6,224 research outputs found
The structural distortion in antiferromagnetic LaFeAsO investigated by a group-theoretical approach
As experimentally well established, undoped LaFeAsO is antiferromagnetic
below 137K with the magnetic moments lying on the Fe sites. We determine the
orthorhombic body-centered group Imma (74) as the space group of the
experimentally observed magnetic structure in the undistorted lattice, i.e., in
a lattice possessing no structural distortions in addition to the
magnetostriction. We show that LaFeAsO possesses a partly filled "magnetic
band" with Bloch functions that can be unitarily transformed into optimally
localized Wannier functions adapted to the space group Imma. This finding is
interpreted in the framework of a nonadiabatic extension of the Heisenberg
model of magnetism, the nonadiabatic Heisenberg model. Within this model,
however, the magnetic structure with the space group Imma is not stable but can
be stabilized by a (slight) distortion of the crystal turning the space group
Imma into the space group Pnn2 (34). This group-theoretical result is in
accordance with the experimentally observed displacements of the Fe and O atoms
in LaFeAsO as reported by Clarina de la Cruz et al. [nature 453, 899 (2008)]
Recombination dynamics in bacterial photosynthetic reaction centers
The time dependence of magnetic field effects on light absorption by triplet-state and radical ions in quinone-depleted reaction centers of Rhodopseudomonas sphaeroides strain R-26 has been investigated. Measurements on the time scale of the hyperfine interaction in the radical pair [(BChl)2+. ...BPh-.)] provided kinetic data characterizing the recombination process. The results have been interpreted in terms of a recently proposed model that assumes an intermediate electron acceptor (close site) between the bacteriochlorophyll "special pair" (BChl)2 and the bacteriopheophytin BPh (distant site). Recombination is assumed to proceed through this intermediate acceptor. The experiments led to effective recombination rates for the singlet and triplet channel: k(Seff) = 3.9 . 107 s-1 and k(Teff) = 7.4 . 10(8) s-1. These correspond to recombination rates ks = 1 . 10(1) s-1 and kT = 7.1 . 10(11) s-1 in the close configuration. The upper bound of the effective spin dephasing rate k2eff approximately equal to 1 . 10(9) s-1 is identical with the rate of the electron hopping between the distant site of zero spin exchange interaction and the close site of large interaction. Interpretation of data for the case of direct recombination yields the recombination rates, spin dephasing rate, and exchange interaction in a straightforward way
Compressive strength and elastic modulus of Comet 67P interpreted from a material science point of view
The analysis of Cometary Acoustic Surface Sounding
Experiment (CASSE) data yielded values of surface
compression strength and elastic modulus at the
landing site Agilkia. These data are interpreted with
fracture mechanical concepts from material science
taking into account the high porosity of Comet 67P
Aspects of the Mass Distribution of Interstellar Dust Grains in the Solar System from In-Situ Measurements
The in-situ detection of interstellar dust grains in the Solar System by the
dust instruments on-board the Ulysses and Galileo spacecraft as well as the
recent measurements of hyperbolic radar meteors give information on the
properties of the interstellar solid particle population in the solar vicinity.
