Exponential Decay of Correlations in a Model for Strongly Disordered 2D Nematic Elastomers

Lattice Monte-Carlo simulations were performed to study the equilibrium ordering in a two-dimensional nematic system with quenched random disorder. When the disordering field, which competes against the aligning effect of the Frank elasticity, is sufficiently strong, the long-range correlation of the director orientation is found to decay as a simple exponential, Exp[-r/x]. The correlation length {x} itself also decays exponentially with increasing strength of the disordering field. This result represents a new type of behavior, distinct from the Gaussian and power-law decays predicted by some theories.Comment: Latex file (4 pages) + 2 EPS figure

Evolution of the fishtail-effect in pure and Ag-doped MG-YBCO

We report on magnetic measurements carried out in a textured YBa$_2$Cu$_3$O$_{7-\delta}$ and YBa$_2$(Cu$_{1-x}$Ag$_x$)$_3$O$_{7-\delta}$ (at $x \approx$ 0.02) crystals. The so-called fishtail-effect (FE) or second magnetization peak has been observed in a wide temperature range 0.4~$<T/T_c<$~0.8 for $\textbf{H}\parallel c$. The origin of the FE arises for the competition between surface barrier and bulk pinning. This is confirmed in a non-monotonically behavior of the relaxation rate $R$. The value $H_{max}$ for Ag-doped crystals is larger than for the pure one due to the presence of additional pinning centers, above all on silver atoms.Comment: 6 pages, 6 figure

Saturable metabolism of continuous high-dose ifosfamide with Mesna and GM-CSF: A pharmacokinetic study in advanced sarcoma patients

Background: The aim of this study was to assess the pharmacology, toxicity and activity of high-dose ifosfamide/mesna ± GM-CSF administered by a five-day continuous infusion at a total ifosfamide dose of 12-18 g/m2 in adult patients with advanced sarcomas. Patients and methods: Between January 1991 and October 1992 32 patients with advanced or metastatic sarcoma were entered the study. Twenty-seven patients were pretreated including twenty-three with prior ifosfamide at less than 8 g/m2 total dose/cycle. In 25 patients (27 cycles) extensive pharmacokinetic analyses were performed. Results: The area under the plasma concentration-time curve (AUC) for ifosfamide increased linearly with dose while the AUC's of the metabolites measured in plasma by thin-layer chromatography did not increase with dose, particularly that of the active metabolite isophosphoramide mustard. Furthermore the AUC of the inactive carboxymetabolite did not increase with dose. Interpatient variability of pharmacokinetic parameters was high. Dose-limiting toxicity was myelosup-pression at 18 g/m2 total dose with grade 4 neutropenia in five of six patients and grade 4 thrombocytopenia in four of six patients. Therefore the maximum tolerated dose was considered to be 18 g/m2 total dose. There was one CR and eleven PR in twenty-nine evaluable patients (overall response rate 41%). Conclusion: Both the activation and inactivation pathways of ifosfamide are non-linear and saturable at high-doses although the pharmacokinetics of the parent drug itself are dose linear. Ifosfamide doses greater than 14-16 g/m2 per cycle appear to result in a relative decrease of the active metabolite isophosphoramide mustard. These data suggest a dose-dependent saturation or even inhibition of ifosfamide metabolism by increasing high dose ifosfamide and suggest the need for further metabolic studie

Surface-Emitted Green Light Generated In Langmuir-Blodgett-Film Wave-Guides

We demonstrate second-harmonic generation due to counterpropagating beams in planar waveguides of 2-docosylamino-5-nitropyridine (DCANP). The DCANP molecules were deposited by Langmuir-Blodgett techniques and have a preferred alignment within the substrate plane. Four-layer waveguide structures were used to optimize the trade-off between propagation loss and efficient surface-emitted green light

Slow stress relaxation in randomly disordered nematic elastomers and gels

Randomly disordered (polydomain) liquid crystalline elastomers align under stress. We study the dynamics of stress relaxation before, during and after the Polydomain-Monodomain transition. The results for different materials show the universal ultra-slow logarithmic behaviour, especially pronounced in the region of the transition. The data is approximated very well by an equation Sigma(t) ~ Sigma_{eq} + A/(1+ Alpha Log[t]). We propose a theoretical model based on the concept of cooperative mechanical resistance for the re-orientation of each domain, attempting to follow the soft-deformation pathway. The exact model solution can be approximated by compact analytical expressions valid at short and at long times of relaxation, with two model parameters determined from the data.Comment: 4 pages (two-column), 5 EPS figures (included via epsfig

Peak effect, vortex-lattice melting-line and order - disorder transition in conventional and high-T superconductors

