3,670 research outputs found
Ultrafast photoinduced enhancement of nonlinear optical response in 15-atom gold clusters on indium tin oxide conducting film
We show that the third order optical nonlinearity of 15-atom gold clusters is
significantly enhanced when in contact with indium tin oxide (ITO) conducting
film. Open and close aperture z-scan experiments together with non-degenerate
pump-probe differential transmission experiments were done using 80 fs laser
pulses centered at 395 nm and 790 nm on gold clusters encased inside
cyclodextrin cavities. We show that two photon absorption coefficient is
enhanced by an order of magnitude as compared to that when the clusters are on
pristine glass plate. The enhancement for the nonlinear optical refraction
coefficient is ~3 times. The photo-induced excited state absorption using
pump-probe experiments at pump wavelength of 395 nm and probe at 790 nm also
show an enhancement by an order of magnitude. These results attributed to the
excited state energy transfer in the coupled gold cluster-ITO system are
different from the enhancement seen so far in charge donor-acceptor complexes
and nanoparticle-conjugate polymer composites.Comment: To appear in Optics Express (2013);
http://dx.doi.org/10.1364/OE.21.00848
Femtosecond Photoexcited Carrier Dynamics in Reduced Graphene Oxide Suspensions and Films
We report ultrafast response of femtosecond photoexcited carriers in single
layer reduced graphene oxide flakes suspended in water as well as few layer
thick film deposited on indium tin oxide coated glass plate using pump-probe
differential transmission spectroscopy at 790 nm. The carrier relaxation
dynamics has three components: ~200 fs, 1 to 2 ps, and ~25 ps, all of them
independent of pump fluence. It is seen that the second component (1 to 2 ps)
assigned to the lifetime of hot optical phonons is larger for graphene in
suspensions whereas other two time constants are the same for both the
suspension and the film. The value of third order nonlinear susceptibility
estimated from the pump-probe experiments is compared with that obtained from
the open aperture Z-scan results for the suspension.Comment: 4 pages, 4 figures, to appear in International Journal of Nanoscience
(IJN), 201
Jordan-Schwinger realizations of three-dimensional polynomial algebras
A three-dimensional polynomial algebra of order is defined by the
commutation relations ,
where is an -th order polynomial in
with the coefficients being constants or central elements of the algebra.
It is shown that two given mutually commuting polynomial algebras of orders
and can be combined to give two distinct -th order polynomial
algebras. This procedure follows from a generalization of the well known
Jordan-Schwinger method of construction of and algebras from
two mutually commuting boson algebras.Comment: 10 pages, LaTeX2
Acoustic and optical phonon dynamics from femtosecond time-resolved optical spectroscopy of superconducting iron pnictide Ca(Fe_0.944Co_0.056)_2As_2
We report temperature evolution of coherently excited acoustic and optical
phonon dynamics in superconducting iron pnictide single crystal
Ca(Fe_0.944Co_0.056)_2As_2 across the spin density wave transition at T_SDW ~
85 K and superconducting transition at T_SC ~20 K. Strain pulse propagation
model applied to the generation of the acoustic phonons yields the temperature
dependence of the optical constants, and longitudinal and transverse sound
velocities in the temperature range of 3.1 K to 300 K. The frequency and
dephasing times of the phonons show anomalous temperature dependence below T_SC
indicating a coupling of these low energy excitations with the Cooper-pair
quasiparticles. A maximum in the amplitude of the acoustic modes at T ~ 170 is
seen, attributed to spin fluctuations and strong spin-lattice coupling before
T_SDW.Comment: 6 pages, 4 figures (revised manuscript
Ultrafast quasiparticle dynamics in superconducting iron pnictide CaFe1.89Co0.11As2
Nonequilibrium quasiparticle relaxation dynamics is reported in
superconducting CaFe1.89Co0.11As2 single crystal using femtosecond
time-resolved pump-probe spectroscopy. The carrier dynamics reflects a
three-channel decay of laser deposited energy with characteristic time scales
varying from few hundreds of femtoseconds to order of few nanoseconds where the
amplitudes and time-constants of the individual electronic relaxation
components show significant changes in the vicinity of the spin density wave
(T_SDW ~ 85 K) and superconducting (T_SC ~ 20 K) phase transition temperatures.
The quasiparticles dynamics in the superconducting state reveals a charge gap
with reduced gap value of 2_0/k_BT_SC ~ 1.8. We have determined the
electron-phonon coupling constant \lemda to be ~ 0.14 from the temperature
dependent relaxation time in the normal state, a value close to those reported
for other types of pnictides. From the peculiar temperature-dependence of the
carrier dynamics in the intermediate temperature region between the
superconducting and spin density wave phase transitions, we infer a temperature
scale where the charge gap associated with the spin ordered phase is maximum
and closes on either side while approaching the two phase transition
temperatures.Comment: 6 pages, 4 figures (revised manuscript);
http://dx.doi.org/10.1016/j.ssc.2013.02.00
Sponge Biodiversity in Kerala and its Biotechnological Potentials
Animals which exist today may be classified under two categories; I) Protozoa or s ingle celled animals
2) Metazoa or multicellular animals. Metazoam in tum, may be divided into two groups: a) Diploblastic,
with two germ layers (ectoderm and endoderm) and b) Triploblastic, with three germ layers (eetoderm,
mesoderm and endoderm). I n sponges thcre are no layers as seen in diploblastic or triobl.astic or triploblastic
groups, but the 'layers', in sponges, are made of loosely arranged cells which can even change their
location at will
Pathological manifestations of sponge infestation in Perna indica Kuriakose & Nair 1976
Pathological manifestations of bioeroding sponges on the brown mussel, Perna indica were studied.
The major manifestation was blister formation (46.3%). Nacre erosis was observed in 7.6% of the total
infested population. Bifacial porosis was noted in 19.1% of infested shells; discolouration of shell was
observed in 19.8 % and melanosis in 13.1 % of the infested population
Large-amplitude chirped coherent phonons in tellurium mediated by ultrafast photoexcited carrier diffusion
We report femtosecond time-resolved reflectivity measurements of coherent
phonons in tellurium performed over a wide range of temperatures (3K to 296K)
and pump laser intensities. A totally symmetric A coherent phonon at 3.6
THz responsible for the oscillations in the reflectivity data is observed to be
strongly positively chirped (i.e, phonon time period decreases at longer
pump-probe delay times) with increasing photoexcited carrier density, more so
at lower temperatures. We show for the first time that the temperature
dependence of the coherent phonon frequency is anomalous (i.e, increasing with
increasing temperature) at high photoexcited carrier density due to
electron-phonon interaction. At the highest photoexcited carrier density of
1.4 10cm and the sample temperature of 3K, the
lattice displacement of the coherent phonon mode is estimated to be as high as
0.24 \AA. Numerical simulations based on coupled effects of optical
absorption and carrier diffusion reveal that the diffusion of carriers
dominates the non-oscillatory electronic part of the time-resolved
reflectivity. Finally, using the pump-probe experiments at low carrier density
of 6 10 cm, we separate the phonon anharmonicity to
obtain the electron-phonon coupling contribution to the phonon frequency and
linewidth.Comment: 22 pages, 6 figures, submitted to PR
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