11 research outputs found

    Toward Tandem Photovoltaic Devices Employing Nanoarray Graphene-Based Sheets

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    Graphene quantum dots (GQDs) are promising photonic materials for light harvesting. However, only low photoelectron conversion efficiency can be generated in single-junction graphene-based solar cells when isolated GQDs with the edge bonding defects are used as semiconductors. To address this issue, a four-junction GQD-based tandem solar cell with high theoretical conversion efficiency was proposed in this paper. Instead of isolated GQDs, nanoarray GQDs embedded in hexagonal host materials, such as graphane or boron nitride, was adopted as the photoactive layer. Utilizing our universal thermodynamic approach to the gap openings in low-dimensional graphene, nanoarray armchair-interfaced GQDs embedded in graphane to achieve the maximal diameter of confined GQDs are found preferential for fabricating tandem solar cell devices. Besides these, the separation between GQDs and the thickness of GQD-based sheets were determined. This contribution is of benefit to the application of graphene for solar cell devices

    Synthesis of a Thin-Layer MnO<sub>2</sub> Nanosheet-Coated Fe<sub>3</sub>O<sub>4</sub> Nanocomposite as a Magnetically Separable Photocatalyst

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    A facile hydrothermal method combined with a mild ultrasonic means has been developed for the fabrication of a magnetically recyclable thin-layer MnO<sub>2</sub> nanosheet-coated Fe<sub>3</sub>O<sub>4</sub> nanocomposite. The photocatalytic studies suggest that the MnO<sub>2</sub>/Fe<sub>3</sub>O<sub>4</sub> nanocomposite shows excellent photocatalytic efficiency and stability simultaneously for the degradation of methylene blue under UV–vis light irradiation. Moreover, its good acid resistance and stable recyclability are very important for its future practical application as a photocatalyst. Magnetic measurements verify that the MnO<sub>2</sub>/Fe<sub>3</sub>O<sub>4</sub> nanocomposite possesses a ferromagnetic nature, which can be effectively separated for reuse by simply applying an external magnetic field after the photocatalytic reaction. This novel composite material may have potential applications in water treatment, degradation of dye pollutants, and environmental cleaning

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost

    Dual Superlyophobic Copper Foam with Good Durability and Recyclability for High Flux, High Efficiency, and Continuous Oil–Water Separation

    No full text
    Traditional oil–water separation materials have to own ultrahigh or ultralow surface energy. Thus, they can only be wetted by one of the two, oil or water. Our experiment here demonstrates that the wettability in oil–water mixtures can be tuned by oil and water initially. Hierarchical voids are built on commercial copper foams with the help of hydrothermally synthesized titanium dioxide nanorods. The foams can be easily wetted by both oil and water. The water prewetted foams are superhydrophilic and superoleophobic under oil–water mixtures, meanwhile the oil prewetted foams are superoleophilic and superhydrophobic. In this paper, many kinds of water–oil mixtures were separated by two foams, prewetted by corresponding oil or water, respectively, combining a straight tee in a high flux, high efficiency, and continuous mode. This research indicates that oil–water mixtures can be separated more eco-friendly and at lower cost
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