1,003 research outputs found

    Instability due to long range Coulomb interaction in a liquid of polarizable particles (polarons, etc.)

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    The interaction Hamiltonian for a system of polarons a la Feynman in the presence of long range Coulomb interaction is derived and the dielectric function is computed in mean field. For large enough concentration a liquid of such particles becomes unstable. The onset of the instability is signaled by the softening of a collective optical mode in which all electrons oscillate in phase in their respective self-trapping potential. We associate the instability with a metallization of the system. Optical experiments in slightly doped cuprates and doped nickelates are analyzed within this theory. We discuss why doped cuprates matallize whereas nickelates do not.Comment: 5 pages,1 figur

    Photoemission spectroscopy and sum rules in dilute electron-phonon systems

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    A family of exact sum rules for the one-polaron spectral function in the low-density limit is derived. An algorithm to calculate energy moments of arbitrary order of the spectral function is presented. Explicit expressions are given for the first two moments of a model with general electron-phonon interaction, and for the first four moments of the Holstein polaron. The sum rules are linked to experiments on momentum-resolved photoemission spectroscopy. The bare electronic dispersion and the electron-phonon coupling constant can be extracted from the first and second moments of spectrum. The sum rules could serve as constraints in analytical and numerical studies of electron-phonon models.Comment: 4 page

    Model ab initio study of charge carrier solvation and large polaron formation on conjugated carbon chains

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    Using long C_{N}H_{2} conjugated carbon chains with the polyynic structure as prototypical examples of one-dimensional (1D) semiconductors, we discuss self-localization of excess charge carriers into 1D large polarons in the presence of the interaction with a surrounding polar solvent. The solvation mechanism of self-trapping is different from the polaron formation due to coupling with bond-length modulations of the underlying atomic lattice well-known in conjugated polymers. Model ab initio computations employing the hybrid B3LYP density functional in conjunction with the polarizable continuum model are carried out demonstrating the formation of both electron- and hole-polarons. Polarons can emerge entirely due to solvation but even larger degrees of charge localization occur when accompanied by atomic displacements

    Monitoring 2009 Forest Disturbance Across the Conterminous United States, Based on Near-Real Time and Historical MODIS 250 Meter NDVI Products

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    This case study shows the promise of computing current season forest disturbance detection products at regional to CONUS scales. Use of the eMODIS expedited product enabled a NRT CONUS forest disturbance detection product, a requirement for an eventual, operational forest threat EWS. The 2009 classification product from this study can be used to quantify the areal extent of forest disturbance across CONUS, although a quantitative accuracy assessment still needs to be completed. However, the results would not include disturbances that occurred after July 27, such as the Station Fire. While not shown here, the project also produced maximum NDVI products for the June 10-July 27 period of each year of the 2000-2009 time frame. These products could be applied to compute forest change products on an annual basis. GIS could then be used to assess disturbance persistence. Such follow-on work could lead to attribution of year in which a disturbance occurred. These products (e.g., Figures 6 and 7) may also be useful for assessing forest change associated with climate change, such as carbon losses from bark beetle-induced forest mortality in the Western United States. Other MODIS phenological products are being assessed for aiding forest monitoring needs of the EWS, including cumulative NDVI products (Figure 10)

    Tilting instability and other anomalies in the flux-lattice in some magnetic superconductors

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    The flux-line lattice in the compound ErNi2B2CErNi_2B_2C, which has a tendency to ferromagnetic order in the a-b plane is studied with external magnetic field direction close to the c-axis. We show the existence of an instability where the direction of flux-lines spontaneously tilts away from that of the applied field near the onset of ferromagnetic order. The enhanced fluctuations in the flux lattice and the square flux lattice recently observed are explained and further experiments suggested.Comment: 12 pages, Latex file, no figur

    Phonon Coherence and New Set of Sidebands in Phonon-Assisted Photoluminescence

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    We investigate excitonic polaron states comprising a local exciton and phonons in the longitudinal optical (LO) mode by solving the Schr\"{o}dinger equation. We derive an exact expression for the ground state (GS), which includes multi-phonon components with coefficients satisfying the Huang-Rhys factors. The recombination of GS and excited polaron states gives one set of sidebands in photoluminescence (PL): the multi-phonon components in the GS produce the Stokes lines and the zero-phonon components in the excited states produce the anti-Stokes lines. By introducing the mixing of the LO mode and environal phonon modes, the exciton will also couple with the latter, and the resultant polaron states result in another set of phonon sidebands. This set has a zero-phonon line higher and wider than that of the first set due to the tremendous number of the environal modes. The energy spacing between the zero-phonon lines of the first and second sets is proved to be the binding energy of the GS state. The common exciton origin of these two sets can be further verified by a characteristic Fano lineshape induced by the coherence in the mixing of the LO and the environal modes.Comment: 5 pages, 3 figures 1 figure (fig. 1) replaced 1 figure (fig. 2) remove

    An exactly solvable phase transition model: generalized statistics and generalized Bose-Einstein condensation

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    In this paper, we present an exactly solvable phase transition model in which the phase transition is purely statistically derived. The phase transition in this model is a generalized Bose-Einstein condensation. The exact expression of the thermodynamic quantity which can simultaneously describe both gas phase and condensed phase is solved with the help of the homogeneous Riemann-Hilbert problem, so one can judge whether there exists a phase transition and determine the phase transition point mathematically rigorously. A generalized statistics in which the maximum occupation numbers of different quantum states can take on different values is introduced, as a generalization of Bose-Einstein and Fermi-Dirac statistics.Comment: 17 pages, 2 figure

    Quantum Simulations of Extended Hubbard Models with Dipolar Crystals

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    In this paper we study the realization of lattice models in mixtures of atomic and dipolar molecular quantum gases. We consider a situation where polar molecules form a self-assembled dipolar lattice, in which atoms or molecules of a second species can move and scatter. We describe the system dynamics in a master equation approach in the Brownian motion limit of slow particles and fast phonons, which we find appropriate for our system. In a wide regime of parameters, the reduced dynamics of the particles leads to physical realizations of extended Hubbard models with tuneable long-range interactions mediated by crystal phonons. This extends the notion of quantum simulation of strongly correlated systems with cold atoms and molecules to include phonon-dynamics, where all coupling parameters can be controlled by external fields.Comment: 44 pages, 14 figure

    Absence of Meissner State and Robust Ferromagnetism in the Superconducting State of UCoGe: Possible Evidence of Spontaneous Vortex State

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    We report ac magnetic susceptibility and dc magnetization measurements on the superconducting ferromagnet UCoGe (with superconducting and Curie temperatures of TSC∼0.5T_{{\rm SC}} \sim 0.5~K and TCurie∼2.5T_{{\rm Curie}} \sim 2.5~K, respectively). In the normal, ferromagnetic state (TSC<T<TCurieT_{{\rm SC}} < T < T_{{\rm Curie}}), the magnetization curve exhibits a hysteresis loop similar to that of a regular itinerant ferromagnet. Upon lowering the temperature below TSCT_{{\rm SC}}, the spontaneous magnetization is unchanged, but the hysteresis is markedly enhanced. Even deeply inside the superconducting state, ferromagnetism is not completely shielded, and there is no Meissner region, a magnetic field region of H<Hc1H < H_{\rm c1} (a lower critical field). From these results, we suggest that UCoGe is the first material in which ferromagnetism robustly survives in the superconducting state and a spontaneous vortex state without the Meissner state is realized.Comment: 5 pages, 4 figures, to be published in J. Phys. Soc. Jp
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