Uncovering a pressure-tuned electronic transition in BiSrYCu2O8 using Raman scattering and x-ray diffraction

We report pressure tuned Raman and x-ray diffraction data of Bi1.98Sr2.06Y0.68Cu2O8 revealing a critical pressure at 21 GPa with anomalies in six physical quantities: electronic Raman background, electron-phonon coupling, spectral weight transfer from high to low frequency, density dependent behaviour of phonon and magnon frequencies, and a compressibility change in the c-axis. For the first time in a cuprate, mobile charge carriers, lattice, and magnetism all show anomalies at a distinct critical pressure in the same experimental setting. Furthermore, the Raman spectral changes are similar to that seen traversing the superconducting dome with doping, suggesting that the critical pressure at 21 GPa is related to the much discussed critical point at optimal doping.Comment: 5 pages, 4 figures, submitted to PR

Comment on "Superconducting gap anisotropy vs. doping level in high-T_c cuprates" by C. Kendziora et al, PRL 77, 727 (1996)

In a recent paper Kendziora et al concluded that the superconducting gap in overdoped Bi-2212 is isotropic. From data obtained from electronic Raman scattering measurements, their conclusion was based on the observation that pair breaking peaks occured at approximately the same frequency in different scattering geometries and that the normalized scattering intensity at low energies was strongly depleted. We discuss a different interpretation of the raw data and present new data which is consistent with a strongly anisotropic gap with nodes. The spectra can be successfully described by a model for Raman scattering in a d_{x^{2}-y^{2}} superconductor with spin fluctuations and impurity scattering included.Comment: 1 page revtex plus 1 postscript figur

No Far-Infrared-Spectroscopic Gap in Clean and Dirty High-TC_C Superconductors

We report far infrared transmission measurements on single crystal samples derived from Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8}$. The impurity scattering rate of the samples was varied by electron-beam irradiation, 50MeV $^{16}$O$^{+6}$ ion irradiation, heat treatment in vacuum, and Y doping. Although substantial changes in the infrared spectra were produced, in no case was a feature observed that could be associated with the superconducting energy gap. These results all but rule out ``clean limit'' explanations for the absence of the spectroscopic gap in this material, and provide evidence that the superconductivity in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8}$ is gapless.Comment: 4 pages and 3 postscript figures attached. REVTEX v3.0. Accepted for publication in Phys. Rev. Lett. IRDIRT

Predominantly Superconducting Origin of Large Energy Gaps in Underdoped Bi2Sr2CaCu2O8-d from Tunneling Spectroscopy

New tunneling data are reported in underdoped Bi2Sr2CaCu2O8-d using superconductor-insulator-superconductor break junctions. Energy gaps, Delta, of 51+2, 54+2 and 57+3 meV are observed for three crystals with Tc=77, 74, and 70 K respectively. These energy gaps are nearly three times larger than for overdoped crystals with similar Tc. Detailed examination of tunneling spectra over a wide doping range from underdoped to overdoped, including the Josephson IcRn product, indicate that these energy gaps are predominantly of superconducting origin.Comment: 10 pages, 4 figures, 1 tabl

C-axis electronic Raman scattering in Bi_2Sr_2CaCu_2O_{8+\delta}

We report a c-axis-polarized electronic Raman scattering study of Bi_2Sr_2CaCu_2O_{8+\delta} single crystals. In the normal state, a resonant electronic continuum extends to 1.5 eV and gains significant intensity as the incoming photon energy increases. In the superconducting state, a coherence 2\Delta peak appears around 50 meV, with a suppression of the scattering intensity at frequencies below the peak position. The peak energy, which is higher than that seen with in-plane polarizations, signifies distinctly different dynamics of quasiparticle excitations created with out-of-plane polarization.Comment: 12 pages, REVTEX, 3 postscript figure

Magnetoresistance of YBa2Cu3O7 in the "cold spots" model

We calculate the in-plane magnetoresistance $\Delta\rho_{xx}/\rho_{xx}$ of YBa$_2$Cu$_3$O$_7$ in a magnetic field applied perpendicular to the $CuO_2$ planes for the ``cold spots'' model. In this model, the electron relaxation time $\tau_2\propto1/T^2$ at small regions on the Fermi surface near the Brillouin zone diagonals is much longer than the relaxation time $\tau_1\propto1/T$ at the rest of the Fermi surface ($T$ is temperature). In qualitative agreement with the experiment, we find that Kohler's rule is strongly violated, but the ratio $\Delta\rho_{xx}/\rho_{xx}\tan^2\theta_H$, where $\tan\theta_H$ is the Hall angle, is approximately temperature-independent. We find the ratio is about 5.5, which is of the same order of magnitude as in the experiment.Comment: RevTeX, 4 pages, 6 figures. V.2: 2 references adde

Measuring anisotropic scattering in the cuprates

A simple model of anisotropic scattering in a quasi two-dimensional metal is studied. Its simplicity allows an analytic calculation of transport properties using the Boltzmann equation and relaxation time approximation. We argue that the c-axis magnetoresistance provides the key test of this model of transport. We compare this model with experiments on overdoped Tl-2201 and find reasonable agreement using only weak scattering anisotropy. We argue that optimally doped Tl-2201 should show strong angular-dependent magnetoresistance within this model and would provide a robust way of determining the in-plane scattering anisotropy in the cuprates.Comment: 12 pages, 8 figures, typset in REVTeX 4. Version 2; added references and corrected typo

C-axis Raman spectra of a normal plane-chain bilayer cuprate and the pseudogap

We investigate the Raman spectra in the geometry where both incident and scattered photon polarizations are parallel to the $\hat{z}$-direction, for a plane-chain bilayer coupled via a single-particle tunneling $t_\perp$. The Raman vertex is derived in the tight-binding limit and in the absence of Coulomb screening, the Raman intensity can be separated into intraband ($\propto t_\perp^4$) and interband ($\propto t_\perp^2$) transitions. In the small-$t_\perp$ limit, the interband part dominates and a pseudogap will appear as it does in the conductivity. Coulomb interactions bring in a two-particle coupling and result in the breakdown of intra- and interband separation. Nevertheless, when $t_\perp$ is small, the Coulomb screening ($\propto t_\perp^4$) has little effect on the intensity to which the unscreened interband transitions contribute most. In general, the total Raman spectra are strongly dependent on the magnitude of $t_\perp$.Comment: 23 pages, 6 figures, submitted to Phys. Rev.