319 research outputs found
Resonant enhancement of the zero-phonon emission from a color center in a diamond cavity
We demonstrate coupling of the zero-phonon line of individual
nitrogen-vacancy centers and the modes of microring resonators fabricated in
single-crystal diamond. A zero-phonon line enhancement exceeding ten-fold is
estimated from lifetime measurements at cryogenic temperatures. The devices are
fabricated using standard semiconductor techniques and off-the-shelf materials,
thus enabling integrated diamond photonics.Comment: 5 pages, 4 figure
Geometry-controlled kinetics
It has long been appreciated that transport properties can control reaction
kinetics. This effect can be characterized by the time it takes a diffusing
molecule to reach a target -- the first-passage time (FPT). Although essential
to quantify the kinetics of reactions on all time scales, determining the FPT
distribution was deemed so far intractable. Here, we calculate analytically
this FPT distribution and show that transport processes as various as regular
diffusion, anomalous diffusion, diffusion in disordered media and in fractals
fall into the same universality classes. Beyond this theoretical aspect, this
result changes the views on standard reaction kinetics. More precisely, we
argue that geometry can become a key parameter so far ignored in this context,
and introduce the concept of "geometry-controlled kinetics". These findings
could help understand the crucial role of spatial organization of genes in
transcription kinetics, and more generally the impact of geometry on
diffusion-limited reactions.Comment: Submitted versio
Enhanced reaction kinetics in biological cells
The cell cytoskeleton is a striking example of "active" medium driven
out-of-equilibrium by ATP hydrolysis. Such activity has been shown recently to
have a spectacular impact on the mechanical and rheological properties of the
cellular medium, as well as on its transport properties : a generic tracer
particle freely diffuses as in a standard equilibrium medium, but also
intermittently binds with random interaction times to motor proteins, which
perform active ballistic excursions along cytoskeletal filaments. Here, we
propose for the first time an analytical model of transport limited reactions
in active media, and show quantitatively how active transport can enhance
reactivity for large enough tracers like vesicles. We derive analytically the
average interaction time with motor proteins which optimizes the reaction rate,
and reveal remarkable universal features of the optimal configuration. We
discuss why active transport may be beneficial in various biological examples:
cell cytoskeleton, membranes and lamellipodia, and tubular structures like
axons.Comment: 10 pages, 2 figure
Quantum Statistics of Surface Plasmon Polaritons in Metallic Stripe Waveguides
Single surface plasmon polaritons are excited using photons generated via
spontaneous parametric down-conversion. The mean excitation rates, intensity
correlations and Fock state populations are studied. The observed dependence of
the second order coherence in our experiment is consistent with a linear
uncorrelated Markovian environment in the quantum regime. Our results provide
important information about the effect of loss for assessing the potential of
plasmonic waveguides for future nanophotonic circuitry in the quantum regime.Comment: 21 pages, 6 figures, published in Nano Letters, publication date
(web): March 27 (2012
Room temperature plasmon laser by total internal reflection
Plasmon lasers create and sustain intense and coherent optical fields below
light's diffraction limit with the unique ability to drastically enhance
light-matter interactions bringing fundamentally new capabilities to
bio-sensing, data storage, photolithography and optical communications.
