Direct measurments of (p,γ) cross sections at astrophysical energies using radioactive beams and the Daresbury Recoil Separator

There are a number of astrophysical environments in which the path of nucleosynthesis proceeds through proton-rich nuclei. Radioactive nuclei have traditionally not been available as beams, and thus proton-capture reactions on these nuclei could only be studied indirectly. At the Holifield Radioactive Ion Beam Facility (HRIBF), some of the first direct measurements of (p,γ) cross sections on radioactive beams have been made. The Daresbury Recoil Separator (DRS) has been used to separate the recoils of interest from the unreacted primary beam and identify them in an isobutane-filled ionization counter. Data from 17F(p,γ)18Ne and 7Be(p,γ)8B measurements are presented

New γ -ray transitions observed in Ne 19 with implications for the O 15 (α,γ) Ne 19 reaction rate

The O15(α,γ)Ne19 reaction is responsible for breakout from the hot CNO cycle in type I x-ray bursts. Understanding the properties of resonances between Ex=4 and 5 MeV in Ne19 is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2- and 7/2-, respectively. γ-ray transitions from these states were studied using triton-γ-γ coincidences from the F19(He3,tγ)Ne19 reaction measured with the GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the Jπ values are actually 7/2- and 9/2-, respectively. These assignments are consistent with the values in the F19 mirror nucleus and in contrast to previously accepted assignments

γ -ray spectroscopy of astrophysically important states in Ca 39

Background: Nova explosions synthesize elements up to A≃40, and discrepancies exist between calculated and observed abundances of Ar and Ca created in the explosion. The K38(p,γ)Ca39 reaction rate has been shown to be influential on these isotopic abundances at the endpoint of nova nucleosynthesis. The energies of the three most important resonances, corresponding to Jπ=5/2+ excited states in the Ca39 nucleus above the proton separation threshold, are uncertain and one has been measured with conflicting values [Er=679(2) versus Er=701(2) keV] in previous experiments. Purpose: Reducing the uncertainties on the resonance energies would allow for a better understanding of the reaction rate. To improve these uncertainties, we searched for γ rays from the depopulation of the corresponding excited states in Ca39. Methods: We report a new measurement of these resonance energies via the observation of previously unobserved γ-ray transitions. These transitions were observed by studying the Ca40(3He,αγ)Ca39 reaction with Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies (GODDESS). The updated resonance energies were then used to calculate the K38(p,γ)Ca39 reaction rate and assess its uncertainties. Results: In total, 23 new transitions were found, including three γ-ray transitions corresponding to the three Jπ=5/2+ states of astrophysical interest at energies of 6156.2(16), 6268.8(22), and 6470.8(19) keV. These correspond to resonance energies in the K38(p,γ)Ca39 reaction of 386(2), 498(2), and 701(2) keV. Conclusions: Updated K38(p,γ)Ca39 reaction rate calculations show a reduced upper limit at nova temperatures. However, the lower-than-previously-measured energy of the 498-keV resonance and uncertainty in its resonance strength increases the upper limit of the rate close to previous estimates at 0.4 GK

Isomers in Pd128 and Pd126: Evidence for a Robust Shell Closure at the Neutron Magic Number 82 in Exotic Palladium Isotopes

The level structures of the very neutron-rich nuclei Pd128 and Pd126 have been investigated for the first time. In the r-process waiting-point nucleus Pd128, a new isomer with a half-life of 5.8(8) μs is proposed to have a spin and parity of 8+ and is a

Astrophysically important 19Ne states studied with the 2H(18F, α+15 O)n reaction

The nuclear structure of 19Ne near the proton threshold is of interest for understanding the rates of proton-induced reactions on 18F in novae. Analogues for several states in the mirror nucleus 19F have not yet been identified in 19Ne indicating the level structure of 19Ne in this region is incomplete. The 18F(d,n)19Ne and 18F(d, p)19F reactions have been measured simultaneously at Ec.m. = 14.9 MeV. The experiments were performed at the Holifield Radioactive Ion Beam Facility (HRIBF) of Oak Ridge National Laboratory (ORNL) by bombarding a 720-μg/cm2 CD2 target with a radioactive 18F beam. The 19Ne states of interest near the proton threshold decay by breakup into a and 15O particles. These decay products were detected in coincidence with position-sensitive E-ΔE silicon telescopes. The α and 15N particles from the break up of the mirror nucleus 19F were also measured with these detectors. Particle identification, coincidence, and Q-value requirements enable us to distinguish the reaction of interest from other reactions. The reconstruction of relative energy of the detected particles reveals the excited states of 19Ne and 19F which are populated. The neutron (proton) angular distributions for states in 19Ne (19F) were extracted using momentum conservation. The observed states in 19Ne and 19F will be presented

S-wave scattering lengths for the Be 7 +p system from an R-matrix analysis

The astrophysical S factor for the radiative proton capture reaction on Be7 (S17) at low energies is affected by the s-wave scattering lengths. We report the measurement of elastic and inelastic scattering cross sections for the Be7+p system in the center-of-mass energy range 0.474-2.740 MeV and center-of-mass angular range 70-150. A radioactive Be7 beam produced at Oak Ridge National Laboratory's (ORNL) Holifield Radioactive Ion Beam Facility was accelerated and bombarded a thin polypropylene (CH2)n target. Scattered ions were detected in the segmented Silicon Detector Array. Using an R-matrix analysis of ORNL and Louvain-la-Neuve cross-section data, the s-wave scattering lengths for channel spins 1 and 2 were determined to be 17.34-1.33+1.11 and -3.18-0.50+0.55 fm, respectively. The uncertainty in the s-wave scattering lengths reported in this work is smaller by a factor of 5-8 compared to the previous measurement, which may reduce the overall uncertainty in S17 at zero energy. The level structure of B8 is discussed based upon the results from this work. Evidence for the existence of 0+ and 2+ levels in B8 at 1.9 and 2.21 MeV, respectively, is observed

