2 research outputs found
Electronic properties of LaOFFeAs in the normal state probed by NMR/NQR
We report 139La, 57Fe and 75As nuclear magnetic resonance (NMR) and nuclear
quadrupole resonance (NQR) measurements on powders of the new LaO1-xFxFeAs
superconductor for x = 0 and x = 0.1 at temperatures up to 480 K, and compare
our measured NQR spectra with local density approximation (LDA) calculations.
For all three nuclei in the x = 0.1 material, it is found that the local Knight
shift increases monotonically with an increase in temperature, and scales with
the macroscopic susceptibility, suggesting a single magnetic degree of freedom.
Surprisingly, the spin lattice relaxation rates for all nuclei also scale with
one another, despite the fact that the form factors for each site sample
different regions of q-space. This result suggests a lack of any q-space
structure in the dynamical spin susceptibility that might be expected in the
presence of antiferromagnetic correlations. Rather, our results are more
compatible with simple quasi-particle scattering. Furthermore, we find that the
increase in the electric field gradient at the As cannot be accounted for by
LDA calculations, suggesting that structural changes, in particular the
position of the As in the unit cell, dominate the NQR response.Comment: 17 pages, 6 figure
Pressure-induced magnetic transition and volume collapse in FeAs superconductors: An orbital-selective Mott scenario
Motivated by pressure experiments on FeAs-122 superconductors, we propose a
scenario based on local-moment physics to explain the simultaneous
disappearance of magnetism, reduction of the unit cell volume, and decrease in
resistivity. In this scenario, the low-pressure magnetic phase derives from Fe
moments, which become screened in the paramagnetic high-pressure phase. The
quantum phase transition can be described as an orbital-selective Mott
transition, which is rendered first order by coupling to the lattice, in
analogy to a Kondo volume collapse. Spin-fluctuation driven superconductivity
competes with antiferromagnetism and may be stabilized at low temperatures in
the high-pressure phase. The ideas are illustrated by a suitable mean-field
analysis of an Anderson lattice model.Comment: 9 pages, 3 figs; (v2) robustness of OS Mott transition vs. fragility
of superconductivity discussed, final version to be publishe