However, these important applications require room temperature operation, which
remains a major hurdle. Here, we report a room temperature semiconductor
plasmon laser with both strong cavity feedback and optical confinement to
1/20th of the wavelength. The strong feedback arises from total internal
reflection of surface plasmons, while the confinement enhances the spontaneous
emission rate by up to 20 times.Comment: 8 Page, 2 Figure
Radiation hydrodynamics of SN 1987A: I. Global analysis of the light curve for the first 4 months
The optical/UV light curves of SN 1987A are analyzed with the multi-energy
group radiation hydrodynamics code STELLA. The calculated monochromatic and
bolometric light curves are compared with observations shortly after shock
breakout, during the early plateau, through the broad second maximum, and
during the earliest phase of the radioactive tail. We have concentrated on a
progenitor model calculated by Nomoto & Hashimoto and Saio, Nomoto, & Kato,
which assumes that 14 solar masses of the stellar mass is ejected. Using this
model, we have updated constraints on the explosion energy and the extent of
mixing in the ejecta. In particular, we determine the most likely range of E/M
(explosion energy over ejecta mass) and R_0 (radius of the progenitor). In
general, our best models have energies in the range E = (1.1 +/- 0.3) x 10^{51}
ergs, and the agreement is better than in earlier, flux-limited diffusion
calculations for the same explosion energy. Our modeled B and V fluxes compare
well with observations, while the flux in U undershoots after about 10 days by
a factor of a few, presumably due to NLTE and line transfer effects. We also
compare our results with IUE observations, and a very good quantitative
agreement is found for the first days, and for one IUE band (2500-3000 A) as
long as for 3 months. We point out that the V flux estimated by McNaught &
Zoltowski should probably be revised to a lower value.Comment: 27 pages AASTeX v.4.0 + 35 postscript figures. ApJ, accepte
Multiorder coherent Raman scattering of a quantum probe field
We study the multiorder coherent Raman scattering of a quantum probe field in
a far-off-resonance medium with a prepared coherence. Under the conditions of
negligible dispersion and limited bandwidth, we derive a Bessel-function
solution for the sideband field operators. We analytically and numerically
calculate various quantum statistical characteristics of the sideband fields.
We show that the multiorder coherent Raman process can replicate the
statistical properties of a single-mode quantum probe field into a broad comb
of generated Raman sidebands. We also study the mixing and modulation of photon
statistical properties in the case of two-mode input. We show that the prepared
Raman coherence and the medium length can be used as control parameters to
switch a sideband field from one type of photon statistics to another type, or
from a non-squeezed state to a squeezed state and vice versa.Comment: 12 pages, 7 figures, to be published in Phys. Rev.
Scalable quantum register based on coupled electron spins in a room temperature solid
Realization of devices based on quantum laws might lead to building
processors that outperform their classical analogues and establishing
unconditionally secure communication protocols. Solids do usually present a
serious challenge to quantum coherence. However, owing to their spin-free
lattice and low spin orbit coupling, carbon materials and particularly diamond
are suitable for hosting robust solid state quantum registers. We show that
scalable quantum logic elements can be realized by exploring long range
magnetic dipolar coupling between individually addressable single electron
spins associated with separate color centers in diamond. Strong distance
dependence of coupling was used to characterize the separation of single qubits
98 A with unprecedented accuracy (3 A) close to a crystal lattice spacing. Our
demonstration of coherent control over both electron spins, conditional
dynamics, selective readout as well as switchable interaction, opens the way
towards a room temperature solid state scalable quantum register. Since both
electron spins are optically addressable, this solid state quantum device
operating at ambient conditions provides a degree of control that is currently
available only for atomic systems.Comment: original submitted version of the manuscrip
The Energy Landscape, Folding Pathways and the Kinetics of a Knotted Protein
The folding pathway and rate coefficients of the folding of a knotted protein
are calculated for a potential energy function with minimal energetic
frustration. A kinetic transition network is constructed using the discrete
path sampling approach, and the resulting potential energy surface is
visualized by constructing disconnectivity graphs. Owing to topological
constraints, the low-lying portion of the landscape consists of three distinct
regions, corresponding to the native knotted state and to configurations where
either the N- or C-terminus is not yet folded into the knot. The fastest
folding pathways from denatured states exhibit early formation of the
N-terminus portion of the knot and a rate-determining step where the C-terminus
is incorporated. The low-lying minima with the N-terminus knotted and the
C-terminus free therefore constitute an off-pathway intermediate for this
model. The insertion of both the N- and C-termini into the knot occur late in
the folding process, creating large energy barriers that are the rate limiting
steps in the folding process. When compared to other protein folding proteins
of a similar length, this system folds over six orders of magnitude more
slowly.Comment: 19 page
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