Spin/Orbital Pattern-Dependent Polaron Absorption in Nd(1-x)Sr(x)MnO3

We investigated optical properties of Nd(1-x)Sr(x)MnO3 (x= 0.40, 0.50, 0.55, and 0.65) single crystals. In the spin/orbital disordered state, their conductivity spectra look quite similar, and the strength of the mid-infrared absorption peak is proportional to x(1-x) consistent with the polaron picture. As temperature lowers, the Nd(1-x)Sr(x)MnO3 samples enter into various spin/orbital ordered states, whose optical responses are quite different. These optical responses can be explained by the spin/orbital ordering pattern-dependent polaron hopping.Comment: 3 figures (gzipped

Recent Progress in Droplet-Based Manufacturing Research

This article reports the recent progress of re-search made in the Droplet-Based Manufacturing Laboratory at MIT. The study has been focused on obtaining a fundamental understanding of microdroplet deposition and applying the technology to various practical applications. Specific scientific contributions include the development of an analytical model for droplet splashing/recoiling, an in situ droplet size control methodology, and a study of microstructure design for spray forming. The research per-formed in the lab provides both fundamental knowledge base and practical process developments for a range of manufacturing applications, including electronics packaging, spray forming and freeform fabrication.Singapore-MIT Alliance (SMA

Melting of Charge/Orbital Ordered States in Nd1/2_{1/2}Sr1/2_{1/2}MnO3_3: Temperature and Magnetic Field Dependent Optical Studies

We investigated the temperature ($T=$ 15 $\sim$ 290 K) and the magnetic field ($H=$ 0 $\sim$ 17 T) dependent optical conductivity spectra of a charge/orbital ordered manganite, Nd$_{1/2}$Sr$_{1/2}$MnO$_3$. With variation of $T$ and $H$, large spectral weight changes were observed up to 4.0 eV. These spectral weight changes could be explained using the polaron picture. Interestingly, our results suggested that some local ordered state might remain above the charge ordering temperature, and that the charge/orbital melted state at a high magnetic field (i.e. at $H=$ 17 T and $$ 4.2 K) should be a three dimensional ferromagnetic metal. We also investigated the first order phase transition from the charge/orbital ordered state to ferromagnetic metallic state using the $T$- and $H$% -dependent dielectric constants $\epsilon_1$. In the charge/orbital ordered insulating state, $\epsilon_1$ was positive and $d\epsilon_1/d\omega \approx 0$. With increasing $T$ and $H$, $\epsilon_1$ was increased up to the insulator-metal phase boundaries. And then, $\epsilon_1$ abruptly changed into negative and $d\epsilon_1/d\omega >0$, which was consistent with typical responses of a metal. Through the analysis of $\epsilon_1$ using an effective medium approximation, we found that the melting of charge/orbital ordered states should occur through the percolation of ferromagnetic metal domains.Comment: submitted to Phys. Rev.

Nearly Massless Electrons in the Silicon Interface with a Metal Film

We demonstrate the realization of nearly massless electrons in the most widely used device material, silicon, at the interface with a metal film. Using angle-resolved photoemission, we found that the surface band of a monolayer lead film drives a hole band of the Si inversion layer formed at the interface with the film to have nearly linear dispersion with an effective mass about 20 times lighter than bulk Si and comparable to graphene. The reduction of mass can be accounted for by repulsive interaction between neighboring bands of the metal film and Si substrate. Our result suggests a promising way to take advantage of massless carriers in silicon-based thin-film devices, which can also be applied for various other semiconductor devices.Comment: 4 pages, 4 figures, accepted for publication in Physical Review Letter

High-Performance, Wearable Thermoelectric Generator Based on a Highly Aligned Carbon Nanotube Sheet

A high-performance, wearable thermoelectric generator (TEG) was fabricated with a highly aligned carbon nanotube (CNT) sheet. The aligned CNT sheet exhibits extraordinary electrical conductivity compared to disordered CNT sheets and also can be directly fabricated as a continuous TEG without metal electrode interconnects. This provides a significant reduction in contact resistance between TE legs and electrodes compared to traditional TEGs, resulting in higher power output. In addition, the continuity of the module without any disconnected parts provides high degrees of mechanical stability and durability. This robust and scalable approach to flexible TEG fabrication paves the way for CNT applications in lightweight, flexible, and wearable electronics

A Scaling Behavior of Spectral Weight Changes in Perovskite Manganites La_{0.7-y}Pr_{y}Ca_{0.3}MnO_3

Optical conductivity spectra of La_{0.7-y}Pr_{y}Ca_{0.3}MnO_3 were systematically investigated. For metallic samples, the spectral weight below 0.5 eV, whose magnitude can be represented by the effective carrier number N_{eff}(0.5 eV), increases as temperature becomes lower. Regardless of the Pr doping, all the measured values of N_{eff}(0.5 eV)/T_C fall into one scaling curve. This scaling behavior could be explained by the theoretical model by Roeder et al. [Phys. Rev. Lett. 76, 1356 (1996)], which includes spin double exchange and Jahn-Teller lattice coupling to holes. With the Pr doping, far-infrared conductivities were found to be suppressed, probably due to the Anderson localization.Comment: Latex 2e, 8 pages including 4 postscript figures, submitted at Apr 2

Prompt photon hadroproduction at high energies in off-shell gluon-gluon fusion

The amplitude for production of a single photon associated with quark pair in the fusion of two off-shell gluons is calculated. The matrix element found is applied to the inclusive prompt photon hadroproduction at high energies in the framework of kt-factorization QCD approach. The total and differential cross sections are calculated in both central and forward pseudo-rapidity regions. The conservative error analisys is performed. We used the unintegrated gluon distributions in a proton which were obtained from the full CCFM evolution equation as well as from the Kimber-Martin-Ryskin prescription. Theoretical results were compared with recent experimental data taken by the D0 and CDF collaborations at Fermilab Tevatron. Theoretical predictions for the LHC energies are given.Comment: 32 pages, 18 figure

Optical Investigations of Charge Gap in Orbital Ordered La1/2Sr3/2MnO4

Temperature and polarization dependent electronic structure of La1/2Sr3/2MnO4 were investigated by optical conductivity analyses. With decreasing temperature, for E//ab, a broad mid-infrared (MIR) peak of La1/2Sr3/2MnO4 becomes narrower and moves to the higher frequency, while that of Nd1/2Sr3/2MnO4 nearly temperature independent. We showed that the MIR peak in La1/2Sr3/2MnO4 originates from orbital ordering associated with CE-type magnetic ordering and that the Jahn-Teller distortion has a significant influence on the width and the position of the MIR peak.Comment: 10 pages, 4 figure

Non-Markovian stochastic Liouville equation and anomalous relaxation kinetics

The kinetics of phase and population relaxation in quantum systems induced by noise with anomalously slowly decaying correlation function P (t) ~ (wt)^{- alpha}, where 0 < alpha < 1 is analyzed within continuous time random walk approach. The relaxation kinetics is shown to be anomalously slow. Moreover for alpha < 1 in the limit of short characteristic time of fluctuations w^{-1} the kinetics is independent of w. As alpha \to 1 the relaxation regime changes from the static limit to fluctuation narrowing. Simple analytical expressions are obtained describing the specific features of the kinetics.Comment: 7 pages, 2 figure