29 research outputs found
Implication of the overlap representation for modelling generalized parton distributions
Based on a field theoretically inspired model of light-cone wave functions,
we derive valence-like generalized parton distributions and their double
distributions from the wave function overlap in the parton number conserved
s-channel. The parton number changing contributions in the t-channel are
restored from duality. In our construction constraints of positivity and
polynomiality are simultaneously satisfied and it also implies a model
dependent relation between generalized parton distributions and transverse
momentum dependent parton distribution functions. The model predicts that the
t-behavior of resulting hadronic amplitudes depends on the Bjorken variable
x_Bj. We also propose an improved ansatz for double distributions that embeds
this property.Comment: 15 pages, 8 eps figure
Modelling the sputtering of Au surfaces using a multi time-scale technique
This article was published in the journal, Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences [© The Author(s). Published by the Royal Society] and the definitive version is available at: http://dx.doi.org/10.1098/rspa.2012.0480We present results from an atomistic computer
simulation model of the sputtering of gold crystal
surfaces under 500 eV ion bombardment by Au and
Ar ions for doses up to 1014 ions cm−2. The multi
time-scale technique uses molecular dynamics to
calculate the fast ballistic collision processes in the
early stages of the cascade, whereas an on-the fly
kinetic Monte Carlo technique is used to model the
relaxation and diffusion processes between successive
ion impacts when the defect motion has begun to
be dominated by rare events. The results indicate
a large amount of crystalline recovery between
impacts, some facetting of the crystal surfaces but
no large sub-surface defect accumulation. Because of
this recovery process, sputtering yields and energy
distributions are in good agreement with those
obtained assuming a perfect crystal surface and also
with those experimentally measured
Ab inito thermodynamics and statistical mechanics of diffusion, growth, and self-assembly of quantum dots
Les affections courantes du pied (conseils à l'officine)
AIX-MARSEILLE2-BU Pharmacie (130552105) / SudocSudocFranceF
In situ observation of self-assembled hydrocarbon Fischer–Tropsch products on a cobalt catalyst
Fischer-Tropsch synthesis is a heterogeneous catalytic reaction that creates approximately 2% of the world's fuel. It involves the synthesis of linear hydrocarbon molecules from a gaseous mixture of carbon monoxide and hydrogen at high pressures (from a few to tens of bars) and high temperatures (200-350 €...°C). To gain further insight into the fundamental mechanisms of this industrial process, we have used a purpose-built scanning tunnelling microscope to monitor a cobalt model catalyst under reaction conditions. We show that, after 30 €...minutes of reaction, the terraces of the cobalt catalyst are covered by parallel arrays of stripes. We propose that the stripes are formed by the self-assembly of linear hydrocarbon product molecules. Surprisingly, the width of the stripes corresponds to molecules that are 14 or 15 carbon atoms long. We introduce a simple model that explains the accumulation of such long molecules by describing their monomer-by-monomer synthesis and explicitly accounting for their thermal desorption