reactive ion etching. Coaxial cylindrical discharge is generated between a powered inner electrode and the grounded outer electrode, which is the cavity wall to be etched. Plasma sheath voltages were tailored to process the outer wall by providing an additional dc current to the inner electrode with the help of an external compensating dc power supply and corrugated design of the inner electrode. The dc bias potential difference is established between two electrodes to make the set-up favorable for SRF wall processing. To establish guidelines for reversing the asymmetry and establishing the optimal sheath voltage at the cavity wall, the dc self-bias potential and dc current dependence on process parameters, such as gas pressure, rf power and chlorine content in the Ar/Cl2 gas mixture was measured. The process is potentially applicable to all concave metallic surfaces. © 2018 Author(s)

Characterization of the Supersonic Flowing Microwave Discharge Using Two Dimensional Plasma Tomography

A tomographic numerical method based on the two-dimensional Radon formula for a cylindrical cavity has been employed for obtaining spatial distributions of the argon excited levels. The spectroscopy measurements were taken at different positions and directions to observe populations of excited species in the plasmoid region and the corresponding excitation temperatures. Excited argon states are concentrated near the tube walls, thus, confirming the assumption that the post discharge plasma is dominantly sustained by travelling surface wave. An automated optical measurement system has been developed for reconstruction of local plasma parameters of the plasmoid structure formed in an argon supersonic flowing microwave discharge. The system carries out angle and distance measurements using a rotating, flat mirror, as well as two high precision stepper motors operated by a microcontroller-based system and several sensors for precise feedback control

Plasma Processing of Large Curved Surfaces for Superconducting rf Cavity Modification

Plasma-based surface modification of niobium is a promising alternative to wet etching of superconducting radio frequency (SRF) cavities. We have demonstrated surface layer removal in an asymmetric nonplanar geometry, using a simple cylindrical cavity. The etching rate is highly correlated with the shape of the inner electrode, radio-frequency (rf) circuit elements, gas pressure, rf power, chlorine concentration in the Cl2/Ar gas mixtures, residence time of reactive species, and temperature of the cavity. Using variable radius cylindrical electrodes, large-surface ring-shaped samples, and dc bias in the external circuit, we have measured substantial average etching rates and outlined the possibility of optimizing plasma properties with respect to maximum surface processing effect