16,491 research outputs found
Island formation without attractive interactions
We show that adsorbates on surfaces can form islands even if there are no
attractive interactions. Instead strong repulsion between adsorbates at short
distances can lead to islands, because such islands increase the entropy of the
adsorbates that are not part of the islands. We suggest that this mechanism
cause the observed island formation in O/Pt(111), but it may be important for
many other systems as well.Comment: 11 pages, 4 figure
3D-2D crossover in the naturally layered superconductor (LaSe)1.14(NbSe2)
The temperature and angular dependencies of the resistive upper critical
magnetic field reveal a dimensional crossover of the superconducting
state in the highly anisotropic misfit-layer single crystal of
(LaSe)(NbSe) with the critical temperature of 1.23 K. The
temperature dependence of the upper critical field for
a field orientation along the conducting -planes displays a
characteristic upturn at 1.1 K and below this temperature the angular
dependence of has a cusp around the parallel field orientation. Both
these typical features are observed for the first time in a naturally
crystalline layered system.Comment: 7 pages incl. 3 figure
Phonon-modulated magnetic interactions and spin Tomonaga-Luttinger liquid in the p-orbital antiferromagnet CsO2
The magnetic response of antiferromagnetic CsO2, coming from the p-orbital
S=1/2 spins of anionic O2- molecules, is followed by 133Cs nuclear magnetic
resonance across the structural phase transition occuring at Ts1=61 K on
cooling. Above Ts1, where spins form a square magnetic lattice, we observe a
huge, nonmonotonic temperature dependence of the exchange coupling originating
from thermal librations of O2- molecules. Below Ts1, where antiferromagnetic
spin chains are formed as a result of p-orbital ordering, we observe a spin
Tomonaga-Luttinger-liquid behavior of spin dynamics. These two interesting
phenomena, which provide rare simple manifestations of the coupling between
spin, lattice and orbital degrees of freedom, establish CsO2 as a model system
for molecular solids.Comment: 9 pages, 5 figures (with Supplemental Material), to appear in
Physical Review Letter
One-dimensional quantum antiferromagnetism in the orbital CsO compound revealed by electron paramagnetic resonance
Recently it was proposed that the orbital ordering of molecular
orbitals in the superoxide CsO compound leads to the formation of spin-1/2
chains below the structural phase transition occuring at ~K on
cooling. Here we report a detailed X-band electron paramagnetic resonance (EPR)
study of this phase in CsO powder. The EPR signal appears as a broad line
below , which is replaced by the antiferromagnetic resonance below
the N\'{e}el temperature ~K. The temperature dependence of the
EPR linewidth between and agrees with the
predictions for the one-dimensional Heisenberg antiferromagnetic chain of
spins in the presence of symmetric anisotropic exchange interaction.
Complementary analysis of the EPR lineshape, linewidth and the signal intensity
within the Tomonaga-Luttinger liquid (TLL) framework allows for a determination
of the TLL exponent . Present EPR data thus fully comply with the
quantum antiferromagnetic state of spin-1/2 chains in the orbitally ordered
phase of CsO, which is, therefore, a unique orbital system where such a
state could be studied.Comment: 6 pages, 3 figure
Upper critical field in {BaKBiO}: magnetotransport versus magnetotunneling
Elastic tunneling is used as a powerful direct tool to determine the upper
critical field in the high- oxide BaKBiO. The
temperature dependence of inferred from the tunneling follows the
Werthamer-Helfand-Hohenberg prediction for type-II superconductors. A
comparison will be made with resistively determined critical field data.Comment: 4 pages incl. 5 figure
Magnetic excitations and phonons in the spin-chain compound NaCu2O2
We report an inelastic light scattering study of single-crystalline
NaCuO, a spin-chain compound known to exhibit a phase with helical
magnetic order at low temperatures. Phonon excitations were studied as a
function of temperature and light polarization, and the phonon frequencies are
compared to the results of ab-initio lattice dynamical calculations, which are
also reported here. The good agreement between the observed and calculated
modes allows an assignment of the phonon eigenvectors. Two distinct high-energy
two-magnon features as well as a sharp low-energy one-magnon peak were also
observed. These features are discussed in terms of the magnon modes expected in
a helically ordered state. Their polarization dependence provides evidence of
substantial exchange interactions between two closely spaced spin chains within
a unit cell. At high temperatures, the spectral features attributable to
magnetic excitations are replaced by a broad, quasielastic mode due to
overdamped spin excitations
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