46 research outputs found
EvolveGCN: Evolving Graph Convolutional Networks for Dynamic Graphs
Graph representation learning resurges as a trending research subject owing
to the widespread use of deep learning for Euclidean data, which inspire
various creative designs of neural networks in the non-Euclidean domain,
particularly graphs. With the success of these graph neural networks (GNN) in
the static setting, we approach further practical scenarios where the graph
dynamically evolves. Existing approaches typically resort to node embeddings
and use a recurrent neural network (RNN, broadly speaking) to regulate the
embeddings and learn the temporal dynamics. These methods require the knowledge
of a node in the full time span (including both training and testing) and are
less applicable to the frequent change of the node set. In some extreme
scenarios, the node sets at different time steps may completely differ. To
resolve this challenge, we propose EvolveGCN, which adapts the graph
convolutional network (GCN) model along the temporal dimension without
resorting to node embeddings. The proposed approach captures the dynamism of
the graph sequence through using an RNN to evolve the GCN parameters. Two
architectures are considered for the parameter evolution. We evaluate the
proposed approach on tasks including link prediction, edge classification, and
node classification. The experimental results indicate a generally higher
performance of EvolveGCN compared with related approaches. The code is
available at \url{https://github.com/IBM/EvolveGCN}.Comment: AAAI 2020. The code is available at https://github.com/IBM/EvolveGC
Development of an acetylacetonate-modified silica-zirconia composite membrane applicable to gas separation
In this work, an acetylacetonate-modified equimolar SiO2–ZrO2 composite-derived membrane with molecular sieving properties was successfully fabricated. The sol-gel method was successfully employed to chemically modify zirconium tetrabutoxide prior to co-hydrolysis and -condensation with tetraethoxysilane, the resulting sol then used to fabricate a gas separation layer. An acetylacetonate-modified SiO2–ZrO2-derived membrane prepared at 300 °C showed H2 permeance of 9.9 × 10 −7 mol m−2 s−1 Pa−1 with a H2/SF6 permeance ratio of 7,600, which was a significant improvement over pure SiO2–ZrO2-derived membranes (H2 permeance: 1.4 × 10 −6 mol m−2 s−1 Pa−1, H2/SF6 permeance ratio: 11). Heat-treatment of an acac−-modified SiO2–ZrO2-derived membrane prepared at temperatures that ranged from 250 °C (H2 permeance: 4.5 × 10−8 mol m−2 s−1 Pa−1, H2/CH4: 100, CO2/CH4: 60, H2/SF6: >18,000 at 50 °C) to 550 °C resulted in an improved H2 permeance of 3.4 × 10−6 mol m−2 s−1 Pa−1 with reduced permeance ratios (H2/CH4: 3, H2/SF6: 9) at 50 °C. A membrane prepared by heat-treating a 250 °C-fired membrane at 300 °C showed the best trade-off with H2 permeance-H2/SF6 permeance ratios above the trade-off line compared with membranes prepared at other temperatures