53 research outputs found
Single spin optical read-out in CdTe/ZnTe quantum dot studied by photon correlation spectroscopy
Spin dynamics of a single electron and an exciton confined in CdTe/ZnTe
quantum dot is investigated by polarization-resolved correlation spectroscopy.
Spin memory effects extending over at least a few tens of nanoseconds have been
directly observed in magnetic field and described quantitatively in terms of a
simple rate equation model. We demonstrate an effective (68%) all-optical
read-out of the single carrier spin state through probing the degree of
circular polarization of exciton emission after capture of an oppositely
charged carrier. The perturbation introduced by the pulsed optical excitation
serving to study the spin dynamics has been found to be the main source of the
polarization loss in the read-out process. In the limit of low laser power the
read-out efficiency extrapolates to a value close to 100%. The measurements
allowed us as well to determine neutral exciton spin relaxation time ranging
from 3.4 +/- 0.1 ns at B = 0 T to 16 +/- 3 ns at B = 5 T.Comment: to appear in Phys. Rev.
Revealing exciton masses and dielectric properties of monolayer semiconductors with high magnetic fields
In semiconductor physics, many essential optoelectronic material parameters
can be experimentally revealed via optical spectroscopy in sufficiently large
magnetic fields. For monolayer transition-metal dichalcogenide semiconductors,
this field scale is substantial --tens of teslas or more-- due to heavy carrier
masses and huge exciton binding energies. Here we report absorption
spectroscopy of monolayer MoS, MoSe, MoTe, and WS in very high
magnetic fields to 91~T. We follow the diamagnetic shifts and valley Zeeman
splittings of not only the exciton's ground state but also its excited
, , ..., Rydberg states. This provides a direct experimental
measure of the effective (reduced) exciton masses and dielectric properties.
Exciton binding energies, exciton radii, and free-particle bandgaps are also
determined. The measured exciton masses are heavier than theoretically
predicted, especially for Mo-based monolayers. These results provide essential
and quantitative parameters for the rational design of opto-electronic van der
Waals heterostructures incorporating 2D semiconductors.Comment: updated; now also including data on MoTe2. Accepted & in press,
Nature Commu
Enhancement of electron magnetic susceptibility due to many-body interactions in monolayer MoSe
Employing the original, all-optical method, we quantify the magnetic
susceptibility of a two-dimensional electron gas (2DEG) confined in the
MoSe monolayer in the range of low and moderate carrier densities. The
impact of electron-electron interactions on the 2DEG magnetic susceptibility is
found to be particularly strong in the limit of, studied in detail, low carrier
densities. Following the existing models, we derive for the
bare (single particle) g-factor of the ground state electronic band in the
MoSe monolayer. The derived value of this parameter is discussed in the
context of estimations from other experimental approaches. Surprisingly, the
conclusions drawn differ from theoretical ab-initio studies
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