Complex non-equilibrium dynamics in plasmas

Two new forms of strongly coupled plasmas will be discussed. They have become possible to create and observe in the laboratory only recently and exhibit a wealth of intriguing complex behavior which can be studied, in many cases for the first time, experimentally. Plasmas, gases of charged particles, are universal in the sense that certain properties of complex behavior do only depend on ratios of characteristic parameters of the plasma, not on the parameters themselves. Therefore, it is of fundamental and far reaching consequence, to be able to create and observe a strongly coupled plasma since its behavior is paradigmatic for an entire class of plasmas.Comment: 14 pages, to be published in European Revie

Attosecond light pulse induced photo-association

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before, typically with an attosecond pump pulse at an atomic center different from the one of photo-association. We will show that the electron absorption is maximal for a certain delay between the pulses. Two ways of enhancing and controlling stimulated photo-association are proposed, namely using an additional infrared pulse to steer the electronic wave packet and using a train of attosecond pulses instead of a single pair. A direct application of ultrafast stimulated photo-association is the measurement of atomic distances.Comment: 7 pages, 8 figure

Floquet approach for dynamics in short and intense laser pulses

We present a two-timescale Floquet method that allows one to apply the Kramers-Henneberger approach to short pulses and arbitrary laser frequencies. An efficient numerical procedure to propagate the Floquet Hamiltonian is provided that relies on the Toeplitz matrix formalism and Fast Fourier Transformations. It enables efficient time propagation with large Floquet expansions, while still taking advantage of the cycle-averaged Kramers-Henneberger basis. Three illustrative cases of ionization with different photon energies are analyzed, where the envelope of a short and intense pulse is crucial to the underlying dynamics.Comment: 39 pages, 11 figure

Polyatomic trilobite Rydberg molecules in a dense random gas

Trilobites are exotic giant dimers with enormous dipole moments. They consist of a Rydberg atom and a distant ground-state atom bound together by short-range electron-neutral attraction. We show that highly polar, polyatomic trilobite states unexpectedly persist and thrive in a dense ultracold gas of randomly positioned atoms. This is caused by perturbation-induced quantum scarring and the localization of electron density on randomly occurring atom clusters. At certain densities these states also mix with a s-state, overcoming selection rules that hinder the photoassociation of ordinary trilobites

Polyatomic trilobite Rydberg molecules in a dense random gas

Trilobites are exotic giant dimers with enormous dipole moments. They consist of a Rydberg atom and a distant ground-state atom bound together by short-range electron-neutral attraction. We show that highly polar, polyatomic trilobite states unexpectedly persist and thrive in a dense ultracold gas of randomly positioned atoms. This is caused by perturbation-induced quantum scarring and the localization of electron density on randomly occurring atom clusters. At certain densities these states also mix with a s-state, overcoming selection rules that hinder the photoassociation of ordinary trilobites

Proton ejection from molecular hydride clusters exposed to strong X-ray pulses

Clusters consisting of small molecules containing hydrogen do eject fast protons when illuminated by short X-ray pulses. A suitable overall charging of the cluster controlled by the X-ray intensity induces electron migration from the surface to the bulk leading to efficient segregation of the protons and to a globally hindered explosion of the heavy atoms even outside the screened volume. We investigate this peculiar effect systematically along the iso-electronic sequence of methane over ammonia and water to the atomic limit of neon as a reference. In contrast to core-shell systems where the outer shell is sacrificed to reduce radiation damage, the intricate proton dynamics of hydride clusters allows one to keep the entire backbone of heavy atoms intact.Comment: 5 pages, 5 figure

Break-up of Rydberg superatoms via dipole-dipole interactions

We investigate resonant dipole-dipole interactions between two "superatoms" of different angular momentum, consisting of two Rydberg-blockaded atom clouds where each of them carries initially a coherently shared single excitation. We demonstrate that the dipole-dipole interaction breaks up the superatoms by removing the excitations from the clouds. The dynamics is akin to an ensemble average over systems where only one atom per cloud participates in entangled motion and excitation transfer. Our findings should thus facilitate the experimental realization of adiabatic exciton transport in Rydberg systems by replacing single sites with atom clouds.Comment: 10 pages, 5 figure

Non-adiabatic molecular association in thermal gases driven by radio-frequency pulses

The molecular association process in a thermal gas of $^{85}$Rb is investigated where the effects of the envelope of the radio-frequency field are taken into account. For experimentally relevant parameters our analysis shows that with increasing pulse length the corresponding molecular conversion efficiency exhibits low-frequency interference fringes which are robust under thermal averaging over a wide range of temperatures. This dynamical interference phenomenon is attributed to St\"uckelberg phase accumulation between the low-energy continuum states and the dressed molecular state which exhibits a shift proportional to the envelope of the radio-frequency pulse intensity.Comment: 5 pages, 3 figure