Nutation versus angular dependent NQR spectroscopy and the impact of underdoping on charge inhomogeneities in YBa2_2Cu3_3Oy_y

We describe two different nuclear quadrupole resonance (NQR) based techniques, designed to measure the local asymmetry of the internal electric field gradient, and the tilt angle of the main NQR principal axis z from the crystallographic axis c. These techniques use the dependence of the NQR signal on the duration of the radio frequency (rf) pulse and on the direction of the rf field H1 with respect to the crystal axis. The techniques are applied to oriented powder of YBa$_{2}$Cu$$O$_{y}$ fully enriched with 63Cu. Measurements were performed at different frequencies, corresponding to different in-plane copper sites with respect to the dopant. Combining the results from both techniques, we conclude that oxygen deficiency in the chain layer lead to a rotation of the NQR main principal axis at the nearby Cu on the CuO2 planes by 20+-degrees. This occurs with no change to the asymmetry. The axis rotation associated with oxygen deficiency means that there must be electric field inhomogeneities in the CuO2 planes only in the vicinity of the missing oxygen.Comment: 9 pages, 10 figure

Ga NMR study of the local susceptibility in SrCr8Ga4O19: pseudogap and paramagnetic defects

We present the first Ga(4f) NMR study of the Cr susceptibility in the archetype of Kagome based frustrated antiferromagnets, SrCr$_{8}$Ga$_{4}$O$_{19}$. Our major finding is that the susceptibility of the frustrated lattice goes through a maximum around 50 K. Our data also supports the existence of paramagnetic ``clusters'' of spins, responsible for the Curie behavior observed in the macroscopic susceptibility at low T. These results set novel features for the constantly debated physics of geometrically frustrated magnets.Comment: 4 pages, 5 figures Submitted to Phys. Rev. Let

The Herbertsmithite Hamiltonian: μ\muSR measurements on single crystals

We present transverse field muon spin rotation/relaxation measurements on single crystals of the spin-1/2 kagome antiferromagnet Herbertsmithite. We find that the spins are more easily polarized when the field is perpendicular to the kagome plane. We demonstrate that the difference in magnetization between the different directions cannot be accounted for by Dzyaloshinksii-Moriya type interactions alone, and that anisotropic axial interaction is present.Comment: 8 pages, 3 figures, accepted to JPCM special issue on geometrically frustrated magnetis

Evolution from a nodeless gap to d(x2-y2) form in underdoped La(2-x)SrxCuO4

Using angle-resolved photoemission (ARPES), it is revealed that the low-energy electronic excitation spectra of highly underdoped superconducting and non-superconducting La(2-x)SrxCuO4 cuprates are gapped along the entire underlying Fermi surface at low temperatures. We show how the gap function evolves to a d(x2-y2) form as increasing temperature or doping, consistent with the vast majority of ARPES studies of cuprates. Our results provide essential information for uncovering the symmetry of the order parameter(s) in strongly underdoped cuprates, which is a prerequisite for understanding the pairing mechanism and how superconductivity emerges from a Mott insulator.Comment: 5 pages, 4 figure

Muon spin rotation study of the magnetic penetration depth in the intercalated graphite superconductor CaC6

We report temperature- and magnetic field-dependent bulk muon spin rotation measurements in a c-axis oriented superconductor CaC6 in the mixed state. Using both a simple second moment analysis and the more precise analytical Ginzburg-Landau model, we obtained a field independent in-plane magnetic penetration depth {\lambda}ab (0) = 72(3) nm. The temperature dependencies of the normalized muon spin relaxation rate and of the normalized superfluid density result to be identical, and both are well represented by the clean limit BCS model with 2\Delta/kB Tc = 3.6(1), suggesting that CaC6 is a fully gapped BCS superconductor in the clean limit regime.Comment: Accepted for publication in PR

Spin Echo Decay in a Stochastic Field Environment

We derive a general formalism with which it is possible to obtain the time dependence of the echo size for a spin in a stochastic field environment. Our model is based on ``strong collisions''. We examine in detail three cases where: (I) the local field is Ising-like, (II) the field distribution is continuous and has a finite second moment, and (III) the distribution is Lorentzian. The first two cases show a T2 minimum effect and are exponential in time cubed for short times. The last case can be approximated by a phenomenological stretched exponential.Comment: 11 pages + 3 postscript figure

Frustration driven lattice distortion; an NMR investigation of Y2Mo2O7

We have investigated the 89Y NMR spectrum and spin lattice relaxation, T1, in the magnetically frustrated pyrochlore Y2Mo2O7. We find that upon cooling the spectrum shifts, and broadens asymmetrically. A detailed examination of the low T spectrum reveals that it is constructed from multiple peaks, each shifted by a different amount. We argue that this spectrum is due to discrete lattice distortions, and speculate that these distortions relieve the frustration and reduce the system's energy.Comment: To be published in Phys. Rev. Let