New γ -ray transitions observed in Ne 19 with implications for the O 15 (α,γ) Ne 19 reaction rate

The O15(α,γ)Ne19 reaction is responsible for breakout from the hot CNO cycle in type I x-ray bursts. Understanding the properties of resonances between Ex=4 and 5 MeV in Ne19 is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2- and 7/2-, respectively. γ-ray transitions from these states were studied using triton-γ-γ coincidences from the F19(He3,tγ)Ne19 reaction measured with the GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the Jπ values are actually 7/2- and 9/2-, respectively. These assignments are consistent with the values in the F19 mirror nucleus and in contrast to previously accepted assignments

Key Ne 19 States Identified Affecting γ-Ray Emission from F 18 in Novae

Detection of nuclear-decay γ rays provides a sensitive thermometer of nova nucleosynthesis. The most intense γ-ray flux is thought to be annihilation radiation from the β+ decay of F18, which is destroyed prior to decay by the F18(p,α)O15 reaction. Estimates of F18 production had been uncertain, however, because key near-threshold levels in the compound nucleus, Ne19, had yet to be identified. We report the first measurement of the F19(He3,tγ)Ne19 reaction, in which the placement of two long-sought 3/2+ levels is suggested via triton-γ-γ coincidences. The precise determination of their resonance energies reduces the upper limit of the rate by a factor of 1.5-17 at nova temperatures and reduces the average uncertainty on the nova detection probability by a factor of 2.1

Ne 19 level structure for explosive nucleosynthesis

Background: Ne19 is an important isotope in nuclear astrophysics due to its role in both the F18(p,α)O15 and O15(α,γ)Ne19 reactions in novae and Type I x-ray bursts, respectively. The energy levels of Ne19 near the α and proton thresholds (Sα=3529 keV, Sp=6410 keV) correspond to resonances in both of these reactions. Previous measurements to study the structure of Ne19 have focused on both regions in an effort to constrain these reaction rates. Purpose: Discrepancies in the energies, spins, and parities for levels in Ne19 from previous measurements contribute to the reaction-rate uncertainties. Gamma rays from the depopulation of excited states in Ne19 were measured to reduce the level-energy uncertainties and inconsistencies in previous spin-parity assignments. Methods: The F19(He3,t)Ne19 reaction was used to elucidate the structure of Ne19 levels up to Ex=6.9 MeV. The reaction products were measured using Gammasphere ORRUBA: Dual Detectors for Experimental Structure Studies - a coupling of the Oak Ridge Rutgers University Barrel Array and Gammasphere at Argonne National Laboratory. Tritons produced in the reaction were measured in coincidence with γ rays from the deexcitation of Ne19 energy levels. Results: Previously unobserved transitions allowed for discrepancies in the resonance properties relevant to these two reactions to be resolved. In total, 41 transitions from 21 energy levels were measured in Ne19, with 21 of those transitions being previously unobserved. Of particular importance, transitions from two 3/2+ states with energies of 6423(3) and 6441(3) keV, crucial for accurate estimations of the F18(p,α)O15 reaction rate, were found. Conclusions: Energies and spin-parities of important energy levels near the proton and α thresholds were measured and some of the discrepancies in previous measurements were resolved. Measurement of the two near-threshold 3/2+ states reduced the calculated upper limit of the F18(p,α)O15 reaction rate by factors of 1.5-17 in the nova temperature range

γ -ray spectroscopy of astrophysically important states in Ca 39

Background: Nova explosions synthesize elements up to A≃40, and discrepancies exist between calculated and observed abundances of Ar and Ca created in the explosion. The K38(p,γ)Ca39 reaction rate has been shown to be influential on these isotopic abundances at the endpoint of nova nucleosynthesis. The energies of the three most important resonances, corresponding to Jπ=5/2+ excited states in the Ca39 nucleus above the proton separation threshold, are uncertain and one has been measured with conflicting values [Er=679(2) versus Er=701(2) keV] in previous experiments. Purpose: Reducing the uncertainties on the resonance energies would allow for a better understanding of the reaction rate. To improve these uncertainties, we searched for γ rays from the depopulation of the corresponding excited states in Ca39. Methods: We report a new measurement of these resonance energies via the observation of previously unobserved γ-ray transitions. These transitions were observed by studying the Ca40(3He,αγ)Ca39 reaction with Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies (GODDESS). The updated resonance energies were then used to calculate the K38(p,γ)Ca39 reaction rate and assess its uncertainties. Results: In total, 23 new transitions were found, including three γ-ray transitions corresponding to the three Jπ=5/2+ states of astrophysical interest at energies of 6156.2(16), 6268.8(22), and 6470.8(19) keV. These correspond to resonance energies in the K38(p,γ)Ca39 reaction of 386(2), 498(2), and 701(2) keV. Conclusions: Updated K38(p,γ)Ca39 reaction rate calculations show a reduced upper limit at nova temperatures. However, the lower-than-previously-measured energy of the 498-keV resonance and uncertainty in its resonance strength increases the upper limit of the rate close to previous estimates at 0.4 GK