Systematic study of the influence of coherent phonon wave packets on the lasing properties of a quantum dot ensemble

Kohärente Phononen können die Licht-Materie-Wechselwirkung in Halbleiter Nanostrukturen stark ändern. Bei einem Ensemble von Quantenpunkten (QP) als aktivem Lasermedium sind Phononen im Stande, die Laserintensität deutlich zu verstärken oder abzuschwächen. Die Physik des gekoppelten Phonon-Exziton-Licht-Systems wird von verschiedenen Mechanismen dominiert, die im Experiment nicht eindeutig unterschieden werden können, da die komplizierte Probenstruktur zu einem komplexen Verspannungspuls führt, der auf das QP-Ensemble trifft. Hier zeigen wir durch eine umfassende theoretische Studie, wie die Laseremission durch Phononpulse verschiedener Form und QP-Ensembles verschiedener spektraler Verteilung beeinflusst wird. Dies erlaubt einen Einblick in die grundlegenden Wechselspiele des gekoppelten Gesamtsystems. Dadurch können wir zwischen zwei Mechanismen unterschieden: der adiabatischen Verschiebung des Ensembles und dem Schüttel-Effekt. Dies ebnet den Weg zu einer gezielten Kontrolle der Laser Emission durch kohärente Phononen.Coherent phonons can greatly vary light–matter interaction in semiconductor nanostructures placed inside an optical resonator on a picosecond time scale. For an ensemble of quantum dots (QDs) as active laser medium, phonons are able to induce a large enhancement or attenuation of the emission intensity, as has been recently demonstrated. The physics of this coupled phonon–exciton–light system consists of various effects, which in the experiment typically cannot be clearly separated, in particular, due to the complicated sample structure a rather complex strain pulse impinges on the QD ensemble. Here we present a comprehensive theoretical study how the laser emission is affected by phonon pulses of various shapes as well as by ensembles with different spectral distributions of the QDs. This gives insight into the fundamental interaction dynamics of the coupled phonon–exciton–light system, while it allows us to clearly discriminate between two prominent effects: the adiabatic shifting of the ensemble and the shaking effect. This paves the way to a tailored laser emission controlled by phonons.</p

Distinctive characteristics of carrier-phonon interactions in optically driven semiconductor quantum dots

We review distinct features arising from the unique nature of the carrier-phonon coupling in self-assembled semiconductor quantum dots. Because of the discrete electronic energy structure, the pure dephasing coupling usually dominates the phonon effects, of which two properties are of key importance: The resonant nature of the dot-phonon coupling, i.e. its non-monotonic behavior as a function of energy, and the fact that it is of super-Ohmic type. Phonons do not only act destructively in quantum dots by introducing dephasing, they also offer new opportunities, e.g. in state preparation protocols. Apart from being an interesting model systems for studying fundamental physical aspects, quantum dot and quantum dot-microcavity systems are a hotspot for many innovative applications. We discuss recent developments related to the decisive impact of phonons on key figures of merit of photonic devices like single or entangled photon sources under aspects like indistinguishability, purity and brightness. All in all it follows that understanding and controlling the carrier-phonon interaction in semiconductor quantum dots is vital for their usage in quantum information technology

Influence of local fields on the dynamics of four-wave mixing signals from 2D semiconductor systems

In recent years the physics of two-dimensional semiconductors was revived by the discovery of the class of transition metal dichalcogenides. In these systems excitons dominate the optical response in the visible range and open many perspectives for nonlinear spectroscopy. To describe the coherence and polarization dynamics of excitons after ultrafast excitation in these systems, we employ the Bloch equation model of a two-level system extended by a local field describing the exciton–exciton interaction. We calculate four-wave mixing (FWM) signals and analyze the dependence of the temporal and spectral signals as a function of the delay between the exciting pulses. Exact analytical results obtained for the case of ultrafast (δ-shaped) pulses are compared to numerical solutions obtained for finite pulse durations. If two pulses are used to generate the nonlinear signal, characteristic spectral line splittings are restricted to short delays. When considering a three-pulse excitation the line splittings, induced by the local field effect, persist for long delays. All of the found features are instructively explained within the Bloch vector picture and we show how the exciton occupation dynamics govern the different FWM signals