Enhancement of the electric dipole moment of the electron in the YbF molecule

We calculate an effective electric field on the unpaired electron in the YbF molecule. This field determines sensitivity of the molecular experiment to the electric dipole moment of the electron. We use experimental value of the spin-doubling constant to estimate the admixture of the configuration with the hole in the 4f-shell of Ytterbium to the ground state of the molecule. This admixture reduces the field by 7%. Our value for the effictive field is 5.1 a.u. = 2.5 10^{10} V/cm.Comment: 5 pages, LATEX, uses revtex.st

Microspectroscopy and Imaging in the THz Range Using Coherent CW Radiation

A novel THz near-field spectrometer is presented which allows to perform biological and medical studies with high spectral resolution combined with a spatial resolution down to l/100. In the setup an aperture much smaller than the used wavelength is placed in the beam very close to the sample. The sample is probed by the evanescent wave behind the aperture. The distance is measured extremely accurate by a confocal microscope. We use monochromatic sources which provide powerful coherent cw radiation tuneable from 50 GHz up to 1.5 THz. Transmission and reflection experiments can be performed which enable us to study solids and molecules in aqueous solution. Examples for spectroscopic investigations on biological tissues are presented.Comment: 4 pages, 5 figures, email: [email protected]

Electric dipole moment of the electron in YbF molecule

Ab initio calculation of the hyperfine, P-odd, and P,T-odd constants for the YbF molecule was performed with the help of the recently developed technique, which allows to take into account correlations and polarization in the outercore region. The ground state electronic wave function of the YbF molecule is found with the help of the Relativistic Effective Core Potential method followed by the restoration of molecular four-component spinors in the core region of ytterbium in the framework of a non-variational procedure. Core polarization effects are included with the help of the atomic Many Body Perturbation Theory for Yb atom. For the isotropic hyperfine constant A, accuracy of our calculation is about 3% as compared to the experimental datum. The dipole constant Ad (which is much smaller in magnitude), though better than in all previous calculations, is still underestimated by almost 23%. Being corrected within a semiempirical approach for a perturbation of 4f-shell in the core of Yb due to the bond making, this error is reduced to 8%. Our value for the effective electric field on the unpaired electron is 4.9 a.u.=2.5E+10 V/cm.Comment: 7 pages, REVTE

Enhancement of the electric dipole moment of the electron in PbO

The a(1) state of PbO can be used to measure the electric dipole moment of the electron d_e. We discuss a semiempirical model for this state, which yields an estimate of the effective electric field on the valence electrons in PbO. Our final result is an upper limit on the measurable energy shift, which is significantly larger than was anticipated earlier: $2|W_d|d_e \ge 2.4\times 10^{25} \textrm{Hz} [ \frac{d_e}{e \textrm{cm}} ]$.Comment: 4 pages, revtex4, no figures, submitted to PR

Electric dipole moment enhancement factor of thallium

The goal of this work is to resolve the present controversy in the value of the EDM enhancement factor of Tl. We have carried out several calculations by different high-precision methods, studied previously omitted corrections, as well as tested our methodology on other parity conserving quantities. We find the EDM enhancement factor of Tl to be equal to -573(20). This value is 20% larger than the recently published result of Nataraj et al. [Phys. Rev. Lett. 106, 200403 (2011)], but agrees very well with several earlier results.Comment: 5 pages; v2: link to supplemental material adde

Macroscopic amplification of electroweak effects in molecular Bose-Einstein condensates

We investigate the possible use of Bose-Einstein condensates of diatomic molecules to measure nuclear spin-dependent parity violation effects, outlining a detection method based on the internal Josephson effect between molecular states of opposite parity. When applied to molecular condensates, the fine experimental control achieved in atomic bosonic Josephson junctions could provide data on anapole moments and neutral weak couplings.Comment: 5 pages. To be published Phys. Rev. A (Rapid Communication) (2012

Using Molecules to Measure Nuclear Spin-Dependent Parity Violation

Nuclear spin-dependent parity violation arises from weak interactions between electrons and nucleons, and from nuclear anapole moments. We outline a method to measure such effects, using a Stark-interference technique to determine the mixing between opposite-parity rotational/hyperfine levels of ground-state molecules. The technique is applicable to nuclei over a wide range of atomic number, in diatomic species that are theoretically tractable for interpretation. This should provide data on anapole moments of many nuclei, and on previously unmeasured neutral weak couplings

Trapping polarization of light in nonlinear optical fibers: An ideal Raman polarizer

The main subject of this contribution is the all-optical control over the state of polarization (SOP) of light, understood as the control over the SOP of a signal beam by the SOP of a pump beam. We will show how the possibility of such control arises naturally from a vectorial study of pump-probe Raman interactions in optical fibers. Most studies on the Raman effect in optical fibers assume a scalar model, which is only valid for high-PMD fibers (here, PMD stands for the polarization-mode dispersion). Modern technology enables manufacturing of low-PMD fibers, the description of which requires a full vectorial model. Within this model we gain full control over the SOP of the signal beam. In particular we show how the signal SOP is pulled towards and trapped by the pump SOP. The isotropic symmetry of the fiber is broken by the presence of the polarized pump. This trapping effect is used in experiments for the design of new nonlinear optical devices named Raman polarizers. Along with the property of improved signal amplification, these devices transform an arbitrary input SOP of the signal beam into one and the same SOP towards the output end. This output SOP is fully controlled by the SOP of the pump beam. We overview the sate-of-the-art of the subject and introduce the notion of an "ideal Raman polarizer"

Enhancement of the electric dipole moment of the electron in BaF molecule

We report results of ab initio calculation of the spin-rotational Hamiltonian parameters including P- and P,T-odd terms for the BaF molecule. The ground state wave function of BaF molecule is found with the help of the Relativistic Effective Core Potential method followed by the restoration of molecular four-component spinors in the core region of barium in the framework of a non-variational procedure. Core polarization effects are included with the help of the atomic Many Body Perturbation Theory for Barium atom. For the hyperfine constants the accuracy of this method is about 5-10%.Comment: 8 pages, REVTEX, report at II International Symposium on Symmetries in Subatomic Physics, Seattle 199