268 research outputs found
Coupling to a phononic mode in : Angle-resolved photoemission
The kink in the dispersion and the drop in the width observed by
angle-resolved photoemission in the nodal direction of the Brillouin zone of
(abbreviated as (Pb)Bi2212) has
attracted broad interest [1-3]. Surprisingly optimally lead-doped (Pb)Bi2212
with as well as the shadow band were not investigated so
far, although the origin of the kink and the drop is still under strong debate.
In this context a resonant magnetic-mode scenario and an electron-phonon
coupling scenario are discussed controversially. Here we analyze the relevant
differences between both scenarios and conclude that the kink and the drop are
caused by a coupling of the electronic system to a phononic mode at least in
the nodal direction. It is found that besides the dispersion and the drop in
the width also the peak height as a new criterion can be used to define the
energy scale of the interaction, giving a new means for a precise and
consistent determination of the kink energy
The Non-Trapping Degree of Scattering
We consider classical potential scattering. If no orbit is trapped at energy
E, the Hamiltonian dynamics defines an integer-valued topological degree. This
can be calculated explicitly and be used for symbolic dynamics of
multi-obstacle scattering.
If the potential is bounded, then in the non-trapping case the boundary of
Hill's Region is empty or homeomorphic to a sphere.
We consider classical potential scattering. If at energy E no orbit is
trapped, the Hamiltonian dynamics defines an integer-valued topological degree
deg(E) < 2. This is calculated explicitly for all potentials, and exactly the
integers < 2 are shown to occur for suitable potentials.
The non-trapping condition is restrictive in the sense that for a bounded
potential it is shown to imply that the boundary of Hill's Region in
configuration space is either empty or homeomorphic to a sphere.
However, in many situations one can decompose a potential into a sum of
non-trapping potentials with non-trivial degree and embed symbolic dynamics of
multi-obstacle scattering. This comprises a large number of earlier results,
obtained by different authors on multi-obstacle scattering.Comment: 25 pages, 1 figure Revised and enlarged version, containing more
detailed proofs and remark
Family health climate scale (FHC-scale): Development and validation
Background:
The family environment is important for explaining individual health behaviour. While previous research mostly focused on influences among family members and dyadic interactions (parent-child), the purpose of this study was to develop a new measure, the Family Health Climate Scale (FHC-Scale), using a family-based approach. The FHC is an attribute of the whole family and describes an aspect of the family environment that is related to health and health behaviour. Specifically, a questionnaire measuring the FHC (a) for nutrition (FHC-NU) and (b) for activity behaviour (FHC-PA) was developed and validated.
Methods:
In Study 1 (N = 787) the FHC scales were refined and validated. The sample was randomly divided into two subsamples. With random sample I exploratory factor analyses were conducted and items were selected according to their psychometric quality. In a second step, confirmatory factor analyses were conducted using the random sample II. In Study 2 (N = 210 parental couples) the construct validity was tested by correlating the FHC to self-determined motivation of healthy eating and physical activity as well as the familiesâ food environment and joint physical activities.
Results:
Exploratory factor analyses with random sample I (Study 1) revealed a four (FHC-NU) and a three (FHC-PA) factor model. These models were cross-validated with random sample II and demonstrated an acceptable fit [FHC-PA: Ď2 = 222.69, df = 74, p < .01; Ď2/df = 3.01; CFI = .96; SRMR = .04; RMSEA = .07, CI .06/.08; FHC-NU: Ď2 = 278.30, df = 113, p < .01, Ď2/df = 2.46, CFI = .96; SRMR = .04; RMSEA = .06, CI .05/.07]. The perception of FHC correlated (p < .01) with the intrinsic motivation of healthy eating (r = .42) and physical activity (r = .56). Moreover, parental perceptions of FHC-NU correlated with household soft drink availability (r = â.31) and perceptions of FHC-PA with the frequency of joint physical activities with the child (r = .51). These patterns were found on the intraindividual and interindividual level.
Conclusions:
Two valid instruments measuring the FHC within families were developed. The use of different informantsâ ratings demonstrated that the FHC is a family level variable. The results confirm the high relevance of the FHC for individualsâ health behaviour. The FHC and the measurement instruments are useful for examining health-related aspects of the family environment
Dynamic nuclear polarization at the edge of a two-dimensional electron gas
We have used gated GaAs/AlGaAs heterostructures to explore nonlinear
transport between spin-resolved Landau level (LL) edge states over a submicron
region of two-dimensional electron gas (2DEG). The current I flowing from one
edge state to the other as a function of the voltage V between them shows
diode-like behavior---a rapid increase in I above a well-defined threshold V_t
under forward bias, and a slower increase in I under reverse bias. In these
measurements, a pronounced influence of a current-induced nuclear spin
polarization on the spin splitting is observed, and supported by a series of
NMR experiments. We conclude that the hyperfine interaction plays an important
role in determining the electronic properties at the edge of a 2DEG.Comment: 8 pages RevTeX, 7 figures (GIF); submitted to Phys. Rev.
Electrochemistry at nanoscale electrodes : individual single-walled carbon nanotubes (SWNTs) and SWNT-templated metal nanowires
Individual nanowires (NWs) and native single-walled carbon nanotubes (SWNTs) can be readily used as well-defined nanoscale electrodes (NSEs) for voltammetric analysis. Here, the simple photolithography-free fabrication of submillimeter long Au, Pt, and Pd NWs, with sub-100 nm heights, by templated electrodeposition onto ultralong flow-aligned SWNTs is demonstrated. Both individual Au NWs and SWNTs are employed as NSEs for electron-transfer (ET) kinetic quantification, using cyclic voltammetry (CV), in conjunction with a microcapillary-based electrochemical method. A small capillary with internal diameter in the range 30â70 Îźm, filled with solution containing a redox-active mediator (FcTMA+ ((trimethylammonium)methylferrocene), Fe(CN)64â, or hydrazine) is positioned above the NSE, so that the solution meniscus completes an electrochemical cell. A 3D finite-element model, faithfully reproducing the experimental geometry, is used to both analyze the experimental CVs and derive the rate of heterogeneous ET, using ButlerâVolmer kinetics. For a 70 nm height Au NW, intrinsic rate constants, k0, up to ca. 1 cm sâ1 can be resolved. Using the same experimental configuration the electrochemistry of individual SWNTs can also be accessed. For FcTMA+/2+ electrolysis the simulated ET kinetic parameters yield very fast ET kinetics (k0 > 2 Âą 1 cm sâ1). Some deviation between the experimental voltammetry and the idealized model is noted, suggesting that double-layer effects may influence ET at the nanoscale
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