1,858 research outputs found
Observation of intrinsic inverse spin Hall effect
We report observation of intrinsic inverse spin Hall effect in un-doped GaAs
multiple quantum wells with a sample temperature of 10 K. A transient ballistic
pure spin current is injected by a pair of laser pulses through quantum
interference. By time-resolving the dynamics of the pure spin current, the
momentum relaxation time is deduced, which sets the lower limit of the
scattering time between electrons and holes. The transverse charge current
generated by the pure spin current via the inverse spin Hall effect is
simultaneously resolved. We find that the charge current is generated well
before the first electron-hole scattering event. Generation of the transverse
current in the scattering-free ballistic transport regime provides unambiguous
evidence for the intrinsic inverse spin Hall effect.Comment: 4 pages, 3 figure
All-optical generation and detection of sub-picosecond ac spin current pulses in GaAs
Sub-picosecond ac spin current pulses are generated optically in GaAs bulk
and quantum wells at room temperature and 90K through quantum interference
between one-photon and two-photon absorptions driven by two phase-locked
ultrafast laser pulses that are both circularly polarized. The dynamics of the
current pulses are detected optically by monitoring in real time and real space
nanoscale motion of electrons with high-resolution pump-probe techniques.Comment: 5 pages, 5 figure
Femtosecond Pump-Probe Studies of Reduced Graphene Oxide Thin Films
The dynamics of photocarriers in reduced graphene oxide thin films is studied
by using ultrafast pump-probe spectroscopy. Time dependent differential
transmissions are measured with sample temperatures ranging from 9 to 300 K. At
each sample temperature and probe delay, the sign of differential transmission
remains positive. A fast energy relaxation of hot carriers is observed, and is
found to be independent of sample temperature. Our experiments show that the
carrier dynamics in reduced graphene oxide is similar to other types of
graphene, and that the differential transmission is caused by phase-state
filling of carriers.Comment: 3 pages, 3 figure
Spatially resolved femtosecond pump-probe study of topological insulator Bi2Se3
Carrier and phonon dynamics in Bi2Se3 crystals are studied by a spatially
resolved ultrafast pump-probe technique. Pronounced oscillations in
differential reflection are observed with two distinct frequencies, and are
attributed to coherent optical and acoustic phonons, respectively. The rising
time of the signal indicates that the thermalization and energy relaxation of
hot carriers are both sub-ps in this material. We found that the thermalization
and relaxation time decreases with the carrier density. The expansion of the
differential reflection profile allows us to estimate an ambipolar carrier
diffusion coefficient on the order of 500 square centimeters per second. A
long-term slow expansion of the profile shows a thermal diffusion coefficient
of 1.2 square centimeters per second.Comment: 8 pages, 6 figure
On the Refractive Index of Ageing Dispersions of Laponite
Aqueous dispersion of Laponite at low ionic concentration is of interest
since it undergoes structural evolution with respect to time, which is usually
termed as ageing. In this work we study the refractive index behavior as a
function of ageing time, concentration and temperature. We observed that the
extended Lorenz-Lorentz equation fitted the refractive index dependence on
concentration and temperature very well. The refractive index did not show any
dependence on ageing time. However, the dependence of refractive index on
concentration showed a marked change as the system underwent transition from an
isotropic to a biphasic state. The slope of the refractive index-density data
is remarkably close to that of water at all Laponite concentrations. In the
context of transport phenomena, optical measurements such as interferometry can
exploit the water-like behavior of Laponite dispersions.Comment: 13 pages, 3 figures, to appear in Applied Clay Scienc
Hot carrier diffusion in graphene
We report an optical study of charge transport in graphene. Diffusion of hot
carriers in epitaxial graphene and reduced graphene oxide samples are studied
using an ultrafast pump-probe technique with a high spatial resolution.
Spatiotemporal dynamics of hot carriers after a point-like excitation are
monitored. Carrier diffusion coefficients of 11,000 and 5,500 squared
centimeters per second are measured in epitaxial graphene and reduced graphene
oxide samples, respectively, with a carrier temperature on the order of 3,600
K. The demonstrated optical techniques can be used for non-contact and
non-invasive in-situ detection of transport properties of graphene.Comment: 5 pages, 3 figure
THERMAL PROPERTIES AND HOMOGENITY RANGE OF Bi24+xCo2-xO39 CERAMICS
Samples with different Bi2O3/Co2O3 ratio were prepared by ceramic route. Based on the results of DTA, XRD and SEM – EDX a section of phase diagram of the Bi–Co–O diagram in air atmosphere was calculated using the FactSage software. The sillenite structure of Bi24+xCo2-xO39 was confirmed and described. The Rietveld analysis confirmed SEM – EDX results. The heat capacity and enthalpy increments of Bi24Co2O39 were measured by differential scanning calorimetry (DSC) from 258 K to 355 K and by the drop calorimetry from 573 K to 973 K. Above room temperature the temperature dependence of the molar heat capacity in the form Cpm = (1467.87 + 0.299410 · T – 15888378 · T-2) J K-1 mol-1 was derived by least-squares method from the experimental data
Ambipolar diffusion of photo-excited carriers in bulk GaAs
The ambipolar carrier diffusion in bulk GaAs is studied by using an ultrafast
pump-probe technique with a high spatial resolution. Carriers with a point-like
spatial profile are excited by a tightly focused pump laser pulse. The
spatiotemporal dynamics of the carriers are monitored by a time-delayed and
spatially scanned probe pulse. Ambipolar diffusion coefficients are deduced
from linear fits to the expansion of the area of the profiles, and are found to
decrease from about 170~ at 10 K to about
20~ at room temperature. Our results are
consistent with those deduced from the previously measured mobilities.Comment: 4 pages, 4 figure
Unexpected effect of small viscosity on flow regimes in bubble columns
Bubble column contacting/reacting systems are widely used in many technologies of chemical
and food industry, in biotechnology, and in environmental areas. The transport parameters of
the system depend strongly on the flow regimes in the apparatus (homogeneous and
heterogeneous regimes). One regime can change into the other at critical values of control
parameters - system size and geometry, physico-chemical properties of the phases, etc. This
study concerns the effect of the liquid phase viscosity on the extent the homogeneous regime.
Experiments were performed in cylindrical bubble columns with solutions of different
Newtonian viscosity. The data show that the uniform regime can be both supported and
deteriorated with small changes in viscosity.Supported by GAČR (Grant No. 104/04/0827) and by the EC (BEMUSAC Project No. G1MA-CT-2002-04019 and Marie Curie Training Site Fellowship of P. C. Mena at the Institute of Chemical Process Fundamentals, Prague, CZ, Contract Number HPMT-CT-200000074).
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