92 research outputs found
Acoustic and optical phonon dynamics from femtosecond time-resolved optical spectroscopy of superconducting iron pnictide Ca(Fe_0.944Co_0.056)_2As_2
We report temperature evolution of coherently excited acoustic and optical
phonon dynamics in superconducting iron pnictide single crystal
Ca(Fe_0.944Co_0.056)_2As_2 across the spin density wave transition at T_SDW ~
85 K and superconducting transition at T_SC ~20 K. Strain pulse propagation
model applied to the generation of the acoustic phonons yields the temperature
dependence of the optical constants, and longitudinal and transverse sound
velocities in the temperature range of 3.1 K to 300 K. The frequency and
dephasing times of the phonons show anomalous temperature dependence below T_SC
indicating a coupling of these low energy excitations with the Cooper-pair
quasiparticles. A maximum in the amplitude of the acoustic modes at T ~ 170 is
seen, attributed to spin fluctuations and strong spin-lattice coupling before
T_SDW.Comment: 6 pages, 4 figures (revised manuscript
Ultrafast quasiparticle dynamics in superconducting iron pnictide CaFe1.89Co0.11As2
Nonequilibrium quasiparticle relaxation dynamics is reported in
superconducting CaFe1.89Co0.11As2 single crystal using femtosecond
time-resolved pump-probe spectroscopy. The carrier dynamics reflects a
three-channel decay of laser deposited energy with characteristic time scales
varying from few hundreds of femtoseconds to order of few nanoseconds where the
amplitudes and time-constants of the individual electronic relaxation
components show significant changes in the vicinity of the spin density wave
(T_SDW ~ 85 K) and superconducting (T_SC ~ 20 K) phase transition temperatures.
The quasiparticles dynamics in the superconducting state reveals a charge gap
with reduced gap value of 2_0/k_BT_SC ~ 1.8. We have determined the
electron-phonon coupling constant \lemda to be ~ 0.14 from the temperature
dependent relaxation time in the normal state, a value close to those reported
for other types of pnictides. From the peculiar temperature-dependence of the
carrier dynamics in the intermediate temperature region between the
superconducting and spin density wave phase transitions, we infer a temperature
scale where the charge gap associated with the spin ordered phase is maximum
and closes on either side while approaching the two phase transition
temperatures.Comment: 6 pages, 4 figures (revised manuscript);
http://dx.doi.org/10.1016/j.ssc.2013.02.00
Phonon Anomalies, Orbital-Ordering and Electronic Raman Scattering in iron-pnictide Ca(Fe0.97Co0.03)2As2: Temperature-dependent Raman Study
We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a
wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal
to orthorhombic structural transition as well as magnetic transition at Tsm ~
160K. The mode frequencies of two first-order Raman modes B1g and Eg, both
involving displacement of Fe atoms, show sharp increase below Tsm.
Concomitantly, the linewidths of all the first-order Raman modes show anomalous
broadening below Tsm, attributed to strong spin-phonon coupling. The high
frequency modes observed between 400-1200 cm-1 are attributed to the electronic
Raman scattering involving the crystal field levels of d-orbitals of Fe2+. The
splitting between xz and yz d-orbital levels is shown to be ~ 25 meV which
increases as temperature decreases below Tsm. A broad Raman band observed at ~
3200 cm-1 is assigned to two-magnon excitation of the itinerant Fe 3d
antiferromagnet.Comment: Accepted for Publication in JPC
Fishtail effect and vortex dynamics in LiFeAs single crystals
We investigate the fishtail effect, critical current density () and
vortex dynamics in LiFeAs single crystals. The sample exhibits a second peak
(SP) in the magnetization loop only with the field c-axis. We calculate a
reasonably high , however, values are lower than in 'Ba-122' and
'1111'-type FeAs-compounds. Magnetic relaxation data imply a strong pinning
which appears not to be due to conventional defects. Instead, its behavior is
similar to that of the triplet superconductor SrRuO. Our data suggest
that the origin of the SP may be related to a vortex lattice phase transition.
We have constructed the vortex phase diagram for LiFeAs on the
field-temperature plane.Comment: 5 pages, 5 figure
Incommensurate antiferromagnetic fluctuations in single-crystalline LiFeAs studied by inelastic neutron scattering
We present an inelastic neutron scattering study on single-crystalline LiFeAs
devoted to the characterization of the incommensurate antiferromagnetic
fluctuations at . Time-of-flight
measurements show the presence of these magnetic fluctuations up to an energy
transfer of 60 meV, while polarized neutrons in combination with longitudinal
polarization analysis on a triple-axis spectrometer prove the pure magnetic
origin of this signal. The normalization of the magnetic scattering to an
absolute scale yields that magnetic fluctuations in LiFeAs are by a factor
eight weaker than the resonance signal in nearly optimally Co-doped
BaFeAs, although a factor two is recovered due to the split peaks owing
to the incommensurability. The longitudinal polarization analysis indicates
weak spin space anisotropy with slightly stronger out-of-plane component
between 6 and 12 meV. Furthermore, our data suggest a fine structure of the
magnetic signal most likely arising from superposing nesting vectors.Comment: 9 pages, 8 figure
Resistivity and Hall effect of LiFeAs: Evidence for electron-electron scattering
LiFeAs is unique among the broad family of FeAs-based superconductors,
because it is superconducting with a rather large K under
ambient conditions although it is a stoichiometric compound. We studied the
electrical transport on a high-quality single crystal. The resistivity shows
quadratic temperature dependence at low temperature giving evidence for strong
electron-electron scattering and a tendency towards saturation around room
temperature. The Hall constant is negative and changes with temperature, what
most probably arises from a van Hove singularity close to the Fermi energy in
one of the hole-like bands. Using band structure calculations based on angular
resolved photoemission spectra we are able to reproduce all the basic features
of both the resistivity as well as the Hall effect data.Comment: 6 pages, 3 figures included; V2 has been considerably revised and
contain a more detailed analysis of the Hall effect dat
- …