Especially the distribution of grain masses is indicative of growth and
destruction mechanisms that govern the grain evolution in the interstellar
medium. The mass of an impacting dust grain is derived from its impact velocity
and the amount of plasma generated by the impact. Because the initial velocity
and the dynamics of interstellar particles in the Solar System are well known,
we use an approximated theoretical instead of the measured impact velocity to
derive the mass of interstellar grains from the Ulysses and Galileo in-situ
data. The revised mass distributions are steeper and thus contain less large
grains than the ones that use measured impact velocities, but large grains
still contribute significantly to the overall mass of the detected grains. The
flux of interstellar grains with masses is determined to
be . The comparison of radar data
with the extrapolation of the Ulysses and Galileo mass distribution indicates
that the very large () hyperbolic meteoroids detected by
the radar are not kinematically related to the interstellar dust population
detected by the spacecraft.Comment: 14 pages, 11 figures, to appear in JG
From Equilibrium to Steady-State Dynamics after Switch-On of Shear
A relation between equilibrium, steady-state, and waiting-time dependent
dynamical two-time correlation functions in dense glass-forming liquids subject
to homogeneous steady shear flow is discussed. The systems under study show
pronounced shear thinning, i.e., a significant speedup in their steady-state
slow relaxation as compared to equilibrium. An approximate relation that
recovers the exact limit for small waiting times is derived following the
integration through transients (ITT) approach for the nonequilibrium
Smoluchowski dynamics, and is exemplified within a schematic model in the
framework of the mode-coupling theory of the glass transition (MCT). Computer
simulation results for the tagged-particle density correlation functions
corresponding to wave vectors in the shear-gradient directions from both
event-driven stochastic dynamics of a two-dimensional hard-disk system and from
previously published Newtonian-dynamics simulations of a three-dimensional
soft-sphere mixture are analyzed and compared with the predictions of the
ITT-based approximation. Good qualitative and semi-quantitative agreement is
found. Furthermore, for short waiting times, the theoretical description of the
waiting time dependence shows excellent quantitative agreement to the
simulations. This confirms the accuracy of the central approximation used
earlier to derive fluctuation dissipation ratios (Phys. Rev. Lett. 102,
135701). For intermediate waiting times, the correlation functions decay faster
at long times than the stationary ones. This behavior is predicted by our
theory and observed in simulations.Comment: 16 pages, 12 figures, submitted to Phys Rev
A dynamic density functional theory for particles in a flowing solvent
We present a dynamic density functional theory (dDFT) which takes into accou
nt the advection of the particles by a flowing solvent. For potential flows we
can use the same closure as in the absence of solvent flow. The structure of
the resulting advected dDFT suggests that it could be used for non-potential
flows as well. We apply this dDFT to Brownian particles (e.g., polymer coils)
in a solvent flowing around a spherical obstacle (e.g., a colloid) and compare
the results with direct simulations of the underlying Brownian dynamics.
Although numerical limitations do not allow for an accurate quantitative
check of the advected dDFT both show the same qualitative features. In contrast
to previous works which neglected the deformation of the flow by the obstacle,
we find that the bow-wave in the density distribution of particles in front of
the obstacle as well as the wake behind it are reduced dramatically. As a
consequence the friction force exerted by the (polymer) particles on the
colloid can be reduced drastically.Comment: 7 pages, 5 figures, 2 tables, submitte
An atom fiber for guiding cold neutral atoms
We present an omnidirectional matter wave guide on an atom chip. The
rotational symmetry of the guide is maintained by a combination of two current
carrying wires and a bias field pointing perpendicular to the chip surface. We
demonstrate guiding of thermal atoms around more than two complete turns along
a spiral shaped 25mm long curved path (curve radii down to 200m) at
various atom--surface distances (35-450m). An extension of the scheme for
the guiding of Bose-Einstein condensates is outlined
Gaussian Entanglement of Formation
We introduce a Gaussian version of the entanglement of formation adapted to
bipartite Gaussian states by considering decompositions into pure Gaussian
states only. We show that this quantity is an entanglement monotone under
Gaussian operations and provide a simplified computation for states of
arbitrary many modes. For the case of one mode per site the remaining
variational problem can be solved analytically. If the considered state is in
addition symmetric with respect to interchanging the two modes, we prove
additivity of the considered entanglement measure. Moreover, in this case and
considering only a single copy, our entanglement measure coincides with the
true entanglement of formation.Comment: 8 pages (references updated, typos corrected
Non-equilibrium Casimir forces: Spheres and sphere-plate
We discuss non-equilibrium extensions of the Casimir force (due to
electromagnetic fluctuations), where the objects as well as the environment are
held at different temperatures. While the formalism we develop is quite
general, we focus on a sphere in front of a plate, as well as two spheres, when
the radius is small compared to separation and thermal wavelengths. In this
limit the forces can be expressed analytically in terms of the lowest order
multipoles, and corroborated with results obtained by diluting parallel plates
of vanishing thickness. Non-equilibrium forces are generally stronger than
their equilibrium counterpart, and may oscillate with separation (at a scale
set by material resonances). For both geometries we obtain stable points of
zero net force, while two spheres may have equal forces in magnitude and
direction resulting in a self-propelling state.Comment: 6 pages, 6 figure
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