We investigate the order - disorder transition line from a Bragg glass to an amorphous vortex glass in the H-T phase diagram of three-dimensional type-II superconductors with account of both pinning-caused and thermal fluctuations of the vortex lattice. Our approach is based on the Lindemann criterion and on results of the collective pinning theory and generalizes previous work of other authors. It is shown that the shapes of the order - disorder transition line and the vortex lattice melting curve are determined only by the Ginzburg number, which characterizes thermal fluctuations, and by a parameter which describes the strength of the quenched disorder in the flux-line lattice. In the framework of this unified approach we obtain the H-T phase diagrams for both conventional and high-Tc superconductors. Several well-known experimental results concerning the fishtail effect and the phase diagram of high-Tc superconductors are naturally explained by assuming that a peak effect in the critical current density versus H signalizes the order - disorder transition line in superconductors with point defects.Comment: 15 pages including 11 figure

Low field vortex dynamics over seven time decades in a Bi_2Sr_2CaCu_2O_{8+\delta} single crystal for temperatures 13 K < T < 83 K

Using a custom made dc-SQUID magnetometer, we have measured the time relaxation of the remanent magnetization M_rem of a Bi_2Sr_2CaCu_2O_{8+\delta} single crystal from the fully critical state for temperatures 13 K < T < 83 K. The measurements cover a time window of seven decades 10^{-2} s < t < 10^5 s, so that the current density j can be studied from values very close to j_c down to values considerably smaller than j_c. From the data we have obtained: (i) the flux creep activation barriers U as a function of current density j, (ii) the current-voltage characteristics E(j) in a typical range of 10^{-7} V/cm to 10^{-15} V/cm, and (iii) the critical current density j_c(0) at T = 0. Three different regimes of vortex dynamics are observed: For temperatures T < 20 K the activation barrier U(j) is logarithmic, no unique functional dependence U(j) could be found for the intermediate temperature interval 20 K < T < 40 K, and finally for T > 40 K the activation barrier U(j) follows a power-law behavior with an exponent mu = 0.6. From the analysis of the data within the weak collective pinning theory for strongly layered superconductors, it is argued that for temperatures T < 20 K pancake-vortices are pinned individually, while for temperatures T > 40 K pinning involves large collectively pinned vortex bundles. A description of the vortex dynamics in the intermediate temperature interval 20 K < T < 40 K is given on the basis of a qualitative low field phase diagram of the vortex state in Bi_2Sr_2CaCu_2O_{8+\delta}. Within this description a second peak in the magnetization loop should occur for temperatures between 20 K and 40 K, as it has been observed in several magnetization measurements in the literature.Comment: 12 pages, 10 figure

Soft and non-soft structural transitions in disordered nematic networks

Properties of disordered nematic elastomers and gels are theoretically investigated with emphasis on the roles of non-local elastic interactions and crosslinking conditions. Networks originally crosslinked in the isotropic phase lose their long-range orientational order by the action of quenched random stresses, which we incorporate into the affine-deformation model of nematic rubber elasticity. We present a detailed picture of mechanical quasi-Goldstone modes, which accounts for an almost completely soft polydomain-monodomain (P-M) transition under strain as well as a ``four-leaf clover'' pattern in depolarized light scattering intensity. Dynamical relaxation of the domain structure is studied using a simple model. The peak wavenumber of the structure factor obeys a power-law-type slow kinetics and goes to zero in true mechanical equilibrium. The effect of quenched disorder on director fluctuation in the monodomain state is analyzed. The random frozen contribution to the fluctuation amplitude dominates the thermal one, at long wavelengths and near the P-M transition threshold. We also study networks obtained by crosslinking polydomain nematic polymer melts. The memory of initial director configuration acts as correlated and strong quenched disorder, which renders the P-M transition non-soft. The spatial distribution of the elastic free energy is strongly dehomogenized by external strain, in contrast to the case of isotropically crosslinked networks.Comment: 19 pages, 15 EPS figure

Elastic-to-plastic crossover below the peak effect in the vortex solid of YBa2Cu3O7 single crystals

We report on transport and ac susceptibility studies below the peak effect in twinned YBa2Cu3O7 single crystals. We find that disorder generated at the peak effect can be partially inhibited by forcing vortices to move with an ac driving current. The vortex system can be additionally ordered below a well-defined temperature where elastic interactions between vortices overcome pinning-generated stress and a plastic to elastic crossover seems to occur. The combined effect of these two processes results in vortex structures with different mobilities that give place to history effects.Comment: 4 pages, 4 figures. Published in PRB Rapid Comm., February 1, 200

Scaling Behavior of Anomalous Hall Effect and Longitudinal Nonlinear Response in High-Tc Superconductors

Based on existing theoretical model and by considering our longitudinal nonlinear response function, we derive a nonliear equation in which the mixed state Hall resistivity can be expressed as an analytical function of magnetic field, temperature and applied current. This equation enables one to compare quantitatively the experimental data with theoretical model. We also find some new scaling relations of the temperature and field dependency of Hall resistivity. The comparison between our theoretical curves and experimental data shows a fair agreement.Comment: 4 pages, 3 figure