492 research outputs found
Observation of a Distribution of Internal Transverse Magnetic Fields in a Mn12-Based Single Molecule Magnet
A distribution of internal transverse magnetic fields has been observed in
single molecule magnet (SMM) Mn12-BrAc in the pure magnetic quantum tunneling
(MQT) regime. Magnetic relaxation experiments at 0.4 K are used to produce a
hole in the distribution of transverse fields whose angle and depth depend on
the orientation and amplitude of an applied transverse ``digging field.'' The
presence of such transverse magnetic fields can explain the main features of
resonant MQT in this material, including the tunneling rates, the form of the
relaxation and the absence of tunneling selection rules. We propose a model in
which the transverse fields originate from a distribution of tilts of the
molecular magnetic easy axes.Comment: 4 page
Asymmetric Berry-Phase Interference Patterns in a Single-Molecule Magnet
A Mn4 single-molecule magnet displays asymmetric Berry-phase interference
patterns in the transverse-field (HT) dependence of the magnetization tunneling
probability when a longitudinal field (HL) is present, contrary to symmetric
patterns observed for HL=0. Reversal of HL results in a reflection of the
transverse-field asymmetry about HT=0, as expected on the basis of the
time-reversal invariance of the spin-orbit Hamiltonian which is responsible for
the tunneling oscillations. A fascinating motion of Berry-phase minima within
the transverse-field magnitude-direction phase space results from a competition
between noncollinear magnetoanisotropy tensors at the two distinct Mn sites.Comment: 4 double-column page
Magnetization and EPR studies of the single molecule magnet Ni with integrated sensors
Integrated magnetic sensors that allow simultaneous EPR and magnetization
measurements have been developed to study single molecule magnets. A high
frequency microstrip resonator has been integrated with a micro-Hall effect
magnetometer. EPR spectroscopy is used to determine the energy splitting
between the low lying spin-states of a Ni single crystal, with an S=4
ground state, as a function of applied fields, both longitudinal and transverse
to the easy axis at 0.4 K. Concurrent magnetization measurements show changes
in spin-population associated with microwave absorption. Such studies enable
determination of the energy relaxation time of the spin system.Comment: 4 pages, 4 figures, accepted for publication (Proceedings of the 10th
Joint MMM/Intermag Conference, which will be published as special issues of
the Journal of Applied Physics
Definitive spectroscopic determination of the transverse interactions responsible for the magnetic quantum tunneling in Mn12-acetate
We present detailed angle-dependent single crystal electron paramagnetic
resonance (EPR) data for field rotations in the hard plane of the S=10 single
molecule magnet Mn12-acetate. A clear four-fold variation in the resonance
positions may be attributed to an intrinsic fourth order transverse anisotropy
(O44). Meanwhile, a four-fold variation of the EPR lineshapes confirms a
recently proposed model wherein disorder associated with the acetic acid of
crystallization induces a locally varying quadratic (rhombic) transverse
anisotropy (O22). These findings explain most aspects of the magnetic quantum
tunneling observed in Mn12-acetate.Comment: 7 pages, including figures, accepted for publication in Phys. Rev.
Let
High frequency resonant experiments in Fe molecular clusters
Precise resonant experiments on Fe magnetic clusters have been
conducted down to 1.2 K at various tranverse magnetic fields, using a
cylindrical resonator cavity with 40 different frequencies between 37 GHz and
110 GHz. All the observed resonances for both single crystal and oriented
powder, have been fitted by the eigenstates of the hamiltonian . We have identified the
resonances corresponding to the coherent quantum oscillations for different
orientations of spin S = 10.Comment: to appear in Phys.Rev. B (August 2000
Magnetic qubits as hardware for quantum computers
We propose two potential realisations for quantum bits based on nanometre
scale magnetic particles of large spin S and high anisotropy molecular
clusters. In case (1) the bit-value basis states |0> and |1> are the ground and
first excited spin states Sz = S and S-1, separated by an energy gap given by
the ferromagnetic resonance (FMR) frequency. In case (2), when there is
significant tunnelling through the anisotropy barrier, the qubit states
correspond to the symmetric, |0>, and antisymmetric, |1>, combinations of the
two-fold degenerate ground state Sz = +- S. In each case the temperature of
operation must be low compared to the energy gap, \Delta, between the states
|0> and |1>. The gap \Delta in case (2) can be controlled with an external
magnetic field perpendicular to the easy axis of the molecular cluster. The
states of different molecular clusters and magnetic particles may be entangled
by connecting them by superconducting lines with Josephson switches, leading to
the potential for quantum computing hardware.Comment: 17 pages, 3 figure
Magnetic Quantum Tunneling: Insights from Simple Molecule-Based Magnets
This article takes a broad view of the understanding of magnetic bistability
and magnetic quantum tunneling in single-molecule magnets (SMMs), focusing on
three families of relatively simple, low-nuclearity transition metal clusters:
spin S = 4 Ni4, Mn(III)3 (S = 2 and 6) and Mn(III)6 (S = 4 and 12). The Mn(III)
complexes are related by the fact that they contain triangular Mn3 units in
which the exchange may be switched from antiferromagnetic to ferromagnetic
without significantly altering the coordination around the Mn(III) centers,
thereby leaving the single-ion physics more-or-less unaltered. This allows for
a detailed and systematic study of the way in which the individual-ion
anisotropies project onto the molecular spin ground state in otherwise
identical low- and high-spin molecules, thus providing unique insights into the
key factors that control the quantum dynamics of SMMs, namely: (i) the height
of the kinetic barrier to magnetization relaxation; and (ii) the transverse
interactions that cause tunneling through this barrier. Numerical calculations
are supported by an unprecedented experimental data set (17 different
compounds), including very detailed spectroscopic information obtained from
high-frequency electron paramagnetic resonance and low-temperature hysteresis
measurements. Diagonalization of the multi-spin Hamiltonian matrix is necessary
in order to fully capture the interplay between exchange and local anisotropy,
and the resultant spin-state mixing which ultimately gives rise to the
tunneling matrix elements in the high symmetry SMMs (ferromagnetic Mn3 and
Ni4). The simplicity (low-nuclearity, high-symmetry, weak disorder, etc..) of
the molecules highlighted in this study proves to be of crucial importance.Comment: 32 pages, incl. 6 figure
Implementing Elements of The Physics Suite at a Large Metropolitan Research University
A key question in physics education is the effectiveness of the teaching
methods. A curriculum that has been investigated at the University of Central
Florida (UCF) over a period of two years is the use of particular elements of
The Physics Suite. Select sections of the introductory physics classes at UCF
have made use of Interactive Lecture Demonstrations as part of the lecture
component of the class. The lab component of the class has implemented the
RealTime Physics curriculum, again in select sections. The remaining sections
have continued with the teaching methods traditionally used. Using pre- and
post-semester concept inventory tests, a student survey, student interviews,
and a standard for successful completion of the course, the data indicates
improved student learning
On the Energy Transfer Performance of Mechanical Nanoresonators Coupled with Electromagnetic Fields
We study the energy transfer performance in electrically and magnetically
coupled mechanical nanoresonators. Using the resonant scattering theory, we
show that magnetically coupled resonators can achieve the same energy transfer
performance as for their electrically coupled counterparts, or even outperform
them within the scale of interest. Magnetic and electric coupling are compared
in the Nanotube Radio, a realistic example of a nano-scale mechanical
resonator. The energy transfer performance is also discussed for a newly
proposed bio-nanoresonator composed of a magnetosomes coated with a net of
protein fibers.Comment: 9 Pages, 3 Figure
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