Coherent Population Trapping of Single Spins in Diamond Under Optical Excitation

Coherent population trapping is demonstrated in single nitrogen-vacancy centers in diamond under optical excitation. For sufficient excitation power, the fluorescence intensity drops almost to the background level when the laser modulation frequency matches the 2.88 GHz splitting of the ground states. The results are well described theoretically by a four-level model, allowing the relative transition strengths to be determined for individual centers. The results show that all-optical control of single spins is possible in diamond.Comment: minor correction

Coherence properties of a single dipole emitter in diamond

On-demand, high repetition rate sources of indistinguishable, polarised single photons are the key component for future photonic quantum technologies. Colour centres in diamond offer a promising solution, and the narrow line-width of the recently identified nickel-based NE8 centre makes it particularly appealing for realising the transform-limited sources necessary for quantum interference. Here we report the characterisation of dipole orientation and coherence properties of a single NE8 colour centre in a diamond nanocrystal at room-temperature. We observe a single photon coherence time of 0.21 ps and an emission lifetime of 1.5 ns. Combined with an emission wavelength that is ideally suited for applications in existing quantum optical systems, these results show that the NE8 is a far more promising source than the more commonly studied nitrogen-vacancy centre and point the way to the realisation of a practical diamond colour centre-based single photon source.Comment: 10 pages, 4 colour figure

Science results from the imaging Fourier transform spectrometer SpIOMM

SpIOMM is an imaging Fourier transform spectrometer designed to obtain the visible range (350 to 850 nm) spectrum of every light source in a circular field of view of 12 arcminutes in diameter. It is attached to the 1.6-m telescope of the Observatoire du Mont Megantic in southern Quebec. We present here some results of three successful observing runs in 2007, which highlight SpIOMMs capabilities to map emission line objects over a very wide field of view and a broad spectral range. In particular, we discuss data cubes from the planetary nebula M27, the supernova remnants NGC 6992 and M1, the barred spiral galaxy NGC7479, as well as Stephans quintet, an interacting group of galaxies.Comment: 10 pages, 7 figures, to appear in "Ground-based and Airborne Instrumentation for Astronomy II", SPIE conference, Marseille, 23-28 June 200

Room temperature coherent control of coupled single spins in solid

Coherent coupling between single quantum objects is at the heart of modern quantum physics. When coupling is strong enough to prevail over decoherence, it can be used for the engineering of correlated quantum states. Especially for solid-state systems, control of quantum correlations has attracted widespread attention because of applications in quantum computing. Such coherent coupling has been demonstrated in a variety of systems at low temperature1, 2. Of all quantum systems, spins are potentially the most important, because they offer very long phase memories, sometimes even at room temperature. Although precise control of spins is well established in conventional magnetic resonance3, 4, existing techniques usually do not allow the readout of single spins because of limited sensitivity. In this paper, we explore dipolar magnetic coupling between two single defects in diamond (nitrogen-vacancy and nitrogen) using optical readout of the single nitrogen-vacancy spin states. Long phase memory combined with a defect separation of a few lattice spacings allow us to explore the strong magnetic coupling regime. As the two-defect system was well-isolated from other defects, the long phase memory times of the single spins was not diminished, despite the fact that dipolar interactions are usually seen as undesirable sources of decoherence. A coherent superposition of spin pair quantum states was achieved. The dipolar coupling was used to transfer spin polarisation from a nitrogen-vacancy centre spin to a nitrogen spin, with optical pumping of a nitrogen-vacancy centre leading to efficient initialisation. At the level anticrossing efficient nuclear spin polarisation was achieved. Our results demonstrate an important step towards controlled spin coupling and multi-particle entanglement in the solid state

The cavity ring-down spectroscopy of C₂ in a diamond forming microwave plasma

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CVD-diamond Raman laser

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573 nm external cavity CVD-diamond Raman laser

We report an external cavity Raman laser based on a single diamond crystal grown by chemical vapour deposition. When pumped with 10ns pulses of 532nm, output pulse energies up to 0.2 mJ were obtained at 573 nm with a slope efficiency of conversion of 18%.1 page(s

Optical engineering of diamond

This is the first comprehensive book on the engineering of diamond optical devices. It will give readers an up-to-date account of the properties of optical quality synthetic diamond (single crystal, nanodiamond and polycrystalline) and reviews the large and growing field of engineering of diamond-based optical devices, with applications in quantum computation, nano-imaging, high performance lasers, and biomedicine. It aims to provide scientists, engineers and physicists with a valuable resource and reference book for the design and performance of diamond-based optical devices.520 page(s

CVD-diamond external cavity Raman laser at 573 nm

Recent progress in diamond growth via chemical vapor deposition (CVD) has enabled the manufacture of single crystal samples of sufficient size and quality for realizing Raman laser devices. Here we report an external cavity CVD-diamond Raman laser pumped by a Q-switched 532 nm laser. In the investigated configuration, the dominant output coupling was by reflection loss at the diamond's uncoated Brewster angle facets caused by the crystal’s inherent birefringence. Output pulses of wavelength 573 nm with a combined energy of 0.3 mJ were obtained with a slope efficiency of conversion of up to 22%.6 page(s